scholarly journals Evaluation of a sensitive, reasonable, and fast detection method for 55Fe in steel

2021 ◽  
Author(s):  
Silke Merchel ◽  
Georg Rugel ◽  
Johannes Lachner ◽  
Anton Wallner ◽  
Diana Walther ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Pilot Study ◽  
Neutron Capture ◽  
Nuclear Power ◽  
Liquid Scintillation ◽  
Detection Method ◽  
Reactor Vessel ◽  
Scintillation Counting ◽  
Measuring Time ◽  
Fast Detection

AbstractA pilot study to quantify 55Fe in steel from a reactor vessel of a nuclear power plant by accelerator mass spectrometry (AMS) without any chemical sample preparation was validated by liquid scintillation counting (LSC) and AMS after radiochemical separation. AMS reaches an uncertainty < 10% at the 1 kBq gFe−1 level within less than 10 min measuring time. The background was < 3 Bq gFe−1, presently limited by the short measurement time. The new instrumental AMS method for analysing 55Fe from neutron capture production is reasonable and fast compared to other analytical methods.

scholarly journals 14C Release in Various Chemical Forms With Gaseous Effluents From the Paks Nuclear Power Plant

Radiocarbon ◽  
1989 ◽  
Vol 31 (03) ◽  
pp. 754-761 ◽  
Author(s):  
Ede Hertelendi ◽  
György Uchrin ◽  
Peter Ormai
Keyword(s):  
Power Plant ◽  
Nuclear Power Plant ◽  
Nuclear Power ◽  
Liquid Scintillation ◽  
Mean Value ◽  
Scintillation Counting ◽  
Pressurized Water ◽  
The Mean ◽  
Water Reactors

We present results of airborne 14C emission measurements from the Paks PWR nuclear power plant. Long-term release of 14C in the form of carbon dioxide or carbon monoxide and hydrocarbons were simultaneously measured. The results of internal gas-proportional and liquid scintillation counting agree well with theoretical assessments of 14C releases from pressurized water reactors. The mean value of the 14C concentration in discharged air is 130Bqm-3 and the normalized release is equal to 740GBq/GWe · yr. &gt; 95% of 14C released is in the form of hydrocarbons, ca 4% is apportioned to CO2, and &lt;1% to CO. Tree-ring measurements were also made and indicated a minute increase of 14C content in the vicinity of the nuclear power plant.

The Brazilian AMS Radiocarbon Laboratory (LAC-UFF) and the Intercomparison of Results with CENA and UGAMS

Radiocarbon ◽  
2013 ◽  
Vol 55 (2) ◽  
pp. 325-330 ◽  
Author(s):  
K D Macario ◽  
P R S Gomes ◽  
R M Anjos ◽  
C Carvalho ◽  
R Linares ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Latin America ◽  
Liquid Scintillation Counting ◽  
Nuclear Energy ◽  
Liquid Scintillation ◽  
Scintillation Counting ◽  
Physics Institute ◽  
University Of Georgia ◽  
The University ◽  
Good Agreement

After 22 yr of the low-level liquid scintillation counting 14C laboratory at the Center for Nuclear Energy in Agriculture (CENA) at São Paulo University (USP), Piracicaba, Brazil, and several collaborative projects with Brazilian and international researchers from distinct scientific areas, the first 14C accelerator mass spectrometry (AMS) laboratory in Latin America was installed at the Physics Institute of the Universidade Federal Fluminense (UFF), Niterói, Brazil. A 250kV single stage accelerator produced by National Electrostatics Corporation began its operation in 2012. In this work, we compare measurements performed at the AMS Radiocarbon Laboratory at UFF (LAC-UFF) with those performed at CENA and the University of Georgia (UGAMS), Georgia, USA. All the results obtained from distinct inorganic and organic samples were in very good agreement.

scholarly journals A Review of the Radiocarbon Dates for the Afanasyevo Culture (Central Asia): Shifting Towards the “Shorter” Chronology

