Investigation of reservoir age variations in Lake Druksiai caused by anthropogenic factors

Author(s):  
Laurynas Butkus ◽  
Rūta Barisevičiūtė ◽  
Justina Šapolaitė ◽  
Žilvinas Ežerinskis ◽  
Evaldas Maceika ◽  
...  

<p>The reservoir effect (RE) is defined as the difference between the radiocarbon isotope ratio (<sup>14</sup>C/<sup>12</sup>C) in the terrestrial and aquatic samples. Both natural processes and anthropogenic activities affecting carbon cycle in the water ecosystem can lead to changes in the RE. Therefore, reservoir effect studies can help to assess the impact of external factors on a hydrological system [1].</p><p>The aim of this research was to evaluate the impact of anthropogenic <sup>14</sup>C contamination from Ignalina nuclear power plant (Ignalina NPP, INPP) on the Lake Drūkšiai system. The lake water was used to cool the reactors of the INPP. The lake sediment and fish (both benthic and pelagic) scale samples were collected from the Drūkšiai lake. ABA (acid-base-acid) chemical pretreatment procedure was used to extract humin (HM) and humic acid (HA) fractions from the sediments. Radiocarbon measurements in these samples were performed using the accelerator mass spectrometer (AMS).</p><p>In 1963, increased concentrations of radiocarbon due to the testing of nuclear weapons showed that atmosphere-lake CO<sub>2</sub> exchange accounted for about 22% carbon in bottom sediments. During the first 15 years of operation of the Ignalina Nuclear Power Plant, <sup>14</sup>C-enriched dissolved inorganic carbon (DIC) was continuously released into Lake Druksiai. During that period, an average of about 0.24 GBq of radiocarbon was released per year. Measurements of radiocarbon concentrations in fish confirm that the <sup>14</sup>C contamination was in dissolved inorganic form.</p><p>Around 2000, <sup>14</sup>C-enriched DIC (2.3 GBq radiocarbon) was released into Lake Druksiai from Ignalina NPP. In addition, organic compounds were additionally released in the same year. These compounds were not <sup>14</sup>C-enriched but affected the interaction between humic and humic acids. Almost a decade after the end of operation of the Ignalina NPP, there is still some <sup>14</sup>C pollution (from INPP) remaining in Lake Druksiai. The concentration of radiocarbon in the bottom sediments is still higher than in the atmosphere. </p><p> </p><p>[1] R. Barisevičiūtė et al., Tracing Carbon Isotope Variations in Lake Sediments Caused by Environmental Factors During the Past Century: A Case Study of Lake Tapeliai, Lithuania, Radiocarbon 61(4), 885–903, (2019).</p>

2013 ◽  
Vol 10 (7) ◽  
pp. 4911-4925 ◽  
Author(s):  
Y. Choi ◽  
S. Kida ◽  
K. Takahashi

Abstract. The mechanism behind the dispersion of radionuclides released from the Fukushima Dai-ichi Nuclear Power Plant on March 2011 is investigated using a numerical model. This model is a Lagrangian particle tracking–ocean circulation coupled model that is capable of solving the movement and migration of radionuclides between seawater, particulates, and bottom sediments. Model simulations show the radionuclides dispersing rapidly into the interior of the North Pacific once they enter a meso-scale eddy. However, some radionuclides also remain near the coast, with spatial distribution depending strongly on the oceanic circulation during the first month after the release. Major adsorption to bottom sediments occurs during this first month and many of these radionuclides remain on the sea floor once they are adsorbed. Model results suggest that weak offshore advection during the first month will increase the adsorption of radionuclides to bottom sediments and decelerate the dispersion to the open ocean. If vertical mixing is weak, however, fewer radionuclides reach the sea floor and adsorb to bottom sediments. More radionuclides will then quickly disperse to the open ocean.


