scholarly journals Space-based observations of fire NO<sub>x</sub> emission coefficients: a global biome-scale comparison

2013 ◽  
Vol 13 (8) ◽  
pp. 21665-21702 ◽  
Author(s):  
A. K. Mebust ◽  
R. C. Cohen

Abstract. Biomass burning represents both a significant and highly variable source of NOx to the atmosphere. This variability stems from both the episodic nature of fires, and from fire conditions such as the modified combustion efficiency of the fire, the nitrogen content of the fuel and possibly other factors that have not been identified or evaluated by comparison with observations. Satellite instruments offer an opportunity to observe emissions from wildfires, providing a large suite of measurements which allow us to study mean behavior and variability on the regional scale in a statistically rigorous manner. Here we use space-based measurements of fire radiative power from the Moderate Resolution Imaging Spectroradiometer in combination with NO2 tropospheric column densities from the Ozone Monitoring Instrument to measure mean emission coefficients (ECs in g NO MJ−1) from fires for global biomes, and across a wide range of smaller-scale ecoregions, defined as spatially-distinct clusters of fires with similar fuel type. Mean ECs for all biomes fall between 0.250–0.362 g NO MJ−1, a range that is smaller than found in previous studies of biome-scale emission factors. The majority of ecoregion ECs fall within or near this range, implying that under most conditions, mean fire emissions per unit energy are similar between different regions regardless of fuel type or spatial variability. In contrast to these similarities, we find that about 24% of individual ecoregion ECs deviate significantly (p < 0.05) from the mean EC for the associated biome, and a similar number of ecoregion ECs falls outside this range, implying that there are some regions where fuel type-specific global emission parameterizations fail to capture local fire NOx emissions.

2014 ◽  
Vol 14 (5) ◽  
pp. 2509-2524 ◽  
Author(s):  
A. K. Mebust ◽  
R. C. Cohen

Abstract. Biomass burning represents both a significant and highly variable source of NOx to the atmosphere. This variability stems from both the episodic nature of fires, and from fire conditions such as the modified combustion efficiency of the fire, the nitrogen content of the fuel and possibly other factors that have not been identified or evaluated by comparison with observations. Satellite instruments offer an opportunity to observe emissions from wildfires, providing a large suite of measurements which allow us to study mean behavior and variability on the regional scale in a statistically rigorous manner. Here we use space-based measurements of fire radiative power from the Moderate Resolution Imaging Spectroradiometer in combination with NO2 tropospheric column densities from the Ozone Monitoring Instrument to measure mean emission coefficients (ECs in g NO MJ−1) from fires for global biomes, and across a wide range of smaller-scale ecoregions, defined as spatially-distinct clusters of fires with similar fuel type. Mean ECs for all biomes fall between 0.250–0.362 g NO MJ−1, a range that is smaller than found in previous studies of biome-scale emission factors. The majority of ecoregion ECs fall within or near this range, implying that under most conditions, mean fire emissions of NOx per unit energy are similar between different regions regardless of fuel type or spatial variability. In contrast to these similarities, we find that about 24% of individual ecoregion ECs deviate significantly (with 95% confidence) from the mean EC for the associated biome, and a similar number of ecoregion ECs falls outside the range of all mean biome ECs, implying that there are some regions where fuel type-specific global emission parameterizations fail to capture local fire NOx emissions.


2011 ◽  
Vol 11 (12) ◽  
pp. 5839-5851 ◽  
Author(s):  
A. K. Mebust ◽  
A. R. Russell ◽  
R. C. Hudman ◽  
L. C. Valin ◽  
R. C. Cohen

Abstract. We use observations of fire radiative power (FRP) from the Moderate Resolution Imaging Spectroradiometer~(MODIS) and tropospheric NO2 column measurements from the Ozone Monitoring Instrument (OMI) to derive NO2 wildfire emission coefficients (g MJ−1) for three land types over California and Nevada. Retrieved emission coefficients were 0.279±0.077, 0.342±0.053, and 0.696±0.088 g MJ−1 NO2 for forest, grass and shrub fuels, respectively. These emission coefficients reproduce ratios of emissions with fuel type reported previously using independent methods. However, the magnitude of these coefficients is lower than prior estimates. While it is possible that a negative bias in the OMI NO2 retrieval over regions of active fire emissions is partly responsible, comparison with several other studies of fire emissions using satellite platforms indicates that current emission factors may overestimate the contributions of flaming combustion and underestimate the contributions of smoldering combustion to total fire emissions. Our results indicate that satellite data can provide an extensive characterization of the variability in fire NOx emissions; 67 % of the variability in emissions in this region can be accounted for using an FRP-based parameterization.


