scholarly journals Review of 'A Holocene black carbon ice-core record of biomass burning in the Amazon Basin from Illimani, Bolivia’

2018 ◽  
Author(s):  
Anonymous
2018 ◽  
Author(s):  
Dimitri Osmont ◽  
Michael Sigl ◽  
Anja Eichler ◽  
Theo M. Jenk ◽  
Margit Schwikowski

Abstract. The Amazon Basin is one of the major contributors to global biomass burning emissions. However, regional paleofire trends remain partially unknown. Due to their proximity to the Amazon Basin, Andean ice cores are suitable to reconstruct paleofire trends in South America and improve our understanding of the complex linkages between fires, climate and humans. Here we present the first refractory black carbon (rBC) ice-core record from the Andes as a proxy for biomass burning emissions in the Amazon Basin, derived from an ice core drilled at 6300 m a.s.l. from Illimani glacier in the Bolivian Andes and spanning the entire Holocene back to the last deglaciation 13 000 years ago. The Illimani rBC record displays a strong seasonality with low values during the wet season and high values during the dry season due to the combination of enhanced biomass burning emissions in the Amazon Basin and less precipitation at the Illimani site. Significant positive (negative) correlations were found with reanalyzed temperature (precipitation) data, respectively, for regions in Eastern Bolivia and Western Brazil characterized by a substantial fire activity. rBC long-term trends indirectly reflect regional climatic variations through changing biomass burning emissions as they show higher (lower) concentrations during warm/dry (cold/wet) periods, respectively, in line with climate variations such as the Younger Dryas, the 8.2 ka event, the Holocene Climatic Optimum, the Medieval Warm Period or the Little Ice Age. The highest rBC concentrations of the entire record occurred during the Holocene Climatic Optimum between 7000 and 3000 BC, suggesting that this outstanding warm and dry period caused an exceptional biomass burning activity, unprecedented in the context of the past 13 000 years. Recent rBC levels, rising since 1730 AD in the context of increasing temperatures and deforestation, are similar to those of the Medieval Warm Period. No decrease was observed in the 20th century, in contradiction with the global picture (broken fire hockey stick hypothesis).


2019 ◽  
Vol 15 (2) ◽  
pp. 579-592 ◽  
Author(s):  
Dimitri Osmont ◽  
Michael Sigl ◽  
Anja Eichler ◽  
Theo M. Jenk ◽  
Margit Schwikowski

Abstract. The Amazon Basin is one of the major contributors to global biomass burning emissions. However, regional paleofire trends remain particularly unknown. Due to their proximity to the Amazon Basin, Andean ice cores are suitable to reconstruct paleofire trends in South America and improve our understanding of the complex linkages between fires, climate and humans. Here we present the first refractory black carbon (rBC) ice-core record from the Andes as a proxy for biomass burning emissions in the Amazon Basin, derived from an ice core drilled at 6300 m a.s.l. from the Illimani glacier in the Bolivian Andes and spanning the entire Holocene back to the last deglaciation 13 000 years ago. The Illimani rBC record displays a strong seasonality with low values during the wet season and high values during the dry season due to the combination of enhanced biomass burning emissions in the Amazon Basin and less precipitation at the Illimani site. Significant positive (negative) correlations were found with reanalyzed temperature (precipitation) data for regions in eastern Bolivia and western Brazil characterized by substantial fire activity. rBC long-term trends indirectly reflect regional climatic variations through changing biomass burning emissions as they show higher (lower) concentrations during warm–dry (cold–wet) periods, in line with climate variations such as the Younger Dryas, the 8.2 ka event, the Holocene Climatic Optimum, the Medieval Warm Period and the Little Ice Age. The highest rBC concentrations of the entire record occurred during the Holocene Climatic Optimum between 7000 and 3000 BCE, suggesting that this exceptionally warm and dry period caused high levels of biomass burning activity, unprecedented in the context of the past 13 000 years. Recent rBC levels, rising since 1730 CE in the context of increasing temperatures and deforestation, are similar to those of the Medieval Warm Period. No decrease in fire activity was observed in the 20th century, in contradiction to global biomass burning reconstructions based on charcoal data.


2016 ◽  
Author(s):  
Saehee Lim ◽  
Xavier Faïn ◽  
Patrick Ginot ◽  
Vladimir Mikhalenko ◽  
Stanislav Kutuzov ◽  
...  

