scholarly journals Anthropogenic Aerosol Influences on Mixed-Phase Clouds

2017 ◽  
Vol 3 (1) ◽  
pp. 32-44 ◽  
Author(s):  
Ulrike Lohmann
Keyword(s):  
Mixed Phase ◽  
Anthropogenic Aerosol ◽  
Mixed Phase Clouds

scholarly journals Sensitivity studies of different aerosol indirect effects in mixed-phase clouds

2009 ◽  
Vol 9 (4) ◽  
pp. 15045-15081
Author(s):  
U. Lohmann ◽  
C. Hoose
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Mixed Phase ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Activation Effect ◽  
Aerosol Effect ◽  
Sensitivity Studies ◽  
Mixed Phase Clouds

Abstract. Aerosols affect the climate system by changing cloud characteristics. Using the global climate model ECHAM5-HAM, we investigate different aerosol effects on mixed-phase clouds: The glaciation effect, which refers to a more frequent glaciation due to anthropogenic aerosols, versus the de-activation effect, which suggests that ice nuclei become less effective because of an anthropogenic sulfate coating. The glaciation effect can partly offset the indirect aerosol effect on warm clouds and thus causes the total anthropogenic aerosol effect to be smaller. It is investigated by varying the parameterization for the Bergeron-Findeisen process and the threshold coating thickness of sulfate (SO4-crit), which is required to convert an externally mixed aerosol particle into an internally mixed particle. Differences in the net radiation at the top-of-the-atmosphere due to anthropogenic aerosols between the different sensitivity studies amount up to 0.5 W m−2. This suggests that the investigated mixed-phase processes have a major effect on the total anthropogenic aerosol effect.

scholarly journals On-line single particle analysis of ice particle residuals from mountain-top mixed-phase clouds using laboratory derived particle type assignment

2016 ◽  
Author(s):  
S. Schmidt ◽  
J. Schneider ◽  
T. Klimach ◽  
S. Mertes ◽  
L. P. Schenk ◽  
...  
Keyword(s):  
Single Particle ◽  
Aerosol Particles ◽  
Mixed Phase ◽  
Particle Analysis ◽  
Single Particle Analysis ◽  
Particle Type ◽  
Industrial Emissions ◽  
Anthropogenic Aerosol ◽  
Outcome Instrument ◽  
Mixed Phase Clouds

Abstract. In-situ single particle analysis of ice particle residuals (IPR) and out-of-cloud aerosol particles was conducted by means of laser ablation mass spectrometry during the intensive INUIT-JFJ/CLACE campaign at the high alpine research station Jungfraujoch (3580 m a.s.l.) in January/February 2013. During the four week campaign more than 70000 out-of-cloud aerosol particles and 595 IPR were analyzed covering a particle size diameter range from 100 nm to 3 µm. The IPR were sampled during 273 hours while the station was covered by mixed-phase clouds at ambient temperatures between −27 °C and −6 °C. The identification of particle types is based on laboratory studies of different types of biological, mineral and anthropogenic aerosol particles. As outcome instrument specific marker peaks for the different investigated particle types were obtained and applied to the field data. The results show that the sampled IPR contain a larger relative amount of natural, primary aerosol, like soil dust (13 %) and minerals (11 %), in comparison to out-of-cloud aerosol particles (2 % and < 1 %, respectively). Additionally, anthropogenic aerosol particles, like particles from industrial emissions and lead-containing particles, were found to be more abundant in the IPR than in the out-of-cloud aerosol. The out-of-cloud aerosol contained a large fraction of aged particles (30 %, including organic material and secondary inorganics), whereas this particle type was much less abundant (3 %) in the IPR. In a selected subset of the data where a direct comparison between out-of-cloud aerosol particles and IPR in air masses with similar origin was possible, a pronounced enhancement of biological particles was found in the IPR.

scholarly journals Sensitivity studies of different aerosol indirect effects in mixed-phase clouds

2009 ◽  
Vol 9 (22) ◽  
pp. 8917-8934 ◽  
Author(s):  
U. Lohmann ◽  
C. Hoose
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Mixed Phase ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Activation Effect ◽  
Aerosol Effect ◽  
Sensitivity Studies ◽  
Mixed Phase Clouds

Abstract. Aerosols affect the climate system by changing cloud characteristics. Using the global climate model ECHAM5-HAM, we investigate different aerosol effects on mixed-phase clouds: The glaciation effect, which refers to a more frequent glaciation due to anthropogenic aerosols, versus the de-activation effect, which suggests that ice nuclei become less effective because of an anthropogenic sulfate coating. The glaciation effect can partly offset the indirect aerosol effect on warm clouds and thus causes the total anthropogenic aerosol effect to be smaller. It is investigated by varying the parameterization for the Bergeron-Findeisen process and the threshold coating thickness of sulfate (SO4-crit), which is required to convert an externally mixed aerosol particle into an internally mixed particle. Differences in the net radiation at the top-of-the-atmosphere due to anthropogenic aerosols between the different sensitivity studies amount up to 0.5 W m−2. This suggests that the investigated mixed-phase processes have a major effect on the total anthropogenic aerosol effect.

