Accumulation of legacy fallout radionuclides in cryoconite on Isfallsglaciären (Arctic Sweden) and their downstream spatial distribution

The release of legacy contaminants such as fallout radionuclides (FRNs) in response to glacier retreat is a process that has received relatively little attention to date, yet may have consequences as a source of secondary contamination as glaciers melt and down-waste in response to a warming climate. The presence of FRNs in glacier-fed catchments is poorly understood in comparison to other contaminants, yet there is now emerging evidence from multiple regions of the global cryosphere for substantially augmented FRN activities in cryoconite. Here we report concentrated FRNs in both cryoconite and proglacial sediments from the Isfallsglaciären catchment in Arctic Sweden. Activities of some FRNs in cryoconite are 2 orders of magnitude above those found elsewhere in the catchment, and above the activities found in other environmental matrices outside of nuclear exclusion zones. We also describe the presence of the short-lived cosmogenic radionuclide 7Be in cryoconite samples, highlighting the importance of meltwater–sediment interactions in radionuclide accumulation in the ice surface environment. It is currently unknown whether high accumulations of fallout radionuclides in glaciers have the potential to impact local environmental quality through down-wasting and downstream transport of contaminants to the proglacial environment through interaction with sediments and meltwater. We thus recommend that future research in this field focusses on processes of accumulation of FRNs and other environmental contaminants in cryoconite and whether these contaminants are present in quantities harmful for downstream ecosystems.

A worldwide meta-analysis (1977–2020) of sediment core dating using fallout radionuclides including ¹³⁷Cs and ²¹⁰Pb_xs

Dating recent sediment archives (< 150 years) constitutes a prerequisite for environmental and climatic reconstructions. Radiocaesium (137Cs) emitted during thermonuclear bomb testing (∼ 1950–1980) and nuclear accidents and the decrease in excess lead-210 (210Pbxs) with depth are often combined to establish sediment core chronology. Although these methods have been widely used during the last several decades, there is a lack of structured and comprehensive worldwide synthesis of fallout radionuclide analyses used for dating sediment cores in environmental and Earth sciences. The current literature overview was based on the compilation of 573 articles published between 1977 and 2020, reporting the collection of 1351 individual dating sediment cores (the dataset can be accessed at https://doi.org/10.1594/PANGAEA.931493; Foucher et al., 2021). This review was conducted in order to map the locations where 137Cs fallout events were detected. These included the thermonuclear bomb testing peak in 1963, the Chernobyl accident in 1986, the Fukushima accident in 2011, and 24 additional events identified at 112 sites that led to local or regional radioactive releases (e.g., Sellafield accidents, Chinese nuclear tests). When 210Pbxs records were used along with 137Cs data, detailed information on the 210Pbxs age–depth models were also synthesized. With the current growing number of studies analyzing sediment cores and the increasing interest in the deployment of sediment fingerprinting techniques including radionuclides as potential discriminant properties, this spatialized synthesis provides a unique worldwide compilation for characterizing fallout radionuclide sources and levels at the global scale. This synthesis provides in particular a reference of 137Cs peak attribution for improving the sediment core dating, and it outlines the main questions that deserve attention in future research as well as the regions where additional 137Cs fallout investigations should be conducted in priority.

Assessing soil redistribution of forest and cropland sites in wet tropical Africa using ^239+240Pufallout radionuclides

Due to the rapidly growing population in tropical Africa, a substantial rise in food demand is predicted in upcoming decades, which will result in higher pressure on soil resources. However, there is limited knowledge on soil redistribution dynamics following land conversion into arable land in tropical Africa that is partly caused by infrastructure limitations for long-term landscape-scale monitoring. In this study, fallout radionuclides 239+240Pu are used to assess soil redistribution along topographic gradients at two cropland sites and at three nearby pristine forest sites located in the DR Congo, Uganda and Rwanda. In the study area, a 239+240Pu baseline inventory is found that is higher than typically expected for tropical regions (mean forest inventory 41 Bq m−2). Pristine forests show no indication of soil redistribution based on 239+240Pu along topographical gradients. In contrast, soil erosion and sedimentation on cropland reached up to 37 cm (81 Mg ha−1 yr−1) and 40 cm (87 Mg ha−1 yr−1) within the last 55 years, respectively. Cropland sites show high intra-slope variability with locations showing severe soil erosion located in direct proximity to sedimentation sites. This study shows the applicability of a valuable method to assess tropical soil redistribution and provides insight into soil degradation rates and patterns in one of the most socio-economically and ecologically vulnerable regions of the world.