2018 ◽  
Vol 18 (16) ◽  
pp. 11831-11845 ◽  
Author(s):  
Albert Ansmann ◽  
Holger Baars ◽  
Alexandra Chudnovsky ◽  
Ina Mattis ◽  
Igor Veselovskii ◽  
...  

Abstract. Light extinction coefficients of 500 Mm−1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by European Aerosol Research Lidar Network (EARLINET) lidars in the stratosphere over central Europe on 21–22 August 2017. Pronounced smoke layers with a 1–2 km vertical extent were found 2–5 km above the local tropopause. Optically dense layers of Canadian wildfire smoke reached central Europe 10 days after their injection into the upper troposphere and lower stratosphere which was caused by rather strong pyrocumulonimbus activity over western Canada. The smoke-related aerosol optical thickness (AOT) identified by lidar was close to 1.0 at 532 nm over Leipzig during the noon hours on 22 August 2017. Smoke particles were found throughout the free troposphere (AOT of 0.3) and in the pronounced 2 km thick stratospheric smoke layer at an altitude of 14–16 km (AOT of 0.6). The lidar observations indicated peak mass concentrations of 70–100 µg m−3 in the stratosphere. In addition to the lidar profiles, we analyzed Moderate Resolution Imaging Spectroradiometer (MODIS) fire radiative power (FRP) over Canada, and the distribution of MODIS AOT and Ozone Monitoring Instrument (OMI) aerosol index across the North Atlantic. These instruments showed a similar pattern and a clear link between the western Canadian fires and the aerosol load over Europe. In this paper, we also present Aerosol Robotic Network (AERONET) sun photometer observations, compare photometer and lidar-derived AOT, and discuss an obvious bias (the smoke AOT is too low) in the photometer observations. Finally, we compare the strength of this record-breaking smoke event (in terms of the particle extinction coefficient and AOT) with major and moderate volcanic events observed over the northern midlatitudes.


2014 ◽  
Vol 14 (2) ◽  
pp. 3099-3168 ◽  
Author(s):  
I. B. Konovalov ◽  
E. V. Berezin ◽  
P. Ciais ◽  
G. Broquet ◽  
M. Beekmann ◽  
...  

Abstract. A method to constrain carbon dioxide (CO2) emissions from open biomass burning by using satellite observations of co-emitted species and a chemistry-transport model (CTM) is proposed and applied to the case of wildfires in Siberia. CO2 emissions are assessed by means of an emission model assuming a direct relationship between the biomass burning rate (BBR) and the Fire Radiative Power (FRP) derived from the MODIS measurements. The key features of the method are (1) estimating the FRP-to-BBR conversion factors (α) for different vegetative land cover types by assimilating the satellite observations of co-emitted species into the CTM, (2) optimal combination of the estimates of α derived independently from satellite observations of different species (CO and aerosol in this study), and (3) estimation of the diurnal cycle of the fire emissions directly from the FRP measurements. Values of α for forest and grassland fires in Siberia and their uncertainties are estimated by using the IASI carbon monoxide (CO) retrievals and the MODIS aerosol optical depth (AOD) measurements combined with outputs from the CHIMERE mesoscale chemistry transport model. The constrained CO emissions are validated through comparison of the respective simulations with the independent data of ground based CO measurements at the ZOTTO site. Using our optimal regional-scale estimates of the conversion factors (which are found to be in agreement with the earlier published estimates obtained from local measurements of experimental fires), the total CO2 emissions from wildfires in Siberia in 2012 are estimated to be in the range from 262 to 477 Tg C, with the optimal (maximum likelihood) value of 354 Tg C. Sensitivity test cases featuring different assumptions regarding the injection height and diurnal variations of emissions indicate that the derived estimates of the total CO2 emissions in Siberia are robust with respect to the modelling options (the different estimates vary within less than 10% of their magnitude). The obtained CO2 emission estimates for several years are compared with the independent estimates provided by the GFED3.1 and GFASv1.0 global emission inventories. It is found that our "top-down" estimates for the total annual biomass burning CO2 emissions in the period from 2007 to 2011 in Siberia are by factors of 2.3 and 1.7 larger than the respective bottom-up estimates; these discrepancies cannot be fully explained by uncertainties in our estimates. There are also considerable differences in the spatial distribution of the different emission estimates; some of those differences have a systematic character and require further analysis.


