Uncertainty of decay heat calculations originating from errors in the nuclear data and the yields of individual fission products

1980 ◽  
Vol 55 (1) ◽  
pp. 79-99 ◽  
Author(s):  
G. Rudstam
2019 ◽  
Vol 211 ◽  
pp. 01001
Author(s):  
M. Estienne ◽  
M. Fallot ◽  
L. Giot ◽  
V. Guadilla-Gomez ◽  
L. Le Meur ◽  
...  

Three observables of interest for present and future reactors depend on the β decay properties of the fission products: antineutrinos from reactors, the reactor decay heat and delayed neutron emission. In these proceedings, we present new results from summation calculations of the first two quantities quoted above, performed with evolved independent yields coupled with fission product decay data, from various nuclear data bases or models. New TAGS results from the latest experiment of the TAGS collaboration at the JYFL facility of Jyväskylä will be displayed as well as their impact on the antineutrino spectra and the decay heat associated to fission pulses of the main actinides.


2018 ◽  
Vol 4 ◽  
pp. 24
Author(s):  
Magali Estienne ◽  
Muriel Fallot ◽  
Lydie Giot ◽  
Loïc Le Meur ◽  
Amanda Porta

Three observables of interest for present and future reactors depend on the β decay data of the fission products: the reactor decay heat, antineutrinos from reactors and delayed neutron emission. Concerning the decay heat, significant discrepancies still exist between summation calculations in − their two main ingredients: the decay data and the fission yields − performed using the most recent evaluated databases available. It has been recently shown that the associated uncertainties are dominated by the ones on the decay data. But the results subtantially differ taking into account or not the correlations between the fission products. So far the uncertainty propagation does not include as well systematic effects on nuclear data such as the Pandemonium effect which impacts a large number of nuclei contributing to the decay heat. The list of nuclei deserving new TAGS measurements has been updated recently in the frame of IAEA working groups. The issues listed above impact in the same way the predicted energy spectra of the antineutrinos from reactors computed with the summation method, the interest of which has been recently reinforced by the Daya Bay latest publication. Nuclear data should definitely contribute to refine and better control these calculations. Lastly, a lot of nuclear data related to delayed neutrons are missing in nuclear databases. Despite the progresses already done these last years with new measurements now requiring to be included in evaluated databases, the experimental efforts which still need to be done are significant. These different issues will be addressed here before to comment on recent experimental results and on their impacts on the quoted observables. Some perspectives will also be presented. Solving the issues listed above will require to bring together experimental, simulation, evaluation and theoretical activities.


2021 ◽  
Vol 247 ◽  
pp. 10002
Author(s):  
V. Vallet ◽  
J. Huyghe ◽  
C. Vaglio-Gaudard ◽  
D. Lecarpentier ◽  
C. Reynard-Carette

Currently there is no integral experimental data for code validation regarding the decay heat of MOX fuels, excepted fission burst experiments (for fission products contributions at short cooling times) or post-irradiated experiments on nuclide inventories (restricted number of nuclide of interest for decay heat). The uncertainty quantification mainly relies on uncertainty propagation of nuclear data covariances. In the recent years, the transposition method, based on the data assimilation theory, was used in order to transpose the experiment-to-calculation discrepancies at a given set of parameters (cooling time, fuel burnup) to another set of parameters. As an example, this method was used on the CLAB experiments and the experiment-to-calculation discrepancies at 13 years were transposed to an UOX fuel between 5 and 27 years and for burnups from 10 to 50 GWd/t. The purpose of this paper is to study to what extent the transposition method could be used for MOX fuels. In particular, the Dickens fission burst experiment of 239Pu was considered for MOX fuels at short cooling times (< 1h30) and low burnup (< 10 GWd/t). The impact of fission yields (FY) correlations was also discussed. As a conclusion, the efficiency of the transposition process is limited by the experimental uncertainties larger than nuclear data uncertainties, and by the fact that fission burst experiments would only be representative to the FY contribution of the decay heat uncertainty of an irradiated reactor fuel. Nevertheless, this method strengthens the decay heat uncertainties at very short cooling times, previously based only on nuclear data covariance propagation through computation.


Separations ◽  
2021 ◽  
Vol 8 (7) ◽  
pp. 104
Author(s):  
Leah M. Arrigo ◽  
Jun Jiang ◽  
Zachary S. Finch ◽  
James M. Bowen ◽  
Staci M. Herman ◽  
...  

The measurement of radioactive fission products from nuclear events has important implications for nuclear data production, environmental monitoring, and nuclear forensics. In a previous paper, the authors reported the optimization of an intra-group lanthanide separation using LN extraction resin from Eichrom Technologies®, Inc. and a nitric acid gradient. In this work, the method was demonstrated for the separation and quantification of multiple short-lived fission product lanthanide isotopes from a fission product sample produced from the thermal irradiation of highly enriched uranium. The separations were performed in parallel in quadruplicate with reproducible results and high decontamination factors for 153Sm, 156Eu, and 161Tb. Based on the results obtained here, the fission yields for 144Ce, 153Sm, 156Eu, and 161Tb are consistent with published fission yields. This work demonstrates the effectiveness of the separations for the intended application of short-lived lanthanide fission product analysis requiring high decontamination factors.


Author(s):  
Antonio Jiménez-Carrascosa ◽  
Nuria Garcia Herranz ◽  
Jiri Krepel ◽  
Marat Margulis ◽  
Una Baker ◽  
...  

Abstract In this work a detailed assessment of the decay heat power for the commercial-size European Sodium-cooled Fast Reactor (ESFR) at the end of its equilibrium cycle has been performed. The summation method has been used to compute very accurate spatial- and time-dependent decay heat by employing state-of-the-art coupled transport-depletion computational codes and nuclear data. This detailed map provides basic information for subsequent transient calculations of the ESFR. A comprehensive analysis of the decay heat has been carried out and interdependencies among decay heat and different parameters characterizing the core state prior to shutdown, such as discharge burnup or type of fuel material, have been identified. That analysis has served as a basis to develop analytic functions to reconstruct the spatial-dependent decay heat power for the ESFR for cooling times within the first day after shutdown.


1979 ◽  
Vol 46 (2) ◽  
pp. 323-331 ◽  
Author(s):  
Virgil E. Schrock
Keyword(s):  

2020 ◽  
Vol 242 ◽  
pp. 01002
Author(s):  
Adam Hecht ◽  
Phoenix Baldez ◽  
Baldez Baldez

The University of New Mexico Fission Spectrometer was developed to measure fission product yield, as part of the LANL SPIDER collaboration. The spectrometer operates as an E-v detector to extract product mass event-by-event, with a time of flight region followed by an ionization chamber for kinetic energy measurements. By using the ionization chamber as a singlecathode/single-anode time projection chamber, stopping power and thus Z information is extracted, for coupled A and Z measurements. New work is being performed to add gamma ray detectors in the data stream, placed near the target region for prompt gammas and near the ionization chamber for quasiprompt (>50 ns) and later gammas, correlated with individual fission products. A stand-alone parallel plate ionization chamber (PPIC) is also being developed for fission tagging gamma ray data. The PPIC will also allow discrimination between charged particle out events and (n,n’γ), and discriminate between alpha emission and fission. Using layers in the PPIC, other targets can be measured simultaneously with a calibration target, giving relative fission cross sections. Past measurements with the spectrometer were performed at LANSCE and we plan to continue measurements there. The current work is supported by the NNSA Stewardship Science Academic Alliance.


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