Radiocarbon ◽  
2018 ◽  
Vol 61 (1) ◽  
pp. 243-263 ◽  
Author(s):  
Andrey V Poliakov ◽  
Svetlana V Svyatko ◽  
Nadezhda F Stepanova
Keyword(s):  
Mass Spectrometry ◽  
Accelerator Mass Spectrometry ◽  
Liquid Scintillation Counting ◽  
Liquid Scintillation ◽  
Scintillation Counting ◽  
Radiocarbon Dates ◽  
Archaeological Data ◽  
Depth Analysis ◽  
Over Time ◽  
Ams Dates

ABSTRACTThis article provides a summary and in-depth analysis of all existing radiocarbon (14C) dates for the Afanasyevo Culture of the Paleometal period. The previous “long” chronology of the culture was widely criticized and contradicted many archaeological observations. The exceedingly wide ranges of the liquid scintillation counting (LSC) dates from bone samples produced in several laboratories and the systematically older ages for the wood/charcoal samples finally reveal the shortcomings of the conventional “long” chronology. From accelerator mass spectrometry (AMS), the Afanasyevo burials of the Altai are dated to the 31st–29th century BC, whereas those of the Middle Yenisei Region to the 29th–25th century BC, which confirms the relatively earlier age of the Altai monuments. The “short” chronology removes the incompatibility of deriving the Afanasyevo Culture from the Yamnaya Culture, which previously appeared “younger” than the Afanasyevo, and also contradictions with the archaeological data. It also explains the small number of sites, the small size of the cemeteries and the lack of the internal periodization. We can now clearly move, from the earlier understanding that the Afanasyevo chronology is too broad, towards a different perception. The new AMS dates only represent a “core” for the Afanasyevo chronology, which cannot be narrowed down, but could be slightly expanded over time.

scholarly journals Comparison of 14C Ages Between LSC and AMS Measurements of Choukai Jindai Cedar Tree Rings at 2600 cal BP

Radiocarbon ◽  
2010 ◽  
Vol 52 (3) ◽  
pp. 895-900 ◽  
Author(s):  
Yui Takahashi ◽  
Hirohisa Sakurai ◽  
Kayo Suzuki ◽  
Taiichi Sato ◽  
Shuichi Gunji ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Tree Rings ◽  
Liquid Scintillation ◽  
Measurement Methods ◽  
Scintillation Counting ◽  
Age Difference ◽  
Data Sets ◽  
Data Set ◽  
The Difference ◽  
Good Agreement

Radiocarbon ages of Choukai Jindai cedar tree rings growing in the excess era of 14C concentrations during 2757–2437 cal BP were measured using 2 types of 14C measurement methods, i.e. liquid scintillation counting (LSC) and accelerator mass spectrometry (AMS). The difference between the 2 methods is 3.7 ± 5.2 14C yr on average for 61 single-year tree rings, indicating good agreement between the methods. The Choukai data sets show a small sharp bump with an average 14C age of 2497.1 ± 3.0 14C yr BP during 2650–2600 cal BP. Although the profile of the Choukai LSC data set compares well with that of IntCal04, having a 14C age difference of 4.6 ± 5.3 14C yr on average, the Choukai LSC 14C ages indicate variability against the smoothed profile of IntCal04.

Measuring 14C Concentration in Wine to Monitor Global Distribution of 14C

Radiocarbon ◽  
2013 ◽  
Vol 55 (3) ◽  
pp. 1827-1833
Author(s):  
Hirohisa Sakurai ◽  
Saori Namai ◽  
Emiko Inui ◽  
Fuyuki Tokanai ◽  
Kazuhiro Kato ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Correlation Coefficient ◽  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Accelerator Mass Spectrometry ◽  
Liquid Scintillation Counting ◽  
Liquid Scintillation ◽  
Fossil Fuel ◽  
Scintillation Counting ◽  
Northern And Southern Hemispheres

Using liquid scintillation counting (LSC) and accelerator mass spectrometry (AMS), radiocarbon concentrations were measured for wine from 8 wineries located in 7 countries in the Northern and Southern hemispheres. The 14C concentrations of ethanol and residual materials in the wine were correlated (correlation coefficient 0.82). The δ14C measurements of wine samples from the mid-latitudes in the Northern Hemisphere were approximately 1l% lower than the extrapolations from Schauinsland data, suggesting a local fossil fuel effect. δ14C measurements from the wine samples from the Southern Hemisphere were higher than those from the Northern Hemisphere. The offsets of the 4 wine δ14C measurements were significant, with values between approximately 8% and 15%. Because the harvest years of the mixed grapes were estimated to be 7–12 yr older than their vintage years, this leads to a caveat when determining the 14C concentrations of the year using the wine vintage.

