Characteristics of the severe March 2021 Gobi Desert dust storm and its impact on air pollution in China

Chemosphere ◽  
2021 ◽  
pp. 132219
Author(s):  
Mikalai Filonchyk
2018 ◽  
Vol 18 (19) ◽  
pp. 14609-14622 ◽  
Author(s):  
Zechen Yu ◽  
Myoseon Jang

Abstract. To improve the simulation of the heterogeneous oxidation of SO2 and NOx in the presence of authentic mineral dust particles under ambient environmental conditions, the explicit kinetic mechanisms were constructed in the Atmospheric Mineral Aerosol Reaction (AMAR) model. The formation of sulfate and nitrate was divided into three phases: the gas phase, the non-dust aqueous phase, and the dust phase. In particular, AMAR established the mechanistic role of dust chemical characteristics (e.g., photoactivation, hygroscopicity, and buffering capacity) in heterogeneous chemistry. The photoactivation kinetic process of different dust particles was built into the model by measuring the photodegradation rate constant of an impregnated surrogate (malachite green dye) on a dust filter sample (e.g., Arizona test dust – ATD – and Gobi Desert dust – GDD) using an online reflective UV–visible spectrometer. The photoactivation parameters were integrated with the heterogeneous chemistry to predict the formation of reactive oxygen species on dust surfaces. A mathematical equation for the hygroscopicity of dust particles was also included in the AMAR model to process the multiphase partitioning of trace gases and in-particle chemistry. The buffering capacity of dust, which is related to the neutralization of dust alkaline carbonates with inorganic acids, was included in the model to dynamically predict the hygroscopicity of aged dust. The AMAR model simulated the formation of sulfate and nitrate using experimental data obtained in the presence of authentic mineral dust under ambient sunlight using a large outdoor smog chamber (University of Florida Atmospheric Photochemical Outdoor Reactor, UF-APHOR). Overall, the influence of GDD on the heterogeneous chemistry was much greater than that of ATD. Based on the model analysis, GDD enhanced the sulfate formation mainly via its high photoactivation capability. In the case of NO2 oxidation, dust-phase nitrate formation is mainly regulated by the buffering capacity of dust. The measured buffering capacity of GDD was 2 times greater than that of ATD, and consequently, the maximum nitrate concentration with GDD was nearly 2 times higher than that with ATD. The model also highlights that in urban areas with high NOx concentrations, hygroscopic nitrate salts quickly form via titration of the carbonates in the dust particles, but in the presence of SO2, the nitrate salts are gradually depleted by the formation of sulfate.


2006 ◽  
Author(s):  
O. A. Bukin ◽  
A. N. Pavlov ◽  
J. N. Kulchin ◽  
K. A. Shmirko ◽  
P. A. Salyuk ◽  
...  

2011 ◽  
Vol 38 (21) ◽  
pp. n/a-n/a ◽  
Author(s):  
Daniel Rosenfeld ◽  
Xing Yu ◽  
Guihua Liu ◽  
Xiaohong Xu ◽  
Yannian Zhu ◽  
...  

2011 ◽  
Vol 11 (20) ◽  
pp. 10637-10648 ◽  
Author(s):  
H. S. Marey ◽  
J. C. Gille ◽  
H. M. El-Askary ◽  
E. A. Shalaby ◽  
M. E. El-Raey

Abstract. Since 1999 Cairo and the Nile delta region have suffered from air pollution episodes called the "black cloud" during the fall season. These have been attributed to either burning of agriculture waste or long-range transport of desert dust. Here we present a detailed analysis of the optical and microphysical aerosol properties, based on satellite data. Monthly mean values of Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth (AOD) at 550 nm were examined for the 10 yr period from 2000–2009. Significant monthly variability is observed in the AOD with maxima in April or May (~0.5) and October (~0.45), and a minimum in December and January (~0.2). Monthly mean values of UV Aerosol Index (UVAI) retrieved by the Ozone Monitoring Instrument (OMI) for 4 yr (2005–2008) exhibit the same AOD pattern. The carbonaceous aerosols during the black cloud periods are confined to the planetary boundary layer (PBL), while dust aerosols exist over a wider range of altitudes, as shown by Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) aerosol profiles. The monthly climatology of Multi-angle Imaging SpectroRadiometer (MISR) data show that the aerosols during the black cloud periods are spherical with a higher percentage of small and medium size particles, whereas the spring aerosols are mostly large non-spherical particles. All of the results show that the air quality in Cairo and the Nile delta region is subject to a complex mixture of air pollution types, especially in the fall season, when biomass burning contributes to a background of urban pollution and desert dust.


Weatherwise ◽  
1959 ◽  
Vol 12 (3) ◽  
pp. 115-116 ◽  
Author(s):  
Harry L. Elser
Keyword(s):  
El Paso ◽  

2018 ◽  
Vol 18 (11) ◽  
pp. 8353-8371 ◽  
Author(s):  
Xiao-Xiao Zhang ◽  
Brenton Sharratt ◽  
Lian-You Liu ◽  
Zi-Fa Wang ◽  
Xiao-Le Pan ◽  
...  

