Stochastic Analysis of the Gas Flow at the Gas Diffusion Layer/Electrode Interface of a High-Temperature Polymer Electrolyte Fuel Cell

2018 ◽  
Vol 123 (2) ◽  
pp. 403-420 ◽  
Author(s):  
Dieter Froning ◽  
Junliang Yu ◽  
Uwe Reimer ◽  
Werner Lehnert
Keyword(s):  
High Temperature ◽  
Fuel Cell ◽  
Polymer Electrolyte ◽  
Diffusion Layer ◽  
Stochastic Analysis ◽  
Gas Flow ◽  
Gas Diffusion Layer ◽  
Gas Diffusion ◽  
Polymer Electrolyte Fuel Cell ◽  
Electrode Interface

scholarly journals Quantifying phosphoric acid in high-temperature polymer electrolyte fuel cell components by X-ray tomographic microscopy

2014 ◽  
Vol 21 (6) ◽  
pp. 1319-1326 ◽  
Author(s):  
S. H. Eberhardt ◽  
F. Marone ◽  
M. Stampanoni ◽  
F. N. Büchi ◽  
T. J. Schmidt
Keyword(s):  
High Temperature ◽  
Fuel Cell ◽  
Phosphoric Acid ◽  
Polymer Electrolyte ◽  
Diffusion Layer ◽  
Gas Diffusion Layer ◽  
Gas Diffusion ◽  
X Ray ◽  
Wide Range ◽  
Cell Components

Synchrotron-based X-ray tomographic microscopy is investigated for imaging the local distribution and concentration of phosphoric acid in high-temperature polymer electrolyte fuel cells. Phosphoric acid fills the pores of the macro- and microporous fuel cell components. Its concentration in the fuel cell varies over a wide range (40–100 wt% H3PO4). This renders the quantification and concentration determination challenging. The problem is solved by using propagation-based phase contrast imaging and a referencing method. Fuel cell components with known acid concentrations were used to correlate greyscale values and acid concentrations. Thus calibration curves were established for the gas diffusion layer, catalyst layer and membrane in a non-operating fuel cell. The non-destructive imaging methodology was verified by comparing image-based values for acid content and concentration in the gas diffusion layer with those from chemical analysis.

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