The presented modelling results in this article show that electrochemical CO2 reduction performed at commercially-relevant current densities will ultimately lead to locally alkaline reaction conditions regardless of the electrolyte, configuration and reasonable mass transport scenarios. Discussed in detail are the large implications that this result has for the CO2 reduction reaction itself, and the current way in which catalysts are designed and tested in different electrochemical cell architectures.
The presented modelling results in this article show that electrochemical CO2 reduction performed at commercially-relevant current densities will ultimately lead to locally alkaline reaction conditions regardless of the electrolyte, configuration and reasonable mass transport scenarios. Discussed in detail are the large implications that this result has for the CO2 reduction reaction itself, and the current way in which catalysts are designed and tested in different electrochemical cell architectures.
Metal-organic framework (MOF) derived single-atom catalysts (SACs), featured unique active sites and adjustable topological structures, exhibit high electrocatalytic performance on carbon dioxide reduction reactions (CO2RR). By modulating elements and atomic...
Electrochemical CO2 reduction reaction (CO2RR) is a very important approach to realize sustainable development. Single-atom catalysts show advantages in both homogeneous and heterogeneous catalysis, and considerable progress has been made...
The direct production of syngas via electrochemical CO2 reduction reaction (CO2RR) is a highly potential process for its environmental-friendly and product adjustability advantages. However, it is challenging to synthesize syngas...
Enhancing Electrocatalytic CO2 Reduction Using a System-Integrated Approach to Catalyst Discovery
