scholarly journals The potential of elastic and polarization lidars to retrieve extinction profiles

2020 ◽  
Vol 13 (2) ◽  
pp. 893-905 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  

Abstract. A new method, called ElEx (elastic extinction), is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. ElEx uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are also taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. In this study, ElEx was applied in an aerosol mixture of marine and dust particles at Finokalia station during the CHARADMExp campaign. Any difference between ElEx and Raman extinction profiles indicates that the nondust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun photometer aerosol optical depth observations is performed as well during daytime. Differences in the total aerosol optical depth are varying between 1.2 % and 72 %, and these differences are attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to the overlap problem.

2019 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  

Abstract. In this study we estimate the particle extinction profiles at Finokalia, Crete, using only the information provided by the elastic and polarization channels of a PollyXT lidar system. Most of the time Finokalia site is affected by only two aerosol types, i.e. marine and dust particles. These two aerosol types, having different optical properties, permit the separation of aerosol mixture. The proposed method uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. Any difference between the proposed methodology and Raman extinction profiles indicates that the non-dust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun-photometric aerosol optical depth observations is performed as well during daytime with reasonable differences between the two instruments. Differences in the total aerosol optical depth is attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to overlap problem.


2016 ◽  
Author(s):  
Silke Groß ◽  
Josef Gasteiger ◽  
Volker Freudenthaler ◽  
Thomas Müller ◽  
Daniel Sauer ◽  
...  

Abstract. Dual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high accurate measurements of the linear depolarization ratio down to about 150–200 m above ground level, the dust volume fraction and the dust mass concentration within the Caribbean boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information of the boundary layer height and the meteorological situation within the boundary layer. We investigate the lidar derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find over all mean values and mean uncertainties of 0.04 ± 0.03 and 0.05 ± 0.04 at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and 26 ± 5 sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the Caribbean boundary layer we find that most values are between 20 and 50 g/m3, and that on most days the dust contribution to total aerosol volume is about 30–40 %. Comparing the dust contribution to the columnintegrated sun-photometer measurements we see a correlation of high dust contribution, high total aerosol optical depth and a corresponding low Angström exponent, and of low dust contribution with low total aerosol optical depth and corresponding high Angström exponent. The relative humidity within the boundary layer was high with values around 80 % on most of the days.


2020 ◽  
Vol 237 ◽  
pp. 02036
Author(s):  
Moritz Haarig ◽  
Holger Baars ◽  
Albert Ansmann ◽  
Ronny Engelmann ◽  
Kevin Ohneiser ◽  
...  

Canadian wildfire smoke was detected in the troposphere and lower stratosphere over Europe in August and September 2017. Lidar measurements from various stations of the European Aerosol Research Lidar Network (EARLINET) observed the stratospheric smoke layer. Triple-wavelength (355, 532, and 1064 nm) lidar measurements of the depolarization and the lidar ratio are reported from Leipzig, Germany. The particle linear depolarization ratio of the wildfire smoke in the stratosphere had an exceptional strong wavelength dependence reaching from 0.22 at 355 nm, to 0.18 at 532 nm, and 0.04 at 1064 nm. The lidar ratio increased with wavelength from 40±16 sr at 355 nm, to 66±12 sr at 532 nm, and 92±27 sr at 1064 nm. The development of the stratospheric smoke plume over several months was studied by long-term lidar measurements in Cyprus. The stratospheric smoke layers increased in altitude up to 24 km height.


2016 ◽  
Vol 16 (18) ◽  
pp. 11535-11546 ◽  
Author(s):  
Silke Groß ◽  
Josef Gasteiger ◽  
Volker Freudenthaler ◽  
Thomas Müller ◽  
Daniel Sauer ◽  
...  

Abstract. Dual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high-accuracy measurements of the linear depolarization ratio down to about 200 m above ground level, the dust volume fraction and the dust mass concentration within the convective marine boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information on the convective marine boundary layer height and the meteorological situation within the convective marine boundary layer. We investigate the lidar-derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find mean values of 0.04 (SD 0.03) and 0.05 (SD 0.04) at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and (26 ± 5) sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the convective marine boundary layer we find that most values were between 20 and 50 µgm−3. On most days the dust contribution to total aerosol volume was about 30–40 %. Comparing the dust contribution to the column-integrated sun-photometer measurements we see a correlation between high dust contribution, high total aerosol optical depth and a low Angström exponent, and of low dust contribution with low total aerosol optical depth.


2011 ◽  
Vol 11 (4) ◽  
pp. 12763-12803 ◽  
Author(s):  
L. Mona ◽  
A. Amodeo ◽  
G. D'Amico ◽  
A. Giunta ◽  
F. Madonna ◽  
...  