Comparative Dendrochronological and14C Dating of 15th Century Russian Icon

Radiocarbon ◽  
2015 ◽  
Vol 57 (1) ◽  
pp. 173-182 ◽  
Author(s):  
Konstantin Voronin ◽  
Andrey Dolgikh ◽  
Vladimir Matskovsky ◽  
Alexander Cherkinsky ◽  
Vadim Skripkin ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Calibration Curve ◽  
Liquid Scintillation Counting ◽  
Liquid Scintillation ◽  
Fine Art ◽  
Scintillation Counting ◽  
13Th Century ◽  
15Th Century ◽  
Complete Tree ◽  
Ams Dates

A 15th century Russian icon from the Novgorod region was analyzed using both dendrochronological and radiocarbon methods [liquid scintillation counting (LSC) and accelerator mass spectrometry (AMS)]. This orthodox icon represents the Mother of God (Dexiokratusa). Fine art experts attribute the icon to between the late 14th to the early 15th centuries. The last complete tree ring was dated to AD 1409. There are indications that the trees were cut down during the summer of AD 1410. Taking into account the time for seasoning (about 8 months), the icon would have been painted in AD 1411. Wiggle-matching of the six AMS samples failed. Two of six AMS dates correspond to dendrochronological dates, while four of the six AMS dates showed differences with the dendrochronological dates by 5–39 yr. This discrepancy raises the issue of a possible regional offset from the calibration curve for the 13th century AD in NW Russia.

scholarly journals Gas Proportional Versus Liquid Scintillation Counting, Radiometric Versus AMS Dating

Radiocarbon ◽  
1991 ◽  
Vol 33 (1) ◽  
pp. 9-13 ◽  
Author(s):  
Páll Theodórsson
Keyword(s):  
Mass Spectrometry ◽  
Radiocarbon Dating ◽  
Liquid Scintillation ◽  
Scintillation Counting ◽  
Comparison Of Methods ◽  
Mass Spectrometry Technique ◽  
Single Detector ◽  
Ams Dating ◽  
Spectrometry Technique ◽  
Single Figure

I discuss here the basis of a comparison of methods for radiocarbon dating and introduce a new index for the relative merit of a system, factor of counting capacity, that is generally more appropriate than the commonly used factor of merit. The merit of a dating system cannot be based on a single figure but other factors must also be considered. A comparison of the gas proportional, liquid scintillation and accelerator mass spectrometry technique is presented that for gas proportional counters is based on a multi-detector system rather than a single detector.

Optical Detection of Radiocarbon Dioxide: First Results and AMS Intercomparison

Radiocarbon ◽  
2013 ◽  
Vol 55 (2) ◽  
pp. 213-223 ◽  
Author(s):  
I Galli ◽  
S Bartalini ◽  
P Cancio ◽  
P De Natale ◽  
D Mazzotti ◽  
...  
Keyword(s):  
Mass Spectrometry ◽  
Liquid Scintillation ◽  
Scintillation Counting ◽  
Perfect Agreement ◽  
Measured Concentration ◽  
Mid Infrared ◽  
Future Developments ◽  
Carbon Dioxide Gas ◽  
Infrared Laser Spectroscopy ◽  
First Results

The first results of an optical method for measuring radiocarbon concentrations, based on mid-infrared laser spectroscopy of a carbon dioxide gas sample, are presented with the theoretical bases explained in detail. The first measurements on modern and highly enriched samples show the extreme linearity of this technique over more than 5 decades. An intercomparison with accelerator mass spectrometry (AMS) is performed both for modern and 14C-dead samples, assessing the almost perfect agreement of their respectively measured concentration values. The main features of our technique are compared with liquid scintillation counting (LSC) and AMS, and future developments of the current setup are discussed.

Sign in / Sign up

Export Citation Format

Share Document