Water ◽  
2021 ◽  
Vol 13 (10) ◽  
pp. 1397
Author(s):  
Rūta Barisevičiūtė ◽  
Evaldas Maceika ◽  
Laurynas Juodis ◽  
Algirdas Pabedinskas ◽  
Justina Šapolaitė ◽  
...  

The Ignalina Nuclear Power Plant (INPP) in Lithuania is a rare case when lake water is used instead of river or sea water for cooling. Lake Drūkšiai with water residence time of 3–4 year and undisturbed sediment layers is a unique system to assess the impact of a nuclear facility on the aquatic ecosystem with a sufficiently high temporal resolution. We constructed a model of radiocarbon cycling processes in lake ecosystem which evaluates the 14C specific activity vertical distribution in two organic sediment fractions: alkali-soluble and alkali-insoluble. Model calculations proved that during the first 15 years of operation since 1983, 14C annual aqueous releases from the INPP were in water dissolved inorganic carbon form and varied in the range of 2.4 ÷ 3.7 × 108 Bq/year. The results of the modeling of hypothetic scenarios also showed that there was the only one episode of elevated releases from the INPP in 2000–2001, which changed the interaction between the two organic sediment fractions for the period of 2000–2006. It was caused most probably by released chemicals from INPP but not by 14C contamination. Interaction processes between both sediment fractions recovered to its original state after 2006, indicating that the released additional chemical compounds lake ecosystem have been cleaned-up.


2013 ◽  
Vol 10 (2) ◽  
pp. 3677-3705 ◽  
Author(s):  
Y. Choi ◽  
S. Kida ◽  
K. Takahasi

Abstract. The mechanism behind the dispersion of radionuclides released from the Fukushima Dai-ichi Nuclear Power Plant on March 2011 is investigated using a numerical model. This model is a Lagrangian particle tracking – ocean circulation coupled model that has the capability of solving the concentration of radionuclides for those dissolved in seawater and those adsorbed in particulates and bottom sediments. Model results show the radionuclides dispersing rapidly to the interior of the North Pacific along the Kuroshio Extension once they enter a meso-scale eddy. However, radionuclides are also found to remain near the coast with their spatial pattern depending strongly on the oceanic circulation during the first month of the release. This is when most of the adsorption to bottom sediments occurs. If the offshore advection were weak during this period, many radionuclides will be adsorbed to bottom sediments and remain on the coast for some time. If vertical mixing is weak, less radionuclide reach the sea floor and get adsorbed to bottom sediments. More radionuclides will then disperse to the open ocean.


2021 ◽  
Author(s):  
Yuichi Onda ◽  
Keisuke Taniguchi ◽  
Kazuya Yoshimura ◽  
Yoshifumi Wakiyama

<p>The Fukushima Daiichi Nuclear Power Plant (FDNPP) accident released the largest quantity of radiocaesium into the terrestrial environment since the Chernobyl nuclear accident. The surrounding land received 2.7 PBq of radiocaesium to forests, agricultural lands, grasslands, and urban areas, from which the radionuclides migrated through soil and waterways. In this presentation, the deposition and distribution of radionuclides, especially radiocaesium, in the terrestrial environment as a result of the FDNPP accident are discussed based on the past 10 years' intensive dataset. Anthropogenic activities such as rice and vegetable cultivation and residential activities in the upstream area have led to a rapid decline in the activity concertation of 137Cs of suspended sediment (SS) transport in the river network, and these declines directly control the dissolved 137Cs concentration in the river water. We outline the environmental and anthropogenic factors that influenced the subsequent transport and impacts of radionuclides through the environment. The environmental aftermath of the accident at Fukushima is compared to Chernobyl, and the relatively rapid remediation of the Fukushima region relative to the region surrounding Chernobyl will be explained.</p>


Radiocarbon ◽  
2014 ◽  
Vol 56 (3) ◽  
pp. 1107-1114 ◽  
Author(s):  
Zhongtang Wang ◽  
Dan Hu ◽  
Hong Xu ◽  
Qiuju Guo

