scholarly journals Trapping, chemistry and export of trace gases in the South Asian summer monsoon observed during CARIBIC flights in 2008

2015 ◽  
Vol 15 (5) ◽  
pp. 6967-7018 ◽  
Author(s):  
A. Rauthe-Schöch ◽  
A. K. Baker ◽  
T. J. Schuck ◽  
C. A. M. Brenninkmeijer ◽  
A. Zahn ◽  
...  
Keyword(s):  
South Asian ◽  
Summer Monsoon ◽  
Asian Summer Monsoon ◽  
Trace Gases ◽  
Particle Dispersion ◽  
Atmospheric Pollutants ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Air Masses ◽  
Asian Summer

Abstract. The CARIBIC (Civil Aircraft for the Regular Investigation of the Atmosphere Based on an Instrument Container) passenger aircraft observatory performed in situ measurements at 10–12 km altitude in the South Asian summer monsoon anticyclone between June and September 2008. These measurements enable us to investigate this atmospheric region, which so far has mostly been observed from satellites, using the broad suite of trace gases and aerosols measured by CARIBIC. Elevated levels of a range of atmospheric pollutants were recorded e.g. carbon monoxide, total reactive nitrogen oxides, aerosol particles and several volatile organic compounds. The measurements provide detailed information about the chemical composition of air in different parts of the monsoon anticyclone, particularly of ozone precursors. While covering a range of 3500 km inside the monsoon anticyclone, CARIBIC observations show remarkable consistency, i.e. with regular latitudinal patterns of trace gases during the entire monsoon period. Trajectory calculations indicate that these air masses originated mainly from South Asia and Mainland Southeast Asia. Using the CARIBIC trace gas and aerosol measurements in combination with the Lagrangian particle dispersion model FLEXPART we investigated the characteristics of monsoon outflow and the chemical evolution of air masses during transport. Estimated photochemical ages of the air were found to agree well with transport times from a source region east of 95° E. The photochemical ages of the air in the southern part of the monsoon anticyclone were consistently younger (less than 7 days) and the air masses mostly in an ozone forming chemical regime. In its northern part the air masses were older (up to 13 days) and had unclear ozone formation or destruction potential. Based on analysis of forward trajectories several receptor regions were identified. In addition to predominantly westward transport, we found evidence for efficient transport (within 10 days) to the Pacific and North America, particularly during June and September, and also of cross-tropopause exchange, which was strongest during June and July. Westward transport to Africa and further to the Mediterranean was the main pathway during July.

scholarly journals Trapping, chemistry, and export of trace gases in the South Asian summer monsoon observed during CARIBIC flights in 2008

2016 ◽  
Vol 16 (5) ◽  
pp. 3609-3629 ◽  
Author(s):  
Armin Rauthe-Schöch ◽  
Angela K. Baker ◽  
Tanja J. Schuck ◽  
Carl A. M. Brenninkmeijer ◽  
Andreas Zahn ◽  
...  
Keyword(s):  
South Asian ◽  
Summer Monsoon ◽  
Asian Summer Monsoon ◽  
Aerosol Particles ◽  
Trace Gases ◽  
Atmospheric Pollutants ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Air Masses ◽  
Asian Summer