scholarly journals Online single particle analysis of ice particle residuals from mountain-top mixed-phase clouds using laboratory derived particle type assignment

2017 ◽  
Vol 17 (1) ◽  
pp. 575-594 ◽  
Author(s):  
Susan Schmidt ◽  
Johannes Schneider ◽  
Thomas Klimach ◽  
Stephan Mertes ◽  
Ludwig Paul Schenk ◽  
...  
Keyword(s):  
Single Particle ◽  
Aerosol Particles ◽  
Mixed Phase ◽  
Particle Analysis ◽  
Single Particle Analysis ◽  
Laboratory Studies ◽  
Particle Type ◽  
Industrial Emissions ◽  
Anthropogenic Aerosol ◽  
Mixed Phase Clouds

Abstract. In situ single particle analysis of ice particle residuals (IPRs) and out-of-cloud aerosol particles was conducted by means of laser ablation mass spectrometry during the intensive INUIT-JFJ/CLACE campaign at the high alpine research station Jungfraujoch (3580 m a.s.l.) in January–February 2013. During the 4-week campaign more than 70 000 out-of-cloud aerosol particles and 595 IPRs were analyzed covering a particle size diameter range from 100 nm to 3 µm. The IPRs were sampled during 273 h while the station was covered by mixed-phase clouds at ambient temperatures between −27 and −6 °C. The identification of particle types is based on laboratory studies of different types of biological, mineral and anthropogenic aerosol particles. The outcome of these laboratory studies was characteristic marker peaks for each investigated particle type. These marker peaks were applied to the field data. In the sampled IPRs we identified a larger number fraction of primary aerosol particles, like soil dust (13 ± 5 %) and minerals (11 ± 5 %), in comparison to out-of-cloud aerosol particles (2.4 ± 0.4 and 0.4 ± 0.1 %, respectively). Additionally, anthropogenic aerosol particles, such as particles from industrial emissions and lead-containing particles, were found to be more abundant in the IPRs than in the out-of-cloud aerosol. In the out-of-cloud aerosol we identified a large fraction of aged particles (31 ± 5 %), including organic material and secondary inorganics, whereas this particle type was much less abundant (2.7 ± 1.3 %) in the IPRs. In a selected subset of the data where a direct comparison between out-of-cloud aerosol particles and IPRs in air masses with similar origin was possible, a pronounced enhancement of biological particles was found in the IPRs.

scholarly journals A Modeling Case Study of Mixed-Phase Clouds over the Southern Ocean and Tasmania

2010 ◽  
Vol 138 (3) ◽  
pp. 839-862 ◽  
Author(s):  
Anthony E. Morrison ◽  
Steven T. Siems ◽  
Michael J. Manton ◽  
Alex Nazarov
Keyword(s):  
Southern Ocean ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Weather Research And Forecasting ◽  
Marine Stratocumulus ◽  
Cloud Structure ◽  
In Situ Observations ◽  
Cloud Tops ◽  
Mixed Phase Clouds

Abstract The cloud structure associated with two frontal passages over the Southern Ocean and Tasmania is investigated. The first event, during August 2006, is characterized by large quantities of supercooled liquid water and little ice. The second case, during October 2007, is more mixed phase. The Weather Research and Forecasting model (WRFV2.2.1) is evaluated using remote sensed and in situ observations within the post frontal air mass. The Thompson microphysics module is used to describe in-cloud processes, where ice is initiated using the Cooper parameterization at temperatures lower than −8°C or at ice supersaturations greater than 8%. The evaluated cases are then used to numerically investigate the prevalence of supercooled and mixed-phase clouds over Tasmania and the ocean to the west. The simulations produce marine stratocumulus-like clouds with maximum heights of between 3 and 5 km. These are capped by weak temperature and strong moisture inversions. When the inversion is at temperatures warmer than −10°C, WRF produces widespread supercooled cloud fields with little glaciation. This is consistent with the limited in situ observations. When the inversion is at higher altitudes, allowing cooler cloud tops, glaciated (and to a lesser extent mixed phase) clouds are more common. The simulations are further explored to evaluate any orographic signature within the cloud structure over Tasmania. No consistent signature is found between the two cases.

scholarly journals Processes that generate and deplete liquid water and snow in thin midlevel mixed-phase clouds