2011 ◽  
Vol 11 (2) ◽  
pp. 5351-5378 ◽  
Author(s):  
A. K. Mebust ◽  
A. R. Russell ◽  
R. C. Hudman ◽  
L. C. Valin ◽  
R. C. Cohen

Abstract. We use observations of fire radiative power (FRP) from the Moderate Resolution Imaging Spectroradiometer (MODIS) and tropospheric NO2 column measurements from the Ozone Monitoring Instrument (OMI) to derive NO2 wildfire emission coefficients (g MJ−1) for three land types over California and Nevada. Retrieved emission coefficients were 0.279 ± 0.077, 0.342 ± 0.053, and 0.696 ± 0.088 g MJ−1 NO2 for forest, grass and shrub fuels, respectively. These emission coefficients reproduce ratios of emissions with fuel type reported previously using independent methods. However, the magnitude of these coefficients is lower than prior estimates, which suggests either a negative bias in the OMI NO2 retrieval over regions of active emissions, or that the average fire observed in our study has a smaller ratio of flaming to smoldering combustion than measurements used in prior estimates of emissions. Our results indicate that satellite data can provide an extensive characterization of the variability in fire NOx emissions; 67% of the variability in emissions in this region can be accounted for using an FRP-based parameterization.


2014 ◽  
Vol 14 (19) ◽  
pp. 10383-10410 ◽  
Author(s):  
I. B. Konovalov ◽  
E. V. Berezin ◽  
P. Ciais ◽  
G. Broquet ◽  
M. Beekmann ◽  
...  

Abstract. A method to constrain carbon dioxide (CO2) emissions from open biomass burning by using satellite observations of co-emitted species and a chemistry-transport model (CTM) is proposed and applied to the case of wildfires in Siberia. CO2 emissions are assessed by means of an emission model assuming a direct relationship between the biomass burning rate (BBR) and the fire radiative power (FRP) derived from MODIS measurements. The key features of the method are (1) estimating the FRP-to-BBR conversion factors (α) for different vegetative land cover types by assimilating the satellite observations of co-emitted species into the CTM, (2) optimal combination of the estimates of α derived independently from satellite observations of different species (CO and aerosol in this study), and (3) estimation of the diurnal cycle of the fire emissions directly from the FRP measurements. Values of α for forest and grassland fires in Siberia and their uncertainties are estimated using the Infrared Atmospheric Sounding Interferometer (IASI) carbon monoxide (CO) retrievals and MODIS aerosol optical depth (AOD) measurements combined with outputs from the CHIMERE mesoscale chemistry-transport model. The constrained CO emissions are validated through comparison of the respective simulations with independent data of ground-based CO measurements at the ZOTTO site. Using our optimal regional-scale estimates of the conversion factors (which are found to be in agreement with earlier published estimates obtained from local measurements of experimental fires), the total CO2 emissions from wildfires in Siberia in 2012 are estimated to be in the range from 280 to 550 Tg C, with the optimal (maximum likelihood) value of 392 Tg C. Sensitivity test cases featuring different assumptions regarding the injection height and diurnal variations of emissions indicate that the derived estimates of the total CO2 emissions in Siberia are robust with respect to the modeling options (the different estimates vary within less than 15% of their magnitude). The CO2 emission estimates obtained for several years are compared with independent estimates provided by the GFED3.1 and GFASv1.0 global emission inventories. It is found that our "top-down" estimates for the total annual biomass burning CO2 emissions in the period from 2007 to 2011 in Siberia are by factors of 2.5 and 1.8 larger than the respective bottom-up estimates; these discrepancies cannot be fully explained by uncertainties in our estimates. There are also considerable differences in the spatial distribution of the different emission estimates; some of those differences have a systematic character and require further analysis.


