scholarly journals Saharan dust contribution to the Caribbean summertime boundary layer – A lidar study during SALTRACE

Author(s):  
Silke Groß ◽  
Josef Gasteiger ◽  
Volker Freudenthaler ◽  
Thomas Müller ◽  
Daniel Sauer ◽  
...  

Abstract. Dual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high accurate measurements of the linear depolarization ratio down to about 150–200 m above ground level, the dust volume fraction and the dust mass concentration within the Caribbean boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information of the boundary layer height and the meteorological situation within the boundary layer. We investigate the lidar derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find over all mean values and mean uncertainties of 0.04 ± 0.03 and 0.05 ± 0.04 at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and 26 ± 5 sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the Caribbean boundary layer we find that most values are between 20 and 50 g/m3, and that on most days the dust contribution to total aerosol volume is about 30–40 %. Comparing the dust contribution to the columnintegrated sun-photometer measurements we see a correlation of high dust contribution, high total aerosol optical depth and a corresponding low Angström exponent, and of low dust contribution with low total aerosol optical depth and corresponding high Angström exponent. The relative humidity within the boundary layer was high with values around 80 % on most of the days.

2020 ◽  
Vol 13 (2) ◽  
pp. 893-905 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  

Abstract. A new method, called ElEx (elastic extinction), is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. ElEx uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are also taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. In this study, ElEx was applied in an aerosol mixture of marine and dust particles at Finokalia station during the CHARADMExp campaign. Any difference between ElEx and Raman extinction profiles indicates that the nondust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun photometer aerosol optical depth observations is performed as well during daytime. Differences in the total aerosol optical depth are varying between 1.2 % and 72 %, and these differences are attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to the overlap problem.


2016 ◽  
Vol 16 (18) ◽  
pp. 11535-11546 ◽  
Author(s):  
Silke Groß ◽  
Josef Gasteiger ◽  
Volker Freudenthaler ◽  
Thomas Müller ◽  
Daniel Sauer ◽  
...  

Abstract. Dual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high-accuracy measurements of the linear depolarization ratio down to about 200 m above ground level, the dust volume fraction and the dust mass concentration within the convective marine boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information on the convective marine boundary layer height and the meteorological situation within the convective marine boundary layer. We investigate the lidar-derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find mean values of 0.04 (SD 0.03) and 0.05 (SD 0.04) at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and (26 ± 5) sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the convective marine boundary layer we find that most values were between 20 and 50 µgm−3. On most days the dust contribution to total aerosol volume was about 30–40 %. Comparing the dust contribution to the column-integrated sun-photometer measurements we see a correlation between high dust contribution, high total aerosol optical depth and a low Angström exponent, and of low dust contribution with low total aerosol optical depth.


2019 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  

Abstract. In this study we estimate the particle extinction profiles at Finokalia, Crete, using only the information provided by the elastic and polarization channels of a PollyXT lidar system. Most of the time Finokalia site is affected by only two aerosol types, i.e. marine and dust particles. These two aerosol types, having different optical properties, permit the separation of aerosol mixture. The proposed method uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. Any difference between the proposed methodology and Raman extinction profiles indicates that the non-dust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun-photometric aerosol optical depth observations is performed as well during daytime with reasonable differences between the two instruments. Differences in the total aerosol optical depth is attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to overlap problem.


2021 ◽  
Author(s):  
Mariana Adam ◽  
Iwona S. Stachlewska ◽  
Lucia Mona ◽  
Nikolaos Papagiannopoulos ◽  
Juan Antonio Bravo-Aranda ◽  
...  