Abstract. Black carbon (BC), emitted by fossil fuel combustion and biomass burning, is the second largest man-made contributor to global warming after carbon dioxide (Bond et al., 2013). However, limited information exists on its past emissions and atmospheric variability. In this study, we present the first high-resolution record of refractory BC (rBC, including mass concentration and size) reconstructed from ice cores drilled at a high-altitude Eastern European site in Mt. Elbrus (ELB), Caucasus (5115 m a.s.l.). The ELB ice core record, covering the period 1825–2013, reflects the atmospheric load of rBC particles at the ELB site transported from the European continent with a larger rBC input from sources located in the Eastern part of Europe. In the first half of the 20th century, European anthropogenic emissions resulted in a 1.5-fold increase in the ice core rBC mass concentrations as respect to its level in the preindustrial era (before 1850). The rBC mass concentrations increased by a 5-fold in 1960–1980, followed by a decrease until ~ 2000. Over the last decade, the rBC signal for summer time slightly increased. We have compared the signal with the atmospheric BC load simulated using past BC emissions (ACCMIP and MACCity inventories) and taken into account the contribution of different geographical region to rBC distribution and deposition at the ELB site. Interestingly, the observed rBC variability in the ELB ice core record since the 1960s is not in perfect agreement with the simulated atmospheric BC load. Similar features between the ice core rBC record and the best scenarios for the atmospheric BC load support that anthropogenic BC increase in the 20th century is reflected in the ELB ice core record. However, the peak in BC mass concentration observed in ~ 1970 in the ice core is estimated to occur a decade later from past inventories. BC emission inventories for the period 1960s–1970s may be underestimating European anthropogenic emissions. Furthermore, for summer time snow layers of the last 2000s, the slightly increasing trend of rBC deposition likely reflects recent changes in anthropogenic and biomass burning BC emissions in the Eastern part of Europe. Our study highlights that the past changes in BC emissions of Eastern Europe need to be considered in assessing on-going air quality regulation.


2020 ◽  
Author(s):  
Joel D. Barker ◽  
Susan Kaspari ◽  
Paolo Gabrielli ◽  
Anna Wegner ◽  
Emilie Beaudon ◽  
...  

Abstract. Himalayan glaciers are melting due to atmospheric warming with the potential to limit access to water for more than 25 % of the global population that reside in these glacier meltwater catchments. Black carbon has been implicated as a factor that is contributing to Himalayan glacier melt, but its sources and mechanisms of delivery to the Himalayas remain controversial. Here, we provide a 211-year ice core record spanning 1781–1992 CE for refractory black carbon (rBC) deposition from the Dasuopu glacier ice core, that has to date provided the highest elevation ice core record (7200 m). We report an average rBC concentration of 1.5 µg/L (SD = 5.0, n = 1628) over the 211-year period. An increase in the frequency and magnitude of rBC deposition occurs after 1877 CE, accompanied by decreased snow accumulation associated with a shift in the North Atlantic Oscillation Index to a positive phase. Typically, rBC is deposited onto Dasuopu glacier during the non-monsoon season, and short-lived increases in rBC concentration are associated with periods of drought within neighboring regions in north-west India, Afghanistan and Pakistan. Using a combination of spectral and back trajectory analyses, and comparison with a concurrent analysis of trace metals at equivalent depths in the same ice core, we show that biomass burning resulting from dry conditions is a source of rBC to the central Himalaya, and is responsible for deposition that is up to 60 times higher than the average rBC concentration over the time period analyzed. We suggest that biomass burning is a significant source of rBC to the central Himalaya, and that the rBC record can be used to identify periods of drought in nearby regions that are up-wind of Dasuopu glacier.


2021 ◽  
Vol 21 (7) ◽  
pp. 5615-5633
Author(s):  
Joel D. Barker ◽  
Susan Kaspari ◽  
Paolo Gabrielli ◽  
Anna Wegner ◽  
Emilie Beaudon ◽  
...  

Abstract. Himalayan glaciers are melting due to atmospheric warming, with the potential to limit access to water for more than 25 % of the global population that resides in these glacier meltwater catchments. Black carbon has been implicated as a factor that is contributing to Himalayan glacier melt, but its sources and mechanisms of delivery to the Himalayas remain controversial. Here, we provide a 211-year ice core record spanning 1781–1992 CE for refractory black carbon (rBC) deposition from the Dasuopu glacier ice core that has to date provided the highest-elevation ice core record (7200 m). We report an average rBC concentration of 1.5 µg L−1 (SD=5.0, n=1628) over the 211-year period. An increase in the frequency and magnitude of rBC deposition occurs after 1877 CE, accompanied by decreased snow accumulation associated with a shift in the North Atlantic Oscillation Index to a positive phase. Typically, rBC is deposited onto Dasuopu glacier during the non-monsoon season, and short-lived increases in rBC concentration are associated with periods of drought within neighboring regions in northwestern India, Afghanistan, and Pakistan. Using a combination of spectral and back-trajectory analyses, as well as a comparison with a concurrent analysis of trace metals at equivalent depths in the same ice core, we show that biomass burning resulting from dry conditions is a source of rBC to the central Himalaya and is responsible for deposition that is up to 60 times higher than the average rBC concentration over the time period analyzed. We suggest that biomass burning is a significant source of rBC to the central Himalaya and that the rBC record can be used to identify periods of drought in nearby regions that are upwind of Dasuopu glacier.