2010 ◽  
Vol 10 (4) ◽  
pp. 1491-1510 ◽  
Author(s):  
M. Val Martin ◽  
J. A. Logan ◽  
R. A. Kahn ◽  
F.-Y. Leung ◽  
D. L. Nelson ◽  
...  

Abstract. We analyze an extensive record of aerosol smoke plume heights derived from observations over North America for the fire seasons of 2002 and 2004–2007 made by the Multi-angle Imaging SpectroRadiometer (MISR) instrument on board the NASA Earth Observing System Terra satellite. We characterize the magnitude and variability of smoke plume heights for various biomes, and assess the contribution of local atmospheric and fire conditions to this variability. Plume heights are highly variable, ranging from a few hundred meters up to 5000 m above the terrain at the Terra overpass time (11:00–14:00 local time). The largest plumes are found over the boreal region (median values of ~850 m height, 24 km length and 940 m thickness), whereas the smallest plumes are found over cropland and grassland fires in the contiguous US (median values of ~530 m height, 12 km length and 550–640 m thickness). The analysis of plume heights in combination with assimilated meteorological observations from the NASA Goddard Earth Observing System indicates that a significant fraction (4–12%) of plumes from fires are injected above the boundary layer (BL), consistent with earlier results for Alaska and the Yukon Territories during summer 2004. Most of the plumes located above the BL (>83%) are trapped within stable atmospheric layers. We find a correlation between plume height and the MODerate resolution Imaging Spectroradiometer (MODIS) fire radiative power (FRP) thermal anomalies associated with each plume. Smoke plumes located in the free troposphere (FT) exhibit larger FRP values (1620–1640 MW) than those remaining within the BL (174–465 MW). Plumes located in the FT without a stable layer reach higher altitudes and are more spread-out vertically than those associated with distinct stable layers (2490 m height and 2790 m thickness versus 1880 m height and 1800 m thickness). The MISR plume climatology exhibits a well-defined seasonal cycle of plume heights in boreal and temperate biomes, with greater heights during June–July. MODIS FRP measurements indicate that larger summertime heights are the result of higher fire intensity, likely due to more severe fire weather during these months. This work demonstrates the significant effect of fire intensity and atmospheric structure on the ultimate rise of fire emissions, and underlines the importance of considering such physical processes in modeling smoke dispersion.


2016 ◽  
Vol 25 (1) ◽  
pp. 48 ◽  
Author(s):  
Matthew B. Dickinson ◽  
Andrew T. Hudak ◽  
Thomas Zajkowski ◽  
E. Louise Loudermilk ◽  
Wilfrid Schroeder ◽  
...  

Characterising radiation from wildland fires is an important focus of fire science because radiation relates directly to the combustion process and can be measured across a wide range of spatial extents and resolutions. As part of a more comprehensive set of measurements collected during the 2012 Prescribed Fire Combustion and Atmospheric Dynamics Research (RxCADRE) field campaign, we used ground, airborne and spaceborne sensors to measure fire radiative power (FRP) from whole fires, applying different methods to small (2 ha) and large (>100 ha) burn blocks. For small blocks (n = 6), FRP estimated from an obliquely oriented long-wave infrared (LWIR) camera mounted on a boom lift were compared with FRP derived from combined data from tower-mounted radiometers and remotely piloted aircraft systems (RPAS). For large burn blocks (n = 3), satellite FRP measurements from the Moderate-resolution Imaging Spectroradiometer (MODIS) and Visible Infrared Imaging Radiometer Suite (VIIRS) sensors were compared with near-coincident FRP measurements derived from a LWIR imaging system aboard a piloted aircraft. We describe measurements and consider their strengths and weaknesses. Until quantitative sensors exist for small RPAS, their use in fire research will remain limited. For oblique, airborne and satellite sensors, further FRP measurement development is needed along with greater replication of coincident measurements, which we show to be feasible.