Abstract. The CARIBIC (Civil Aircraft for the Regular Investigation of the Atmosphere Based on an Instrument Container) passenger aircraft observatory performed in situ measurements at 10–12 km altitude in the South Asian summer monsoon anticyclone between June and September 2008. These measurements enable us to investigate this atmospheric region (which so far has mostly been observed from satellites) using the broad suite of trace gases and aerosol particles measured by CARIBIC. Elevated levels of a variety of atmospheric pollutants (e.g. carbon monoxide, total reactive nitrogen oxides, aerosol particles, and several volatile organic compounds) were recorded. The measurements provide detailed information about the chemical composition of air in different parts of the monsoon anticyclone, particularly of ozone precursors. While covering a range of 3500 km inside the monsoon anticyclone, CARIBIC observations show remarkable consistency, i.e. with distinct latitudinal patterns of trace gases during the entire monsoon period. Using the CARIBIC trace gas and aerosol particle measurements in combination with the Lagrangian particle dispersion model FLEXPART, we investigated the characteristics of monsoon outflow and the chemical evolution of air masses during transport. The trajectory calculations indicate that these air masses originated mainly from South Asia and mainland Southeast Asia. Estimated photochemical ages of the air were found to agree well with transport times from a source region east of 90–95° E. The photochemical ages of the air in the southern part of the monsoon anticyclone were systematically younger (less than 7 days) and the air masses were mostly in an ozone-forming chemical mode. In its northern part the air masses were older (up to 13 days) and had unclear ozone formation or destruction potential. Based on analysis of forward trajectories, several receptor regions were identified. In addition to predominantly westward transport, we found evidence for efficient transport (within 10 days) to the Pacific and North America, particularly during June and September, and also of cross-tropopause exchange, which was strongest during June and July. Westward transport to Africa and further to the Mediterranean was the main pathway during July.

scholarly journals Upper tropospheric CH<sub>4</sub> and CO affected by the South Asian summer monsoon during OMO

2018 ◽  
Author(s):  
Laura Tomsche ◽  
Andrea Pozzer ◽  
Narendra Ojha ◽  
Uwe Parchatka ◽  
Jos Lelieveld ◽  
...  
Keyword(s):  
South Asian ◽  
Asian Summer Monsoon ◽  
Trace Gases ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Transport Pathways ◽  
Air Masses ◽  
Upper Troposphere ◽  
Asian Summer

Abstract. The Asian monsoon anticyclone (AMA) is a yearly recurring phenomenon in the northern hemispheric upper troposphere and lower stratosphere. It is connected to the South Asian summer monsoon, and the circulation extends approximately across 20°–120° E and 15°–40° N longitude-latitude. It has a clearly observable signature due to vertical transport of polluted air masses from the surface to the upper troposphere by the monsoon convection. However, the transport pathways and the fate of pollutants in the upper troposphere are not yet fully understood. As pollution emissions in South Asia are increasing, changes in the chemical composition of the AMA can be expected. We performed in situ measurements of carbon monoxide (CO) and methane (CH4) in the region of monsoon outflow and in background air in the upper troposphere (Mediterranean, Arabian Peninsula, Arabian Sea) by optical absorption spectroscopy on board the German High Altitude and Long range (HALO) research aircraft during the OMO (Oxidation Mechanism Observations) mission in summer 2015. We identified the transport pathways and the origin of the trace gases with back trajectories, calculated with the Lagrangian particle dispersion model FLEXPART, and we compared the in situ data with simulations of the atmospheric chemistry general circulation model EMAC. CH4 and CO mixing ratios were found to be enhanced within the AMA, on average by 72.1 ppb and 20.1 ppb, respectively, originating in the South Asian region (Indio-Gangetic Plain, North East India, Bangladesh and Bay of Bengal). It appears that CH4 is an ideal monsoon tracer in the upper troposphere due to its extended lifetime and the strong South Asian emissions. Furthermore, we used the measurements and model results to study the dynamics of the AMA, with an emphasis on the southern and western areas within the upper troposphere. For example, we distinguished four AMA modes based on different meteorological conditions. During one occasion we observed that under the influence of dwindling flow the transport barrier between the anticyclone and its surroundings weakened, expelling air masses from the AMA. The trace gases exhibited a distinct fingerprint of the AMA, and we also found that CH4 accumulated over the course of the OMO campaign.