Abstract. A severe dust storm event originated from the Gobi Desert in Central and East Asia during 2–7 May 2017. Based on Moderate Resolution Imaging Spectroradiometer (MODIS) satellite products, hourly environmental monitoring measurements from Chinese cities and East Asian meteorological observation stations, and numerical simulations, we analysed the spatial and temporal characteristics of this dust event as well as its associated impact on the Asia-Pacific region. The maximum observed hourly PM10 (particulate matter with an aerodynamic diameter ≤ 10 µm) concentration was above 1000 µg m−3 in Beijing, Tianjin, Shijiazhuang, Baoding, and Langfang and above 2000 µg m−3 in Erdos, Hohhot, Baotou, and Alxa in northern China. This dust event affected over 8.35 million km2, or 87 % of the Chinese mainland, and significantly deteriorated air quality in 316 cities of the 367 cities examined across China. The maximum surface wind speed during the dust storm was 23–24 m s−1 in the Mongolian Gobi Desert and 20–22 m s−1 in central Inner Mongolia, indicating the potential source regions of this dust event. Lidar-derived vertical dust profiles in Beijing, Seoul, and Tokyo indicated dust aerosols were uplifted to an altitude of 1.5–3.5 km, whereas simulations by the Weather Research and Forecasting with Chemistry (WRF-Chem) model indicated 20.4 and 5.3 Tg of aeolian dust being deposited respectively across continental Asia and the North Pacific Ocean. According to forward trajectory analysis by the FLEXible PARTicle dispersion (FLEXPART) model, the East Asian dust plume moved across the North Pacific within a week. Dust concentrations decreased from the East Asian continent across the Pacific Ocean from a magnitude of 103 to 10−5 µg m−3, while dust deposition intensity ranged from 104 to 10−1 mg m−2. This dust event was unusual due to its impact on continental China, the Korean Peninsula, Japan, and the North Pacific Ocean. Asian dust storms such as those observed in early May 2017 may lead to wider climate forcing on a global scale.


2018 ◽  
Author(s):  
Xiao-Xiao Zhang ◽  
Brenton Sharratt ◽  
Lian-You Liu ◽  
Zi-Fa Wang ◽  
Xiao-Le Pan ◽  
...  

Abstract. A severe dust storm event originated from the Gobi Desert in Central and East Asia during 2–7 May, 2017. Based on moderate resolution imaging spectroradiometer (MODIS) satellite products, hourly environmental monitoring measurements from 367 Chinese cities and more than 2000 East Asian meteorological observation stations, and numerical simulations, we analysed the spatial and temporal characteristics of this dust event as well as its associated impact on the Asia-Pacific region. The maximum observed hourly PM10 (particulate matter with an aerodynamic diameter ≤ 10 μm) concentration was above 1000 μg m−3 in Beijing, Tianjin, Shijiazhuang, Baoding, and Langfang and above 2000 μg m−3 in Erdos, Hohhot, Baotou, and Alxa in northern China. This dust event affected over 8.35 million km2, or 87 % of mainland China, and significantly deteriorated air quality in 316 cities of the 367 cities examined across China. The maximum surface wind speed during the dust storm was 23–24 m s−1 in the Mongolian Gobi Desert and 20–22 m s−1 in central Inner Mongolia, indicating the potential source regions of this dust event. Lidar-derived vertical dust profiles in Beijing, Seoul, and Tokyo indicated dust aerosols were uplifted to an altitude of 1.5–3.5 km whereas simulations by the Weather Research and Forecasting with Chemistry (WRF-Chem) model indicated 20.4 Tg and 5.3 Tg of aeolian dust being deposited respectively across continental Asia and the North Pacific Ocean. According to forward trajectory analysis by the FLEXible PARTicle dispersion (FLEXPART) model, the East Asian dust plume moved across the North Pacific within a week. Dust concentrations decreased from East Asian continent across the Pacific Ocean from a magnitude of 103 to 10−5 μg m−3, while dust deposition intensity ranged from 104 to 10−1 mg m−2. This dust event was unusual due to its impact on continental China, Korea, Japan and North Pacific Ocean. Asian dust storms such as observed in early May 2017 may lead to wider climate forcing on a global scale.


Author(s):  
Jugder D

A meteorological and dust monitoring tower with 20 m height set up at a Nomgon site in Umnugobi Aimag in the Mongolian Gobi in 2010. The Nomgon monitoring tower equipped with wind speed sensors at 2, 4, 10 and 20 m height above the ground level (AGL), a wind direction sensor at 10 m height, a sonic anemometer to measure turbulent momentum flux at 8 m height and a soil moisture sensor at 5 cm depth. We had a purpose to measure dust concentration of PM10 at two levels using Dust-Trak instruments during an intensive observation period (IOP) of a dust event in spring. A dust storm was expected in the Mongolian Gobi from 30 April to 1 May 2016 and two Dust-Traks were set at 0.9 and 2.95 m heights in the tower during this IOP for measuring PM10. Wind data at 2 and 10 m height, three wind components at 8 m height by a sonic anemometer, soil moisture (volumetric water content) data in 5 cm depth and dust concentrations of PM10 at two levels are used in this study. These data from the sensors and instruments in the tower were used for estimation friction velocity and vertical dust flux at the Nomgon site. In association with a surface cyclone, its frontal system and a trough aloft, the expected dust storm occurred in the Mongolian Gobi during the IOP period. Dust concentrations of PM10 increased during the dust storm period due to raised wind speed in the dry conditions of air and soil. The present study aimed to estimate friction velocity (u*) and vertical dust flux (F) around Nomgon site in the Mongolian Gobi desert during the dust storm period. The estimation results were presented in this paper.


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