2009 ◽  
Vol 9 (5) ◽  
pp. 20515-20566 ◽  
Author(s):  
M. Val Martin ◽  
J. A. Logan ◽  
D. Kahn ◽  
F. Y. Leung ◽  
D. Nelson ◽  
...  

Abstract. We analyze a multi-year record of aerosol smoke plume heights derived from observations over North America made by the Multi-angle Imaging SpectroRadiometer (MISR) instrument on board the NASA Earth Observing System Terra satellite. We characterize the magnitude and variability of smoke plume heights for various biomes, and assess the contribution of local atmospheric and fire conditions to this variability. Plume heights are highly variable, ranging from a few hundred meters up to 5000 m above the terrain at the Terra overpass time (11:00–14:00 local time). The largest plumes are found over the boreal region (median values of ∼850 m height, 24 km length and 940 m thickness), whereas the smallest plumes are found over cropland and grassland fires in the contiguous US (median values of ∼530 m height, 12 km length and 550–640 m thickness). The analysis of plume heights in combination with assimilated meteorological observations from the NASA Goddard Earth Observing System indicates that a significant fraction (4–12%) of plumes from fires are injected above the boundary layer (BL), consistent with earlier results for Alaska and the Yukon Territories during summer 2004. Most of the plumes located above the BL (>83%) are trapped within stable atmospheric layers. We find a correlation between plume height and the MODerate resolution Imaging Spectroradiometer (MODIS) fire radiative power (FRP) thermal anomalies associated with each plume. Smoke plumes located in the free troposphere (FT) exhibit larger FRP values (1620–1640 MW) than those remaining within the BL (174–465 MW). Plumes located in the FT without a stable layer reach higher altitudes and are more spread-out vertically than those associated with distinct stable layers (2490 m height and 2790 m thickness versus 1880 m height and 1800 thickness). The MISR plume climatology exhibits a well-defined seasonal cycle of plume heights in boreal and temperate biomes, with greater heights during June–July. MODIS FRP measurements indicate that larger summertime heights are the result of higher fire intensity, likely due to more severe fire weather during these months. This work demonstrates the significant effect of fire radiative heat and atmospheric structure on the ultimate rise of fire emissions, and underlines the importance of considering such physical processes in modeling smoke dispersion.


2005 ◽  
Vol 5 (5) ◽  
pp. 10455-10516 ◽  
Author(s):  
R. Koppmann ◽  
K. von Czapiewski ◽  
J. S. Reid

Abstract. Biomass burning is the burning of living and dead vegetation. Ninety percent of all biomass-burning events are thought to be human initiated. Human induced fires are used for a variety of ''applications'' such as agricultural expansion, deforestation, bush control, weed and residue burning, and harvesting practices. Natural fires are grassland and forest fires mainly induced by lightning. It is estimated that 8700 Tg of dry matter/year are burnt each year in total. Emissions from biomass burning include a wide range of gaseous compounds and particles that contribute significantly to the tropospheric budgets on a local, regional, and even global scales. The emission of CO, CH4 and VOC affect the oxidation capacity of the troposphere by reacting with OH radicals, and emissions of nitric oxide and VOC lead to the formation of ozone and other photo oxidants. For a large number of compounds biomass burning is one of the largest single sources in the troposphere, especially in the tropics. Biomass-burning emissions play an important role in the biogeochemical cycles of carbon and nitrogen. Following the first systematic investigations on fire emissions in laboratory experiments in the 1960's, the last 20 years saw an increasing number in studies on biomass-burning emissions in various ecosystems. Recently, our knowledge of the emissions of gaseous compounds in the troposphere from fires has increased considerably. This manuscript is the first of four describing the properties biomass burning emissions. The properties of biomass-burning particles are discussed in part II and III of this review series which have been recently published, and their direct radiative effects are in part IV. This paper focuses on the review of emission ratios and emission rates of carbon monoxide, methane, volatile organics, and nitrogen containing compounds and should not be seen as a review of global emission estimates, even though we discuss the implications of our results on such studies.


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