Abstract. Multi-wavelength Raman lidar measurements were performed at CNR-IMAA Atmospheric Observatory (CIAO) during the entire Eyjafjallajökull explosive eruptive period in April–May 2010, whenever weather conditions permitted. A methodology for volcanic layer identification and accurate aerosol typing has been developed on the basis both of the multi-wavelength Raman lidar measurements and EARLINET measurements performed at CIAO since 2000. The aerosol mask for lidar measurements performed at CIAO during the 2010 Eyjafjallajökull eruption has been obtained. Volcanic aerosol layers have been observed in different periods: 19–22 April, 27–29 April, 8–9 May, 13–14 May and 18–19 May. A maximum aerosol optical depth of about 0.12–0.13 was observed on 20 April, 22:00 UTC and 13 May, 20:30 UTC. Volcanic particles have been detected both at low altitudes, in the free troposphere and in the upper troposphere. Intrusions into the PBL have been revealed on 21–22 April and 13 May. In the April–May period Saharan dust intrusions typically occur in Southern Italy. For the period under investigations, a Saharan dust intrusion was observed on 13–14 May: dust and volcanic particles have been simultaneously observed at CIAO both at separated different levels and mixed within the same layer. Lidar ratios at 355 and 532 nm, Ångström exponent at 355/532 nm, backscatter related Ångström exponent at 532/1064 nm and particle linear depolarization ratio at 532 nm measured inside the detected volcanic layers have been discussed. The dependence of these quantities on relative humidity (RH) has been investigated by using co-located microwave profiler measurements. The particle linear depolarization ratio increasing with RH, lidar ratio values at 355 nm around 80 sr, and values of the ratio of lidar ratios greater than 1 suggest the presence of sulfates mixed with continental aerosol. Lower lidar ratio values (around 40 sr) increasing with RH and values of the ratio of lidar ratios lower than 1 indicate the presence of some aged ash inside these sulfate layers.


2021 ◽  
Author(s):  
Hengheng Zhang ◽  
Frank Wagner ◽  
Harald Saathoff ◽  
Heike Vogel ◽  
Gholam Ali Hoshyaripour ◽  
...  

Abstract. The evolution and the properties of a Saharan dust plume were studied near the city of Karlsruhe in south-west Germany (8.4298° E, 49.0953° N) from April 7 to 9, 2018 combining a scanning LIDAR (90°, 30°), a vertical LIDAR (90°), a sun photometer, and the transport model ICON-ART. The LIDAR measurements show that the dust particles had backscatter coefficients of 0.86 ± 0.14 Mm−1 Sr−1, an extinction coefficient of 40 ± 0.8 Mm−1, a LIDAR ratio of 46 ± 5 sr, and a particle depolarization ratio of 0.33 ± 0.07. These values are in good agreement with those obtained in previous studies of Saharan dust plumes in Western Europe. Compared to the remote sensing measurements, the model simulation predicts the plume arrival time, its layer height, and structure very well but overestimates the backscatter coefficient. In this manuscript, we discuss the complementarity and advantages of the different measurement methods as well model simulations to predict Saharan dust plumes. Main conclusions are that the ICON-ART model can predict the structure of Saharan dust plumes very well but overestimates the backscatter coefficients by a factor of 2.2 ± 0.16 at 355 nm and underestimates the aerosol optical depth (AOD) by a factor of 1.5 ± 0.11 at 340 nm for this Saharan dust plume event. Employing a scanning aerosol LIDAR allows determining backscatter coefficient, particle depolarization ratio and especially LIDAR ratio of Saharan dust both for daytime and nighttime independently. Combining LIDAR with sun photometer data allows constraining aerosol optical depth in different ways and determining column integrated LIDAR ratios. These comprehensive datasets allow for a better understanding of Saharan dust plumes in Western Europe.


2016 ◽  
Author(s):  
Josef Gasteiger ◽  
Silke Groß ◽  
Bernadett Weinzierl ◽  
Daniel Sauer ◽  
Volker Freudenthaler

Abstract. Long-range transport of aerosol in the Saharan Air Layer (SAL) across the Atlantic plays an important role for weather, climate, and ocean fertilization. However, processes occurring within the SAL and their effects on aerosol properties are still unclear. In this work we study particle settling and convective mixing within the SAL based on measured and modeled vertical aerosol profiles in the upper 1 km of the transported SAL. We use ground-based POLIS lidar measurements and airborne particle counter measurements over the Western Atlantic, as well as space-based CALIOP lidar measurements from Africa to the Western Atlantic. In our model we take account of the optical properties and the Stokes gravitational settling of irregularly-shaped Saharan dust particles. We test two hypotheses about the occurrence of convective mixing within the SAL over the Atlantic to explain the aerosol properties observed by the lidars and the particle counter. Our first hypothesis (H1) assumes that no mixing occurs in the SAL leading to an altitude separation of super-micron dust particles as a result of settling. The second hypothesis (H2) assumes that convective mixing occurs in the SAL during the day allowing large super-micron dust particles to stay airborne longer than without convective mixing. In general, a decrease of the particle linear depolarization ratio towards the SAL top is found in the measured lidar data but the decrease is much weaker than modeled in case of H1. The in-situ data on particle number concentrations show a presence of large particles near the SAL top that is inconsistent with H1. Furthermore, the analysis of the CALIOP measurements reveals that the average vertical profile of the linear depolarization ratio of the aerosols in the upper 1 km of the SAL does not change along its transport path over the Atlantic. These findings indicate H2 to be much more likely than H1, giving evidence that convective mixing occurs within the SAL over the Atlantic with significant consequences for the evolution of the size distribution of the super-micron dust particles during transport.


