scholarly journals Retrieval of aerosol single-scattering albedo and polarized phase function from polarized sun-photometer measurements for Zanjan's atmosphere

2013 ◽  
Vol 6 (10) ◽  
pp. 2659-2669 ◽  
Author(s):  
A. Bayat ◽  
H. R. Khalesifard ◽  
A. Masoumi

Abstract. The polarized phase function of atmospheric aerosols has been investigated for the atmosphere of Zanjan, a city in northwest Iran. To do this, aerosol optical depth, Ångström exponent, single-scattering albedo, and polarized phase function have been retrieved from the measurements of a Cimel CE 318-2 polarized sun-photometer from February 2010 to December 2012. The results show that the maximum value of aerosol polarized phase function as well as the polarized phase function retrieved for a specific scattering angle (i.e., 60°) are strongly correlated (R = 0.95 and 0.95, respectively) with the Ångström exponent. The latter has a meaningful variation with respect to the changes in the complex refractive index of the atmospheric aerosols. Furthermore the polarized phase function shows a moderate negative correlation with respect to the atmospheric aerosol optical depth and single-scattering albedo (R = −0.76 and −0.33, respectively). Therefore the polarized phase function can be regarded as a key parameter to characterize the atmospheric particles of the region – a populated city in the semi-arid area and surrounded by some dust sources of the Earth's dust belt.

2013 ◽  
Vol 6 (2) ◽  
pp. 3317-3338 ◽  
Author(s):  
A. Bayat ◽  
H. R. Khalesifard ◽  
A. Masoumi

Abstract. Aerosol optical depth, Ångström exponent, single scattering albedo, and polarized phase function have been retrieved from polarized sun-photometer measurements for atmosphere of Zanjan (36.70° N, 48.51° E, and 1800 m a.m.s.l.) from January 2010 to December 2012. The results show that the maximum value of aerosol polarized phase function as well as the polarized phase function retrieved for a specific scattering angle (i.e. 60°), are strongly correlated with the Ångström exponent. The latter one has a meaningful variations respect to the changes in the complex refractive index of the atmospheric aerosols. Furthermore the polarized phase function shows a moderate negative correlation respect to atmospheric aerosol optical depth and single scattering albedo. Therefore the polarized phase function can be regarded as a key parameter to characterize the atmospheric particles.


2019 ◽  
Vol 99 ◽  
pp. 01003
Author(s):  
Athina Avgousta Floutsi ◽  
Marios Bruno Korras Carraca ◽  
Christos Matsoukas ◽  
Nikos Hatzianastassiou ◽  
George Biskos

Central and South Asia are regions of particular interest for studying atmospheric aerosols, being among the largest sources of desert dust aerosols globally. In this study we use the newest collection (C061) of MODIS - Aqua aerosol optical depth (AOD) at 550 nm and Ångström exponent (a) at 412/470 nm over the 15-year period between 2002 and 2017, providing the longest analyzed dataset for this region. According to our results, during spring and summer, high aerosol load (AOD up to 1.2) consisting of coarse desert dust particles, as indicated by a values as low as 0.15, is observed over the Taklamakan, Thar and Registan deserts and the region between the Aral and Caspian seas. The dust load is much lower during winter and autumn (lower AOD and higher a values compared to the other seasons). The interannual variation of AOD and a suggests that the dust load exhibits large decreasing trends (AOD slopes down to -0.22, a slopes up to 0.47 decade-1) over the Thar desert and large increasing trends between the Aral and Caspian seas (AOD and a slopes up to 0.23 decade-1 and down to -0.61 decade-1, respectively.) The AOD data are evaluated against AERONET surface-based measurements. Generally, MODIS and AERONET data are in good agreement with a correlation coefficient (R) equal to 0.835.


2014 ◽  
Vol 14 (10) ◽  
pp. 14351-14397 ◽  
Author(s):  
J. Li ◽  
B. E. Carlson ◽  
O. Dubovik ◽  
A. A. Lacis

Abstract. The Aerosol Robotic Network (AERONET) has been providing high-quality retrievals of aerosol optical properties from the surface at worldwide locations for more than a decade. Many sites have continuous and consistent records for more than 10 years, which enables the investigation of long-term trends of aerosol properties at these locations. In this study, we present trend analysis of AERONET data at 63 selected locations. In addition to commonly studied parameters such as Aerosol Optical Depth (AOD) and Ångström Exponent (AE), we also focus on Absorption Aerosol Optical Depth (ABS), Scattering Optical Depth (SCT), Single Scattering Albedo (SSA) and the Absorption Ångström Exponent (AAE). Two statistical methods are used to detect and estimate the trend: Mann–Kendall test associated with Sen's slope and linear least square fitting. Their results agree well in terms of the significance of the trend for the majority of the cases. The results indicate that Europe and North America experienced a uniform decrease in AOD and SCT, while significant (> 90%) increases of these two parameters are found for Kanpur, India. Most of European and North American sites also show negative trends for ABS, as well as three East Asian stations. The reduction in ABS results in positive SSA trends for these locations. The increase of SCT also leads to a positive SSA trend for Kanpur. Negative SSA trends are mostly found over South America, Australia and a few West European stations, which are mainly attributed to the increase of absorption. Fewer stations are found with significant trends for AE and AAE. In general, the trends do not exhibit obvious seasonality for the majority of the parameters and stations.