Abstract. Biomass burning episodes measured at 14 stations of the European Aerosol Research Lidar Network (EARLINET) over 2008–2017 were analysed using the methodology described in "Biomass burning events measured by lidars in EARLINET – Part 1: Data analysis methodology" (Adam et al., 2020, this issue). The smoke layers were identified in lidar optical properties profiles. A number of 795 layers for which we measured at least one intensive parameter was analysed. These layers were geographically distributed as follows: 399 layers observed in South-East Europe, 119 layers observed in South-West Europe, 243 layers observed in North-East Europe, and 34 layers observed in Central Europe. The mean layer intensive parameters are discussed following two research directions: (I) the long-range transport of smoke particles from North America, and (II) the smoke properties (fresh versus aged), separating the smoke events into four continental source regions (European, North American, African, Asian or a mixture of two), based on back trajectory analysis. The smoke detected in Central Europe (Cabauw, Leipzig, and Hohenpeißenberg) was mostly transported from North America (87 % of fires). In North-East Europe (Belsk, Minsk, Warsaw) smoke advected mostly from Eastern Europe (Ukraine and Russia), but there was a significant contribution (31 %) from North America. In South-West Europe (Barcelona, Evora, Granada) smoke originated mainly from the Iberian Peninsula and North Africa (while 9 % were originating in North America). In the South-East Europe (Athens, Bucharest, Potenza, Sofia, Thessaloniki) the origin of the smoke was mostly local (only 3 % represented North America smoke). The following features, correlated with the increased smoke travel time (corresponding to aging) were found: the colour ratio of the lidar ratio (i.e., the ratio of the lidar ratio at 532 nm to the lidar ratio at 355 nm) and the colour ratio of the backscatter Ångström exponent (i.e., the ratio of the backscatter-related Angstrom exponent for the pair 532 nm – 1064 nm to the one for the pair 355 nm – 532 nm) increase, while the extinction Ångström exponent and the colour ratio of the particle depolarization ratio (i.e., the ratio of the particle linear depolarization ratio at 532 nm to the particle depolarization ratio at 355 nm) decrease. The smoke originating from all continental regions can be characterized on average as aged smoke, with a very few exceptions. In general, the long range transported smoke shows higher lidar ratio and lower depolarization ratio compared to the local smoke.


2011 ◽  
Vol 11 (4) ◽  
pp. 12763-12803 ◽  
Author(s):  
L. Mona ◽  
A. Amodeo ◽  
G. D'Amico ◽  
A. Giunta ◽  
F. Madonna ◽  
...  

Abstract. Multi-wavelength Raman lidar measurements were performed at CNR-IMAA Atmospheric Observatory (CIAO) during the entire Eyjafjallajökull explosive eruptive period in April–May 2010, whenever weather conditions permitted. A methodology for volcanic layer identification and accurate aerosol typing has been developed on the basis both of the multi-wavelength Raman lidar measurements and EARLINET measurements performed at CIAO since 2000. The aerosol mask for lidar measurements performed at CIAO during the 2010 Eyjafjallajökull eruption has been obtained. Volcanic aerosol layers have been observed in different periods: 19–22 April, 27–29 April, 8–9 May, 13–14 May and 18–19 May. A maximum aerosol optical depth of about 0.12–0.13 was observed on 20 April, 22:00 UTC and 13 May, 20:30 UTC. Volcanic particles have been detected both at low altitudes, in the free troposphere and in the upper troposphere. Intrusions into the PBL have been revealed on 21–22 April and 13 May. In the April–May period Saharan dust intrusions typically occur in Southern Italy. For the period under investigations, a Saharan dust intrusion was observed on 13–14 May: dust and volcanic particles have been simultaneously observed at CIAO both at separated different levels and mixed within the same layer. Lidar ratios at 355 and 532 nm, Ångström exponent at 355/532 nm, backscatter related Ångström exponent at 532/1064 nm and particle linear depolarization ratio at 532 nm measured inside the detected volcanic layers have been discussed. The dependence of these quantities on relative humidity (RH) has been investigated by using co-located microwave profiler measurements. The particle linear depolarization ratio increasing with RH, lidar ratio values at 355 nm around 80 sr, and values of the ratio of lidar ratios greater than 1 suggest the presence of sulfates mixed with continental aerosol. Lower lidar ratio values (around 40 sr) increasing with RH and values of the ratio of lidar ratios lower than 1 indicate the presence of some aged ash inside these sulfate layers.


2013 ◽  
Vol 6 (10) ◽  
pp. 2659-2669 ◽  
Author(s):  
A. Bayat ◽  
H. R. Khalesifard ◽  
A. Masoumi

Abstract. The polarized phase function of atmospheric aerosols has been investigated for the atmosphere of Zanjan, a city in northwest Iran. To do this, aerosol optical depth, Ångström exponent, single-scattering albedo, and polarized phase function have been retrieved from the measurements of a Cimel CE 318-2 polarized sun-photometer from February 2010 to December 2012. The results show that the maximum value of aerosol polarized phase function as well as the polarized phase function retrieved for a specific scattering angle (i.e., 60°) are strongly correlated (R = 0.95 and 0.95, respectively) with the Ångström exponent. The latter has a meaningful variation with respect to the changes in the complex refractive index of the atmospheric aerosols. Furthermore the polarized phase function shows a moderate negative correlation with respect to the atmospheric aerosol optical depth and single-scattering albedo (R = −0.76 and −0.33, respectively). Therefore the polarized phase function can be regarded as a key parameter to characterize the atmospheric particles of the region – a populated city in the semi-arid area and surrounded by some dust sources of the Earth's dust belt.