2020 ◽  
Author(s):  
Qiaoyun Hu ◽  
Haofei Wang ◽  
Philippe Goloub ◽  
Zhengqiang Li ◽  
Igor Veselovskii ◽  
...  

Abstract. The Taklamakan desert is an important dust source for the global atmospheric dust budget and a cause of the dust weather in Eastern Asia. The characterization of the properties and vertical distributions of Taklamakan dust in the source region is still very limited. To fill this gap, the DAO (Dust Aerosol Observation) was conducted in Kashi, China in 2019. Kashi site is about 150 km to the west rim of the Taklamakan desert and is strongly impacted by desert dust aerosols, especially in spring time, i.e. April and May. Apart from dust, fine particles coming from local anthropogenic emissions or/and transported aerosols are also a non-negligible aerosol component. In this study, we provide the first profiling of the 2α + 3β + 3δ lidar profiles of Taklamakan dust based on a multi-wavelength Raman polarization lidar. Four cases, including two Taklamakan dust events (Case 1 and 2) and two polluted dust events (Case 3 and 4) are presented. The lidar ratio in the Taklamakan dust outbreak is found to be 51 ± 8–56 ± 8 sr at 355 nm and 45 ± 7 sr at 532 nm. The particle linear depolarization ratios are about 0.28 ± 0.04–0.32 ± 0.05 at 355 nm, 0.35 ± 0.05 at 532 nm and 0.31 ± 0.05 at 1064 nm. The observed polluted dust is commonly featured with reduced particle linear depolarization ratio and enhanced extinction and backscatter Angstrom exponent. In Case 3, the lidar ratio of polluted dust is about 42 ± 6 sr at 355 nm and 40 ± 6 sr at 532 nm. The particles linear depolarization ratios decrease to about 0.25, with a weak spectral dependence. In Case 4, the variability of lidar ratio and particle linear depolarization ratio is higher than in Case 3, which reflects the complexity of the nature of mixed pollutant and the mixing state. The results provide the first reference for the characteristics of Taklamakan dust measured by Raman lidar. The data could contribute to complementing the dust model and improving the accuracy of climate modeling.


2019 ◽  
Vol 99 ◽  
pp. 02006 ◽  
Author(s):  
Hossein Panahifar ◽  
Hamid Reza Khalesifard

Continuous vertically resolved aerosol measurements using lidar were performed in Tehran, Iran. Lidar results has been used in combination with particulate matter monitoring, synoptic meteorology observa- tion as well as satellite-based measurements. The aerosol types are classified by their optical properties. The volume linear depolarization ratio (VLDR) at 532 nm lies mostly between 0:05-0:10. These results show that mostly urban pollution mixed with particles are present in the atmosphere above Tehran. During dust events, the VLDR at 532 nm lies between 0:20-0:35.


2020 ◽  
Vol 20 (22) ◽  
pp. 14005-14021
Author(s):  
Anna Gialitaki ◽  
Alexandra Tsekeri ◽  
Vassilis Amiridis ◽  
Romain Ceolato ◽  
Lucas Paulien ◽  
...  

Abstract. We examine the capability of near-spherical-shaped particles to reproduce the triple-wavelength particle linear depolarization ratio (PLDR) and lidar ratio (LR) values measured over Europe for stratospheric smoke originating from Canadian wildfires. The smoke layers were detected both in the troposphere and the stratosphere, though in the latter case the particles presented PLDR values of almost 18 % at 532 nm as well as a strong spectral dependence from the UV to the near-IR wavelength. Although recent simulation studies of rather complicated smoke particle morphologies have shown that heavily coated smoke aggregates can produce large PLDR, herein we propose a much simpler model of compact near-spherical smoke particles. This assumption allows for the reproduction of the observed intensive optical properties of stratospheric smoke, as well as their spectral dependence. We further examine whether an extension of the current Aerosol Robotic Network (AERONET) scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke cases associated with enhanced PLDR. Results of our study illustrate the fact that triple-wavelength PLDR and LR lidar measurements can provide us with additional insight when it comes to particle characterization.


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