2011 ◽  
Vol 4 (5) ◽  
pp. 857-863 ◽  
Author(s):  
A. Bayat ◽  
A. Masoumi ◽  
H. R. Khalesifard

Abstract. We are reporting the results of ground-based spectroradiometric measurements on aerosols and water vapor in the atmosphere of Zanjan for the period of October 2006 to September 2008 using a CIMEL CE318-2 sun-photometer. Zanjan is a city in Northwest Iran, located at 36.70° N, 48.51° E, and at an altitude of 1800 m a.m.s.l. (above mean sea level). The spectral aerosol optical depth, Ångström exponent, and columnar water vapor have been calculated using the data recorded by the sun-photometer through the direct measurements on the sun radiance (sun-mode). The average values of aerosol optical depth at 440 nm, columnar water vapor, and the Ångström exponent, α, during the mentioned period are measured as, 0.28 ± 0.14, 0.57 ± 0.37 cm and 0.73 ± 0.30, respectively. The maximum (minimum) value of the aerosol optical depth was recorded in May 2007 (November 2007), and that of columnar water vapor, in July 2007 (January 2008). Using the least-squares method, the Ångström exponent was calculated in the spectral interval 440–870 nm along with α1 and α2, the coefficients of a second order polynomial fit to the plotted logarithm of aerosol optical depth versus the logarithm of wavelength. The coefficient α2 shows that most of the aerosols in the Zanjan area have dimensions larger than 1 micron. The calculated values for α2 − α1 indicate that 80 % of the aerosols are in the coarse-mode (>1 μm) and 20 % of them are in the fine-mode (<1 μm). Comparison of α2 − α1 for the atmosphere over Zanjan with other regions indicates dust particles are the most dominant aerosols in the region.


2010 ◽  
Vol 3 (3) ◽  
pp. 2633-2649 ◽  
Author(s):  
A. Bayat ◽  
A. Masoumi ◽  
H. R. Khalesifard

Abstract. We are reporting the results of ground-based spectroradiometric measurements on aerosols and water vapor in the atmosphere of Zanjan for the period of October 2006 to September 2008 using a Cimel CE318-2 sun-photometer. Zanjan is a city in Northwest Iran, located at 36.70° N, 48.51° E, and at an altitude of 1800 above m.s.l. The spectral aerosol optical depth, Ångström exponent, and columnar water vapor have been calculated using the data recorded by the sunphotometer through direct-beam irradiance measurements of sunlight (sun mode). The average values of aerosol optical depth at 440 nm, columnar water vapor, and the Ångström exponent, α, during the mentioned period are measured as, 0.27±0.16, 0.53±0.37 cm and 0.75±0.46, respectively. The maximum (minimum) value of the aerosol optical depth was recorded in May 2007 (January 2007), and that of columnar water vapor, in July 2007 (January 2008). Using the least-squares method, the Ångström exponent was calculated in the spectral interval 440–870 nm along with the coefficients of a second order polynomial fit (α1 and α2) to the log-log plot of aerosol optical depth versus the wavelength. The coefficient α2 shows that most of the aerosols in the Zanjan area have dimensions larger than 1 μm. The values calculated for α2−α1 indicate that 70% of the aerosols are in the coarse-mode (>1 μm) and 30% of them are in the fine-mode (<1 μm). Comparison of α2−α1 for the atmosphere over Zanjan with other regions indicates dust and anthropogenic aerosols are the most dominant aerosols in the region.


2006 ◽  
Vol 6 (3) ◽  
pp. 697-713 ◽  
Author(s):  
G. Pace ◽  
A. di Sarra ◽  
D. Meloni ◽  
S. Piacentino ◽  
P. Chamard