A Moist Entropy Budget View of the South Asian Summer Monsoon Onset

2019 ◽  
Vol 46 (8) ◽  
pp. 4476-4484
Author(s):  
Ding Ma ◽  
Adam H. Sobel ◽  
Zhiming Kuang ◽  
Martin S. Singh ◽  
Ji Nie
Keyword(s):  
South Asian ◽  
Summer Monsoon ◽  
Asian Summer Monsoon ◽  
Monsoon Onset ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Summer Monsoon Onset ◽  
Asian Summer ◽  
Entropy Budget

scholarly journals Interannual Variability in the Large-Scale Dynamics of the South Asian Summer Monsoon

2015 ◽  
Vol 28 (9) ◽  
pp. 3731-3750 ◽  
Author(s):  
Jennifer M. Walker ◽  
Simona Bordoni ◽  
Tapio Schneider
Keyword(s):  
Interannual Variability ◽  
South Asian ◽  
Summer Monsoon ◽  
Large Scale ◽  
Asian Summer Monsoon ◽  
Sea Breeze ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Near Surface ◽  
Asian Summer

Abstract This study identifies coherent and robust large-scale atmospheric patterns of interannual variability of the South Asian summer monsoon (SASM) in observational data. A decomposition of the water vapor budget into dynamic and thermodynamic components shows that interannual variability of SASM net precipitation (P − E) is primarily caused by variations in winds rather than in moisture. Linear regression analyses reveal that strong monsoons are distinguished from weak monsoons by a northward expansion of the cross-equatorial monsoonal circulation, with increased precipitation in the ascending branch. Interestingly, and in disagreement with the view of monsoons as large-scale sea-breeze circulations, strong monsoons are associated with a decreased meridional gradient in the near-surface atmospheric temperature in the SASM region. Teleconnections exist from the SASM region to the Southern Hemisphere, whose midlatitude poleward eddy energy flux correlates with monsoon strength. Possible implications of these teleconnection patterns for understanding SASM interannual variability are discussed.

Investigating the sensitivity of the onset and withdrawal of the south Asian summer monsoon system to changes in anthropogenic emissions using a climate model

2020 ◽  
Author(s):  
Shiwansha Mishra ◽  
Dilip Ganguly ◽  
Puneet Sharma
Keyword(s):  
South Asian ◽  
Summer Monsoon ◽  
Climate Model ◽  
Asian Summer Monsoon ◽  
Anthropogenic Emissions ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Monsoon System ◽  
Asian Summer ◽  
The Impact

&lt;p&gt;While the monsoon onset is recognized as a rapid, substantial, and sustained increase in rainfall over large parts of south Asia, the withdrawal marks the return to dry conditions. Normally, the south Asian summer monsoon onset occurs around 1&lt;sup&gt;st&lt;/sup&gt; June over extreme south of peninsular India, which gradually advances to extreme northwest of India by around 15&lt;sup&gt;th&lt;/sup&gt; July. The withdrawal starts from northwest India from around 1st September and from extreme south peninsular India by around 30th September. The determinations of the onset and withdrawal dates of monsoon have great economic significance for this region as they influence many agriculture and water resource management decisions in one of the most highly populated regions of the world. Several studies involving global model simulations have shown that changing aerosol emissions could result in significant changes in the seasonal mean precipitation distribution over India. A few studies also show that presence of absorbing aerosols in the foothills of Himalayas and over the Tibetan plateau could increase the moisture convergence over India thereby causing an advancement and intensification of the monsoon precipitation. However, most of the previous studies, which investigated the impact of anthropogenic emissions on the monsoon, are limited to understanding the impact of various emission changes on the seasonal mean monsoon characteristics. In the present study, we try to understand the sensitivity of the onset and withdrawal period of the south Asian summer monsoon system to changes in anthropogenic emissions using a climate model (CESM1.2). We diagnose the onset and withdrawal of the south Asian monsoon by analyzing the variability in vertically integrated moisture transport (VIMT) over the south Asian region and following the definition of hydrologic onset and withdrawal index (HOWI) defined by Fasullo et al. (2002). We examined the effect of changing emissions anthropogenic aerosol, greenhouse gases and both on the onset and withdrawal of the south Asian summer monsoon system. Our preliminary results suggest that increases in the emissions of aerosols and greenhouse gases from anthropogenic sources from pre-industrial to present day could possibly result in significant delay in the onset and advancement in withdrawal of the south Asian summer monsoon system thereby shortening the length of the monsoon season. More results with greater detail will be presented.&lt;/p&gt;

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