2006 ◽  
Vol 6 (3) ◽  
pp. 697-713 ◽  
Author(s):  
G. Pace ◽  
A. di Sarra ◽  
D. Meloni ◽  
S. Piacentino ◽  
P. Chamard

Abstract. Aerosol optical depth and Ångström exponent were obtained from multi filter rotating shadowband radiometer (MFRSR) observations carried out at the island of Lampedusa, in the Central Mediterranean, in the period July 2001–September 2003. The average aerosol optical depth at 495.7 nm, τ, is 0.24±0.14; the average Ångström exponent, α, is 0.86±0.63. The observed values of τ range from 0.03 to 1.13, and the values of α vary from −0.32 to 2.05, indicating a large variability in aerosol content and size. In cloud-free conditions, 36% of the airmasses come from Africa, 25% from Central-Eastern Europe, and 19% from Western France, Spain and the North Atlantic. In summer, 42% of the airmasses is of African origin. In almost all cases African aerosols display high values of τ and low values of α, typical of Saharan dust (average values of τ and α are 0.36 and 0.42, respectively). Particles originating from Central-Eastern Europe show relatively large average values of τ and α (0.23 and 1.5, respectively), while particles from Western France, Spain and the North Atlantic show the lowest average values of τ (0.15), and relatively small values of α (0.92). Intermediate values of α are often connected with relatively fast changes of the airmass originating sector, suggesting the contemporary presence of different types of particles in the air column. Clean marine conditions are rare at Lampedusa, and are generally associated with subsidence of the airmasses reaching the island. Average values of τ and α for clean marine conditions are 0.11 and 0.86, respectively. The largest values of α (about 2) were observed in August 2003, when large scale forest fires in Southern Europe produced consistent amounts of fine combustion particles, that were transported to the Central Mediterranean by a persistent high pressure system over Central Europe. Smoke particles in some cases mix with desert dust, producing intermediate values of α. The seasonal distribution of the meteorological patterns over the Mediterranean, the efficiency of the aerosol production mechanisms, and the variability of the particles' residence time produce a distinct seasonal cycle of aerosol optical depths and Ångström exponent values. Particles originating from all sectors show a summer maximum in aerosol optical depth. The summer increase in optical depth for European aerosols is linked with an increment in the values of α, that indicates an enhancement in the number of fine particles. The summer maximum of τ for African particles is associated with a weak reduction in the Ångström exponent, suggesting an increase in the total number of particles and a relatively more intense transport of large particles. The observations were classified according to the aerosol optical properties, and two main classes have been identified: desert dust and biomass burning/urban-industrial aerosols. Values of τ and α averaged over the whole observing period are 0.37 and 0.15 for desert dust, and 0.27 and 1.77 for urban-industrial/biomass burning aerosols.


2019 ◽  
Vol 99 ◽  
pp. 01003
Author(s):  
Athina Avgousta Floutsi ◽  
Marios Bruno Korras Carraca ◽  
Christos Matsoukas ◽  
Nikos Hatzianastassiou ◽  
George Biskos

Central and South Asia are regions of particular interest for studying atmospheric aerosols, being among the largest sources of desert dust aerosols globally. In this study we use the newest collection (C061) of MODIS - Aqua aerosol optical depth (AOD) at 550 nm and Ångström exponent (a) at 412/470 nm over the 15-year period between 2002 and 2017, providing the longest analyzed dataset for this region. According to our results, during spring and summer, high aerosol load (AOD up to 1.2) consisting of coarse desert dust particles, as indicated by a values as low as 0.15, is observed over the Taklamakan, Thar and Registan deserts and the region between the Aral and Caspian seas. The dust load is much lower during winter and autumn (lower AOD and higher a values compared to the other seasons). The interannual variation of AOD and a suggests that the dust load exhibits large decreasing trends (AOD slopes down to -0.22, a slopes up to 0.47 decade-1) over the Thar desert and large increasing trends between the Aral and Caspian seas (AOD and a slopes up to 0.23 decade-1 and down to -0.61 decade-1, respectively.) The AOD data are evaluated against AERONET surface-based measurements. Generally, MODIS and AERONET data are in good agreement with a correlation coefficient (R) equal to 0.835.


