scholarly journals Nonplasmonic Hot-Electron Photocurrents from Mn-Doped Quantum Dots in Photoelectrochemical Cells

ChemPhysChem ◽  
2016 ◽  
Vol 17 (5) ◽  
pp. 660-664 ◽  
Author(s):  
Yitong Dong ◽  
Daniel Rossi ◽  
David Parobek ◽  
Dong Hee Son
JETP Letters ◽  
2019 ◽  
Vol 109 (4) ◽  
pp. 270-275
Author(s):  
A. F. Zinovieva ◽  
V. A. Zinovyev ◽  
N. P. Stepina ◽  
A. V. Katsuba ◽  
A. V. Dvurechenskii ◽  
...  

Author(s):  
Wenbin Xiang ◽  
Yufen Yuan ◽  
Hongyu Yang ◽  
Yi Zhang ◽  
Jiayu Zhang

2006 ◽  
Vol 243 (15) ◽  
pp. 3912-3916 ◽  
Author(s):  
Y. Léger ◽  
L. Besombes ◽  
L. Maingault ◽  
J. Fernández-Rossier ◽  
D. Ferrand ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Junhui Wang ◽  
Lifeng Wang ◽  
Shuwen Yu ◽  
Tao Ding ◽  
Dongmei Xiang ◽  
...  

AbstractUnderstanding and manipulating hot electron dynamics in semiconductors may enable disruptive energy conversion schemes. Hot electrons in bulk semiconductors usually relax via electron-phonon scattering on a sub-picosecond timescale. Quantum-confined semiconductors such as quantum dots offer a unique platform to prolong hot electron lifetime through their size-tunable electronic structures. Here, we study hot electron relaxation in electron-doped (n-doped) colloidal CdSe quantum dots. For lightly-doped dots we observe a slow 1Pe hot electron relaxation (~10 picosecond) resulting from a Pauli spin blockade of the preoccupying 1Se electron. For heavily-doped dots, a large number of electrons residing in the surface states introduce picosecond Auger recombination which annihilates the valance band hole, allowing us to observe 300-picosecond-long hot electrons as a manifestation of a phonon bottleneck effect. This brings the hot electron energy loss rate to a level of sub-meV per picosecond from a usual level of 1 eV per picosecond. These results offer exciting opportunities of hot electron harvesting by exploiting carrier-carrier, carrier-phonon and spin-spin interactions in doped quantum dots.


2005 ◽  
Vol 72 (24) ◽  
Author(s):  
Y. Léger ◽  
L. Besombes ◽  
L. Maingault ◽  
D. Ferrand ◽  
H. Mariette

2016 ◽  
Vol 93 (16) ◽  
Author(s):  
V. Moldoveanu ◽  
I. V. Dinu ◽  
R. Dragomir ◽  
B. Tanatar

2017 ◽  
Vol 95 (20) ◽  
Author(s):  
L. Cabral ◽  
Fernando P. Sabino ◽  
Vivaldo Lopes-Oliveira ◽  
Juarez L. F. Da Silva ◽  
Matheus P. Lima ◽  
...  

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