2009 ◽  
Vol 114 (D12) ◽  
Author(s):  
Adam J. Smith ◽  
Vincent E. Larson ◽  
Jianguo Niu ◽  
J. Adam Kankiewicz ◽  
Lawrence D. Carey
Keyword(s):  
Liquid Water ◽  
Mixed Phase ◽  
Mixed Phase Clouds

Constraining Neoproterozoic subtropical low-level clouds to assess the plausibility of near-Snowball Earth states

2021 ◽  
Author(s):  
Christoph Braun ◽  
Aiko Voigt ◽  
Johannes Hörner ◽  
Joaquim G. Pinto
Keyword(s):  
Sea Ice ◽  
Climate Models ◽  
Global Climate ◽  
Global Climate Models ◽  
Mixed Phase ◽  
Snowball Earth ◽  
Stable Range ◽  
Climate Regime ◽  
Low Level ◽  
Mixed Phase Clouds

&lt;p&gt;Stable waterbelt climate states with close to global ice cover challenge the classical Snowball Earth hypothesis because they provide a robust explanation for the survival of advanced marine species during the Neoproterozoic glaciations (1000 &amp;#8211; 541 Million years ago). Whether Earth&amp;#8217;s climate stabilizes in a waterbelt state or rushes towards a Snowball state is determined by the magnitude of the ice-albedo feedback in the subtropics, where dark, bare sea ice instead of snow-covered sea ice prevails. For a given bare sea-ice albedo, the subtropical ice-albedo feedback and thus the stable range of the waterbelt climate regime is sensitive to the albedo over ice-free ocean, which is largely determined by shortwave cloud-radiative effects (CRE). In the present-day climate, CRE are known to dominate the spread of climate sensitivity across global climate models. We here study the impact of uncertainty associated with CRE on the existence of geologically relevant waterbelt climate regimes using two global climate models and an idealized energy balance model. We find that the stable range of the waterbelt climate regime is very sensitive to the abundance of subtropical low-level mixed-phase clouds. If subtropical cloud cover is low, climate sensitivity becomes so high as to inhibit stable waterbelt states.&lt;/p&gt;&lt;p&gt;The treatment of mixed-phase clouds is highly uncertain in global climate models. Therefore we aim to constrain the uncertainty associated with their CRE by means of a hierarchy of global and regional simulations that span horizontal grid resolutions from 160 km to 300m, and in particular include large eddy simulations of subtropical mixed-phase clouds located over a low-latitude ice edge. In the cold waterbelt climate subtropical CRE arise from convective events caused by strong meridional temperature gradients and stratocumulus decks located in areas of large-scale descending motion. We identify the latter to dominate subtropical CRE and therefore focus our large eddy simulations on subtropical stratocumulus clouds. By conducting simulations with two extreme scenarios for the abundance of atmospheric mineral dust, which serves as ice-nucleating particles and therefore can control mixed-phase cloud physics, we aim to estimate the possible spread of CRE associated with subtropical mixed-phase clouds. From this estimate we may assess whether Neoproterozoic low-level cloud abundance may have been high enough to sustain a stable waterbelt climate regime.&lt;/p&gt;

Understanding the Extratropical Liquid Water Path Feedback in Mixed-Phase Clouds with an Idealized Global Climate Model

2022 ◽  
pp. 1-48
Author(s):  
Yi Ming
Keyword(s):  
Water Content ◽  
Liquid Water ◽  
Climate Model ◽  
Global Climate Model ◽  
Cloud Water ◽  
Mixed Phase ◽  
Liquid Water Path ◽  
Water Path ◽  
Cloud Water Content ◽  
Mixed Phase Clouds

Abstract A negative shortwave cloud feedback associated with higher extratropical liquid water content in mixed-phase clouds is a common feature of global warming simulations, and multiple mechanisms have been hypothesized. A set of process-level experiments performed with an idealized global climate model (a dynamical core with passive water and cloud tracers and full Rotstayn-Klein single-moment microphysics) show that the common picture of the liquid water path (LWP) feedback in mixed-phase clouds being controlled by the amount of ice susceptible to phase change is not robust. Dynamic condensate processes—rather than static phase partitioning—directly change with warming, with varied impacts on liquid and ice amounts. Here, three principal mechanisms are responsible for the LWP response, namely higher adiabatic cloud water content, weaker liquid-to-ice conversion through the Bergeron-Findeisen process, and faster melting of ice and snow to rain. Only melting is accompanied by a substantial loss of ice, while the adiabatic cloud water content increase gives rise to a net increase in ice water path (IWP) such that total cloud water also increases without an accompanying decrease in precipitation efficiency. Perturbed parameter experiments with a wide range of climatological LWP and IWP demonstrate a strong dependence of the LWP feedback on the climatological LWP and independence from the climatological IWP and supercooled liquid fraction. This idealized setup allows for a clean isolation of mechanisms and paints a more nuanced picture of the extratropical mixed-phase cloud water feedback than simple phase change.

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