On Surface-Plasmon-Polariton Waves Excited in the Turbadar–Otto Configuration

A local minimum in the plot of linear reflectance versus angle of incidence, on its own, is insufficient to identify a surface-plasmon-polariton wave (SPPW). Further checks are required in order to confirm the identity of a SPPW. The wavenumber should be compared with that extracted from the dispersion relation for the corresponding canonical boundary-value problem. Also, for prism-coupled configurations such as the Turbadar–Otto configuration which are based on SPPW-excitation via evanescent waves, the angle of incidence should be greater than the critical angle needed for total internal reflection.

Spatiotemporal imaging of 2D polariton wave packet dynamics using free electrons

Coherent optical excitations in two-dimensional (2D) materials, 2D polaritons, can generate a plethora of optical phenomena that arise from the extraordinary dispersion relations that do not exist in regular materials. Probing of the dynamical phenomena of 2D polaritons requires simultaneous spatial and temporal imaging capabilities and could reveal unknown coherent optical phenomena in 2D materials. Here, we present a spatiotemporal measurement of 2D wave packet dynamics, from its formation to its decay, using an ultrafast transmission electron microscope driven by femtosecond midinfrared pulses. The ability to coherently excite phonon-polariton wave packets and probe their evolution in a nondestructive manner reveals intriguing dispersion-dependent dynamics that includes splitting of multibranch wave packets and, unexpectedly, wave packet deceleration and acceleration. Having access to the full spatiotemporal dynamics of 2D wave packets can be used to illuminate puzzles in topological polaritons and discover exotic nonlinear optical phenomena in 2D materials.