Abstract. Aerosol optical depth and Ångström exponent were obtained from multi filter rotating shadowband radiometer (MFRSR) observations carried out at the island of Lampedusa, in the Central Mediterranean, in the period July 2001–September 2003. The average aerosol optical depth at 495.7 nm, τ, is 0.24±0.14; the average Ångström exponent, α, is 0.86±0.63. The observed values of τ range from 0.03 to 1.13, and the values of α vary from −0.32 to 2.05, indicating a large variability in aerosol content and size. In cloud-free conditions, 36% of the airmasses come from Africa, 25% from Central-Eastern Europe, and 19% from Western France, Spain and the North Atlantic. In summer, 42% of the airmasses is of African origin. In almost all cases African aerosols display high values of τ and low values of α, typical of Saharan dust (average values of τ and α are 0.36 and 0.42, respectively). Particles originating from Central-Eastern Europe show relatively large average values of τ and α (0.23 and 1.5, respectively), while particles from Western France, Spain and the North Atlantic show the lowest average values of τ (0.15), and relatively small values of α (0.92). Intermediate values of α are often connected with relatively fast changes of the airmass originating sector, suggesting the contemporary presence of different types of particles in the air column. Clean marine conditions are rare at Lampedusa, and are generally associated with subsidence of the airmasses reaching the island. Average values of τ and α for clean marine conditions are 0.11 and 0.86, respectively. The largest values of α (about 2) were observed in August 2003, when large scale forest fires in Southern Europe produced consistent amounts of fine combustion particles, that were transported to the Central Mediterranean by a persistent high pressure system over Central Europe. Smoke particles in some cases mix with desert dust, producing intermediate values of α. The seasonal distribution of the meteorological patterns over the Mediterranean, the efficiency of the aerosol production mechanisms, and the variability of the particles' residence time produce a distinct seasonal cycle of aerosol optical depths and Ångström exponent values. Particles originating from all sectors show a summer maximum in aerosol optical depth. The summer increase in optical depth for European aerosols is linked with an increment in the values of α, that indicates an enhancement in the number of fine particles. The summer maximum of τ for African particles is associated with a weak reduction in the Ångström exponent, suggesting an increase in the total number of particles and a relatively more intense transport of large particles. The observations were classified according to the aerosol optical properties, and two main classes have been identified: desert dust and biomass burning/urban-industrial aerosols. Values of τ and α averaged over the whole observing period are 0.37 and 0.15 for desert dust, and 0.27 and 1.77 for urban-industrial/biomass burning aerosols.


Atmosphere ◽  
2020 ◽  
Vol 11 (10) ◽  
pp. 1103
Author(s):  
Jie Luo ◽  
Yongming Zhang ◽  
Qixing Zhang

In this work, the absorption Ångström exponent (AAE), extinction Ångström exponent (EAE), and single-scattering albedo (SSA) of black carbon (BC) with different coating materials are numerically investigated. BC with different coating materials can provide explanations for the small AAE, small EAE, and large AAE observed in the atmosphere, which is difficult to be explained by bare BC aggregate models. The addition of organic carbon (OC) does not necessarily increase AAE due to the transformation of BC morphologies and the existence of non-absorbing OC. The addition of coating materials does also not necessarily decrease EAE. While the addition of coating materials can increase the total size of BC-containing particles, the effective refractive index can be modified by introducing the coating materials, so increases the EAE. We found that it is not possible to differentiate between thinly- and heavily-coated BC based on EAE or AAE alone. On the other hand, SSA is much less sensitive to the size and can provide much more information for distinguishing heavily-coated BC from thinly-coated BC. For BC with different coating materials and mixing states, AAE, EAE, and SSA show rather different sensitivities to particle size and composition ratios, and their spectral-dependences also exhibit distinct differences. Different AAE and EAE trends with BC/OC ratio were also found for BC with different coating materials and mixing states. Furthermore, we also found empirical fittings for AAE, EAE, SSA, and optical cross-sections, which may be useful for retrieving the size information based on the optical measurements.


2017 ◽  
Vol 9 (7) ◽  
pp. 693 ◽  
Author(s):  
Yidan Si ◽  
Shenshen Li ◽  
Liangfu Chen ◽  
Huazhe Shang ◽  
Lei Wang ◽  
...  

2015 ◽  
Vol 2015 ◽  
pp. 1-12 ◽  
Author(s):  
Sunmin Park ◽  
Hesham El-Askary ◽  
Ismail Sabbah ◽  
Hanbin Kwak ◽  
Anup K. Prasad ◽  
...  

We investigate the temporal characteristics of major air pollutants collected from 44 air quality stations over the city of Seoul, Korea, namely, nitrogen dioxide, carbon monoxide, particular matter at 10 microns, and sulfur dioxide (SO2) between 2000 and 2009. The corresponding satellite datasets, namely, aerosol optical depth (AODsat), Ångström exponent, and fine mode fraction, collected from moderate resolution imaging spectroradiometer (MODIS) as well as the Aeronet ground aerosol optical depth (AODaeronet), have been analyzed. Pollutants’ seasonal effect has been inferred from the precipitation and temperature. The four pollutants under study show varying temporal characteristics with different annual mean concentration patterns. The monthly mean of mentioned pollutants all show similar low concentrations during the summer season and high concentrations during the winter season. We found that pollution is strongly linked to temperature and precipitation variability, especially during the fall season. Satellite data analysis provides information on the pollutants origin whether of natural or anthropogenic type. Our results indicate that the anthropogenic aerosol is dominant in the summer season even though the concentration was lower than the other seasons. AODaeronetand Ångström exponent indicated high positive and negative correlation coefficients with PM10, 0.60, and −0.45, respectively. Both small and large sizes of aerosols existed in 2007; however coarse size of aerosols was the primary component in 2002.


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