A worldwide meta-analysis (1977–2020) of sediment core dating using fallout radionuclides including ¹³⁷Cs and ²¹⁰Pb_xs

Dating recent sediment archives (< 150 years) constitutes a prerequisite for environmental and climatic reconstructions. Radiocaesium (137Cs) emitted during thermonuclear bomb testing (~1950 ̶ 1980) and nuclear accidents, as well as the decrease of excess lead-210 (210Pbxs) with depth are often combined to establish sediment core chronology. Although these methods have been widely used during the last several decades, there is a lack of structured and comprehensive worldwide synthesis of fallout radionuclide analyses used for dating sediment cores in environmental and Earth sciences. The current literature overview was based on the compilation of 573 articles published between 1977 and 2020, reporting the collection of 1351 individual dating sediment cores (the dataset can be accessed at https://doi.pangaea.de/10.1594/PANGAEA.931493). This review was conducted in order to map the locations where 137Cs fallout events were detected. These included the thermonuclear bomb testing peak in 1963, the Chernobyl accident in 1986, the Fukushima accident in 2011, and 24 additional events identified in 112 sites that led to local radioactive releases (e.g. Sellafield accidents, Chinese nuclear tests). When 210Pbxs records were used along with 137Cs data, detailed information on the 210Pbxs age depth models were also synthesized. Multiple information including the core collection method, sediment properties, radionuclide analysis techniques and catchment characteristics were also compiled. With the current growing number of studies analyzing sediment cores and the increasing interest in the deployment of sediment fingerprinting techniques including radionuclides as potential discriminant properties, this spatialized synthesis provides a unique worldwide compilation for characterizing fallout radionuclide sources and levels at the global scale. This synthesis provides in particular a referential of 137Cs peak attribution for improving the sediment core dating and it outlines the main questions that deserve attention in future research as well as the regions where additional 137Cs fallout investigations should be conducted in priority.

Tracing erosion rates in loess landscape of the Trzebnica Hills (Poland) over time using fallout and cosmogenic nuclides

Purpose Loess landscapes are highly susceptible to soil erosion, which affects soil stability and productivity. Erosion is non-linear in time and space and determines whether soils form or degrade. While the spatial variability of erosion is often assessed by either modelling or on-site measurements, temporal trends over decades to millennia are very often lacking. In this study, we determined long- and short-term erosion rates to trace the dynamics of loess deposits in south-western Poland. Materials and methods We quantified long-term (millennial) erosion rates using cosmogenic (in situ 10Be) and short-term (decadal) rates with fallout radionuclides (239+240Pu). Erosion processes were studied in two slope-soil transects (12 soil pits) with variable erosion features. As a reference site, an undisturbed soil profile under natural forest was sampled. Results and discussion The long-term erosion rates ranged between 0.44 and 0.85 t ha−1 year−1, whereas the short-term erosion rates varied from 1.2 to 10.9 t ha−1 year−1 and seem to be reliable. The short-term erosion rates are up to 10 times higher than the long-term rates. The soil erosion rates are quite consistent with the terrain relief, with erosion increasing in the steeper slope sections and decreasing in the lower parts of the slope, while still maintaining high values. Conclusions Soil erosion rates have increased during the last few decades owing to agriculture intensification and probably climate change. The measured values lie far above tolerable erosion rates, and the soils were found to be strongly imbalanced and exhibit a drastic shallowing of the productive soils horizons.

Hyper-accumulation of legacy fallout radionuclides in cryoconite on Isfallsglaciären (Arctic Sweden) and their downstream distribution

The release of legacy fallout radionuclides (FRNs) in response to glacier retreat is a process that has received relatively little attention to date, yet may have important consequences as a source of secondary contamination as glaciers melt and down-waste in response to a warming climate. The prevalence of FRNs in glacier-fed catchments is poorly understood in comparison to other contaminants, yet there is now emerging evidence from multiple regions of the global cryosphere for substantially augmented FRN activities in cryoconite. Here we report concentrated FRNs in both cryoconite and proglacial sediments from the Isfallsglaciären catchment in Arctic Sweden. Activities of some FRNs in cryoconite are two orders of magnitude above those found elsewhere in the catchment, and above the activities found in other environmental matrices outside of nuclear exclusion zones. We also describe the presence of the short-lived cosmogenic radionuclide 7Be in cryoconite samples, highlighting the importance of meltwater-sediment interactions in radionuclide accumulation in the ice surface environment. The presence of fallout radionuclides in glaciers may have the potential to impact local environmental quality through both isolated hotspots of radioactivity caused by glacier down-wasting, and downstream transport of contaminants to the proglacial environment through interaction with sediments and meltwater. We thus recommend that future research in this field focusses on processes of accumulation of FRNs and other environmental contaminants in cryoconite, and whether these contaminants are present in quantities harmful for both local and downstream ecosystems.