2017 ◽  
Vol 17 (5) ◽  
pp. 3489-3505 ◽  
Author(s):  
Saehee Lim ◽  
Xavier Faïn ◽  
Patrick Ginot ◽  
Vladimir Mikhalenko ◽  
Stanislav Kutuzov ◽  
...  

Abstract. Black carbon (BC), emitted by fossil fuel combustion and biomass burning, is the second largest man-made contributor to global warming after carbon dioxide (Bond et al., 2013). However, limited information exists on its past emissions and atmospheric variability. In this study, we present the first high-resolution record of refractory BC (rBC, including mass concentration and size) reconstructed from ice cores drilled at a high-altitude eastern European site in Mt. Elbrus (ELB), Caucasus (5115 m a.s.l.). The ELB ice core record, covering the period 1825–2013, reflects the atmospheric load of rBC particles at the ELB site transported from the European continent with a larger rBC input from sources located in the eastern part of Europe. In the first half of the 20th century, European anthropogenic emissions resulted in a 1.5-fold increase in the ice core rBC mass concentrations with respect to its level in the preindustrial era (before 1850). The summer (winter) rBC mass concentrations increased 5-fold (3.3-fold) in 1960–1980, followed by a decrease until  ∼  2000. Over the last decade, the rBC signal for summertime slightly increased. We have compared the signal with the atmospheric BC load simulated using past BC emissions (ACCMIP and MACCity inventories) and taken into account the contribution of different geographical regions to rBC distribution and deposition at the ELB site. Interestingly, the observed rBC variability in the ELB ice core record since the 1960s is not in perfect agreement with the simulated atmospheric BC load. Similar features between the ice core rBC record and the best scenarios for the atmospheric BC load support anthropogenic BC increase in the 20th century being reflected in the ELB ice core record. However, the peak in BC mass concentration observed in  ∼  1970 in the ice core is estimated to occur a decade later from past inventories. BC emission inventories for the period 1960s–1970s may be underestimating European anthropogenic emissions. Furthermore, for summertime snow layers of the 2000s, the slightly increasing trend of rBC deposition likely reflects recent changes in anthropogenic and biomass burning BC emissions in the eastern part of Europe. Our study highlights that the past changes in BC emissions of eastern Europe need to be considered in assessing ongoing air quality regulation.


2018 ◽  
Vol 18 (16) ◽  
pp. 12345-12361 ◽  
Author(s):  
Christian M. Zdanowicz ◽  
Bernadette C. Proemse ◽  
Ross Edwards ◽  
Wang Feiteng ◽  
Chad M. Hogan ◽  
...  

Abstract. Black carbon aerosol (BC), which is emitted from natural and anthropogenic sources (e.g., wildfires, coal burning), can contribute to magnify climate warming at high latitudes by darkening snow- and ice-covered surfaces, and subsequently lowering their albedo. Therefore, modeling the atmospheric transport and deposition of BC to the Arctic is important, and historical archives of BC accumulation in polar ice can help to validate such modeling efforts. Here we present a > 250-year ice-core record of refractory BC (rBC) deposition on Devon ice cap, Canada, spanning the years from 1735 to 1992. This is the first such record ever developed from the Canadian Arctic. The estimated mean deposition flux of rBC on Devon ice cap for 1963–1990 is 0.2 mg m−2 a−1, which is at the low end of estimates from Greenland ice cores obtained using the same analytical method ( ∼ 0.1–4 mg m−2 a−1). The Devon ice cap rBC record also differs from the Greenland records in that it shows only a modest increase in rBC deposition during the 20th century. In the Greenland records a pronounced rise in rBC is observed from the 1880s to the 1910s, which is largely attributed to midlatitude coal burning emissions. The deposition of contaminants such as sulfate and lead increased on Devon ice cap in the 20th century but no concomitant rise in rBC is recorded in the ice. Part of the difference with Greenland could be due to local factors such as melt–freeze cycles on Devon ice cap that may limit the detection sensitivity of rBC analyses in melt-impacted core samples, and wind scouring of winter snow at the coring site. Air back-trajectory analyses also suggest that Devon ice cap receives BC from more distant North American and Eurasian sources than Greenland, and aerosol mixing and removal during long-range transport over the Arctic Ocean likely masks some of the specific BC source–receptor relationships. Findings from this study suggest that there could be a large variability in BC aerosol deposition across the Arctic region arising from different transport patterns. This variability needs to be accounted for when estimating the large-scale albedo lowering effect of BC deposition on Arctic snow/ice.