Atmospheric CO2 and aquatic water samples were analyzed to evaluate the environmental 14C enrichment due to operation of the Qinshan nuclear power plant (NPP), where two heavy-water reactors and five pressurized-water reactors are employed. Elevated 14C-specific activities (2–26.7 Bq/kg C) were observed in the short-term air samples collected within a 5-km radius, while samples over 5 km were close to background levels. The 14C-specific activities of dissolved inorganic carbon (DIC) in the surface seawater samples ranged from 196.8 to 206.5 Bq/kg C (average 203.4 Bq/kg C), which are close to the background value. No elevated 14C level in surface seawater was found after 20 years of operation of Qinshan NPP, indicating that the 14C discharged was well diffused. The results of the freshwater samples show that excess 14C-specific activity (average 17.1 Bq/kg C) was found in surface water and well water samples, while no obvious 14C increase was found in drinking water (groundwater and tap water) compared to the background level.


2021 ◽  
Vol 2083 (2) ◽  
pp. 022020
Author(s):  
Jiahuan Yu ◽  
Xiaofeng Zhang

Abstract With the development of the nuclear energy industry and the increasing demand for environmental protection, the impact of nuclear power plant radiation on the environment has gradually entered the public view. This article combs the nuclear power plant radiation environmental management systems of several countries, takes the domestic and foreign management of radioactive effluent discharge from nuclear power plants as a starting point, analyses and compares the laws and standards related to radioactive effluents from nuclear power plants in France, the United States, China, and South Korea. In this paper, the management improvement of radioactive effluent discharge system of Chinese nuclear power plants has been discussed.


Author(s):  
Sang-Nyung Kim ◽  
Sang-Gyu Lim

The safety injection (SI) nozzle of a 1000MWe-class Korean standard nuclear power plant (KSNP) is fitted with thermal sleeves (T/S) to alleviate thermal fatigue. Thermal sleeves in KSNP #3 & #4 in Yeonggwang (YG) & Ulchin (UC) are manufactured out of In-600 and fitted solidly without any problem, whereas KSNP #5 & #6 in the same nuclear power plants, also fitted with thermal sleeves made of In-690 for increased corrosion resistance, experienced a loosening of thermal sleeves in all reactors except KSNP YG #5-1A, resulting in significant loss of generation availability. An investigation into the cause of the loosening of the thermal sleeves only found out that the thermal sleeves were subject to severe vibration and rotation, failing to uncover the root cause and mechanism of the loosening. In an effort to identify the root cause of T/S loosening, three suspected causes were analyzed: (1) the impact force of flow on the T/S when the safety SI nozzle was in operation, (2) the differences between In-600 and In-690 in terms of physical and chemical properties (notably the thermal expansion coefficient), and (3) the positioning error after explosive expansion of the T/S as well as the asymmetric expansion of T/S. It was confirmed that none of the three suspected causes could be considered as the root cause. However, after reviewing design changes applied to the Palo Verde nuclear plant predating KSNP YG #3 & #4 to KSNP #5 & #6, it was realized that the second design modification (in terms of groove depth & material) had required an additional explosive energy by 150% in aggregate, but the amount of gunpowder and the explosive expansion method were the same as before, resulting in insufficient explosive force that led to poor thermal sleeve expansion. T/S measurement data and rubbing copies also support this conclusion. In addition, it is our judgment that the acceptance criteria applicable to T/S fitting was not strict enough, failing to single out thermal sleeves that were not expanded sufficiently. Furthermore, the T/S loosening was also attributable to lenient quality control before and after fitting the T/S that resulted in significant uncertainty. Lastly, in a flow-induced vibration test planned to account for the flow mechanism that had a direct impact upon the loosening of the thermal sleeves that were not fitted completely, it was discovered that the T/S loosening was attributable to RCS main flow. In addition, it was proven theoretically that the rotation of the T/S was induced by vibration.


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