2017 ◽  
Author(s):  
Julian Hofer ◽  
Dietrich Althausen ◽  
Sabur F. Abdullaev ◽  
Abduvosit N. Makhmudov ◽  
Bakhron I. Nazarov ◽  
...  

Abstract. For the first time, continuous vertically resolved aerosol measurements were performed by lidar in Tajikistan, Central Asia. Observations with the multiwavelength polarization/Raman lidar PollyXT were conducted during CADEX (Central Asian Dust EXperiment) in Dushanbe, Tajikistan, from March 2015 to August 2016. Co-located with the lidar a sun photometer was operated. The goal of CADEX is to provide an unprecedented data set on vertically resolved aerosol optical properties in Central Asia, an area highly affected by climate change but largely missing vertically resolved aerosol measurements. During the 18-months measurement campaign, mineral dust was detected frequently from ground to cirrus level height. In this study, an overview of the measurement period is given and four typical but different example measurement cases are discussed in detail. Three of them are dust cases and one is a contrasting pollution aerosol case. Vertical profiles of the measured optical properties and the calculated dust and non-dust mass concentrations are presented. Dust source regions were identified by means of backward trajectory analyses. A lofted layer of Middle Eastern dust with an aerosol optical thickness (AOT) of 0.4 and an extinction-related Ångström exponent of 0.41 was measured. In comparison, two near-ground dust cases have Central Asian sources. One is an extreme dust event with an AOT of 1.5 and Ångström exponent of 0.12 and the other one is a most extreme dust event with an AOT of above 4 (measured by sun photometer) and an Ångström exponent of −0.08. The observed lidar ratios (particle linear depolarization ratios) in the presented dust cases range from 40.3 sr to 46.9 sr (0.18–0.29) at 355 nm and from 35.7 sr to 42.9 sr (0.31–0.35) at 532 nm wavelength. The particle linear depolarization ratios indicate almost unpolluted dust in the case of a lofted dust layer and pure dust in the near-ground dust cases. The lidar ratio values are lower than typical lidar ratio values for Saharan dust (50–60 sr) and comparable to Middle Eastern/West-Asian dust lidar ratios (35–45 sr). In contrast, the presented case of pollution aerosol of local origin has an Ångström exponent of 2.07 and a lidar ratio (particle linear depolarization ratio) of 55.8 sr (0.03) at 355 nm and 32.8 sr (0.08) at 532 nm wavelength.


Atmosphere ◽  
2019 ◽  
Vol 10 (9) ◽  
pp. 482 ◽  
Author(s):  
Victor Nicolae ◽  
Camelia Talianu ◽  
Simona Andrei ◽  
Bogdan Antonescu ◽  
Dragoș Ene ◽  
...  

In this study, AERONET (Aerosol Robotic Network) and EARLINET (European Aerosol Research Lidar Network) data from 17 collocated lidar and sun photometer stations were used to characterize the optical properties of aerosol and their types for the 2008–2018 period in various regions of Europe. The analysis was done on six cluster domains defined using circulation types around each station and their common circulation features. As concluded from the lidar photometer measurements, the typical aerosol particles observed during 2008–2018 over Europe were medium-sized, medium absorbing particles with low spectral dependence. The highest mean values for the lidar ratio at 532 nm were recorded over Northeastern Europe and were associated with Smoke particles, while the lowest mean values for the Angstrom exponent were identified over the Southwest cluster and were associated with Dust and Marine particles. Smoke (37%) and Continental (25%) aerosol types were the predominant aerosol types in Europe, followed by Continental Polluted (17%), Dust (10%), and Marine/Cloud (10%) types. The seasonal variability was insignificant at the continental scale, showing a small increase in the percentage of Smoke during spring and a small increase of Dust during autumn. The aerosol optical depth (AOD) slightly decreased with time, while the Angstrom exponent oscillated between “hot and smoky” years (2011–2015) on the one hand and “dusty” years (2008–2010) and “wet” years (2017–2018) on the other hand. The high variability from year to year showed that aerosol transport in the troposphere became more and more important in the overall balance of the columnar aerosol load.


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