2019 ◽  
Author(s):  
Bruna A. Holanda ◽  
Mira L. Pöhlker ◽  
Jorge Saturno ◽  
Matthias Sörgel ◽  
Jeannine Ditas ◽  
...  

Abstract. Black carbon (BC) aerosols are influencing the Earth’s atmosphere and climate, but their microphysical properties, spatiotemporal distribution and long-range transport are not well constrained. This study analyzes the transatlantic transport of BC-rich African biomass burning (BB) pollution into the Amazon Basin, based on airborne observations of aerosol particles and trace gases in and off the Brazilian coast during the ACRIDICON-CHUVA campaign in September 2014, combining in-situ measurements on the research aircraft HALO with satellite remote-sensing and numerical model results. During flight AC19 over land and ocean at the Brazilian coastline in the northeast of the Amazon Basin, we observed a BC-rich atmospheric layer at ~ 3.5 km altitude with a vertical extension of ~ 0.3 km. Backward trajectory analyses suggest that fires in African grasslands, savannas, and shrublands were the main source of this pollution layer, and that the observed BB smoke had undergone more than 10 days of atmospheric transport and aging. The BC mass concentrations in the layer ranged from 0.5 to 2 μg m−3, and the BC particle number fraction of ~ 40 % was about 8 times higher than observed in a fresh Amazonian BB plume, representing the highest value ever observed in the region. Upon entering the Amazon Basin, the layer started to broaden and to subside, due to convective mixing and entrainment of the BB aerosol into the boundary layer. Satellite observations show that the transatlantic transport of pollution layers is a frequently occurring process, seasonally peaking in August/September. By analyzing the aircraft observations within the broader context of the long-term data from the Amazon Tall Tower Observatory (ATTO), we found that the transatlantic transport of African BB smoke layers has a strong impact on the north-central Amazonian aerosol population during the BB-influenced season (July to November). Specifically, the early BB season in this part of the Amazon appears to be dominated by African smoke, whereas the later BB season appears to be dominated by South American fires. This dichotomy is reflected in pronounced changes of aerosol optical properties such as the single scattering albedo (increasing from 0.85 in August to 0.90 in November) and the BC-to-CO enhancement ratio (decreasing from 7.4 to 4.4 ng m−3 ppb−1). Our results suggest that, despite the high amount of BC particles, the African BB aerosol act as efficient cloud condensation nuclei (CCN) with potentially important implications for aerosol-cloud interactions and the hydrological cycle in the Amazon Basin.


2021 ◽  
Vol 17 (4) ◽  
pp. 1533-1545
Author(s):  
Delia Segato ◽  
Maria Del Carmen Villoslada Hidalgo ◽  
Ross Edwards ◽  
Elena Barbaro ◽  
Paul Vallelonga ◽  
...  

Abstract. Biomass burning influences global atmospheric chemistry by releasing greenhouse gases and climate-forcing aerosols. There is controversy about the magnitude and timing of Holocene changes in biomass burning emissions from millennial to centennial timescales and, in particular, about the possible impact of ancient civilizations. Here we present a 5 kyr record of fire activity proxies levoglucosan, black carbon, and ammonium measured in the RECAP (Renland ice cap) ice core, drilled in coastal eastern Greenland, and therefore affected by processes occurring in the high North Atlantic region. Levoglucosan and ammonium fluxes are high from 5 to 4.5 kyr BP (thousand years before 2000 CE) followed by an abrupt decline, possibly due to monotonic decline in Northern Hemisphere summer insolation. Levoglucosan and black carbon show an abrupt decline at 1.1 kyr BP, suggesting a decline in the wildfire regime in Iceland due to the extensive land clearing caused by Viking colonizers. All fire proxies reach a minimum during the second half of the last century, after which levoglucosan and ammonium fluxes increase again, in particular over the last 200 years. We find that the fire regime reconstructed from RECAP fluxes seems mainly related to climatic changes; however over the last millennium human activities might have influenced wildfire frequency/occurrence substantially.


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