The effect of preheating temperature on PAH/soot formation in methane/air co-flow flames at elevated pressure

Fuel ◽  
2021 ◽  
pp. 122656
Author(s):  
Peng Liu ◽  
JunJun Guo ◽  
Erica Quadarella ◽  
Anthony Bennett ◽  
Sreenivasa R. Gubba ◽  
...  
2021 ◽  
Author(s):  
Mingshan Sun ◽  
Zhiwen Gan

Abstract The hydrogen addition is a potential way to reduce the soot emission of aviation kerosene. The current study analyzed the effect of hydrogen addition on aviation kerosene (Jet A1) soot formation in a laminar flame at elevated pressure to obtain a fundamental understanding of the reduced soot formation by hydrogen addition. The soot formation of flame was simulated by CoFlame code. The soot formation of kerosene-nitrogen-air, (kerosene + replaced hydrogen addition)-nitrogen-air, (kerosene + direct hydrogen addition)-nitrogen-air and (kerosene + direct nitrogen addition)-nitrogen-air laminar flames were simulated. The calculated pressure includes 1, 2 and 5 atm. The hydrogen addition increases the peak temperature of Jet A1 flame and extends the height of flame. The hydrogen addition suppresses the soot precursor formation of Jet A1 by physical dilution effect and chemical inhibition effect, which weaken the poly-aromatic hydrocarbon (PAH) condensation process and reduce the soot formation. The elevated pressure significantly accelerates the soot precursor formation and increases the soot formation in flame. Meanwhile, the ratio of reduced soot volume fraction to base soot volume fraction by hydrogen addition decreases with the increase of pressure, indicating that the elevated pressure weakens the suppression effect of hydrogen addition on soot formation in Jet A1 flame.


2011 ◽  
Vol 110-116 ◽  
pp. 18-22 ◽  
Author(s):  
A. Yunardi ◽  
B. Elwina ◽  
Sylvia Novi ◽  
D. Wusnah ◽  
Bindar Yazid

This paper presents results obtained from the application of a computational fluid dynamics (CFD) code Fluent 6.3 to modeling of elevated pressure methane non-premixed sooting flames. The study focuses on comparing the two soot models available in the code for the prediction of the soot level in the flames. A standard k-ε model and Eddy Dissipation model are utilized for the representation of flow field and combustion of the flame being investigated. For performance comparison study, a single step soot model of Khan and Greeves and two-step soot model proposed by Tesner are tested. The results of calculations are compared with experimental data of methane sooting flame taken from literature. The results of the study show that a combination of the standard k-ε turbulence model and eddy dissipation model is capable of producing reasonable predictions of temperature both in axial and radial profiles; although further downstream of the flame over-predicted temperature is evidence. With regard to soot model performance study, it shows that the two-step model clearly performed far better than the single-step model in predicting the soot level in ethylene flame at both axial and radial profiles. With a modification in the constant α of the soot formation equation, the two-step model was capable of producing prediction of soot level closer to experimental data. In contrast, the single-step soot model produced very poor results, leading to a significant under-prediction of soot levels in both flames. Although the Tesner’s soot model is simpler than the current available models, this model is still capable of providing reasonable agreement with experimental data, allowing its application for the purpose of design and operation of an industrial combustion system.


1991 ◽  
Vol 23 (1) ◽  
pp. 1581-1587 ◽  
Author(s):  
M. Bönig ◽  
ChR. Feldermann ◽  
H. Jander ◽  
B. Lüers ◽  
G. Rudolph ◽  
...  

1989 ◽  
Vol 22 (1) ◽  
pp. 413-423 ◽  
Author(s):  
J.B. Moss ◽  
C.D. Stewart ◽  
K.J. Syed

Author(s):  
Klaus Peter Geigle ◽  
Redjem Hadef ◽  
Wolfgang Meier

Swirl-stabilized, nonpremixed ethylene/air flames were investigated at pressures up to 5 bar to study the effect of different operating parameters on soot formation and oxidation. Focus of the experiments was the establishment of a database describing well-defined flames, serving for validation of numerical simulation. Good optical access via pressure chamber windows and combustion chamber windows enables application of laser-induced incandescence to derive soot volume fractions after suitable calibration. This results in ensemble averaged, as well as instantaneous soot distributions. Beyond pressure, parameters under study were the equivalence ratio, thermal power, and amount of oxidation air. The latter could be injected radially into the combustor downstream of the main reaction zone through holes in the combustion chamber posts. Combustion air was introduced through a dual swirl injector whose two flow rates were controlled separately. The split of those air flows provided an additional parameter variation. Nominal power of the operating points was approximately 10 kW/bar leading to a maximum power of roughly 50 kW, not including oxidation air.


Author(s):  
Klaus Peter Geigle ◽  
Redjem Hadef ◽  
Wolfgang Meier

Swirl-stabilized, non-premixed ethylene/air flames were investigated at pressures up to 5 bars to study the effect of different operating parameters on soot formation and oxidation. Focus of the experiments was the establishment of a data base describing well defined flames, serving for validation of numerical simulation. Good optical access via pressure chamber windows and combustion chamber windows enables application of laser-induced incandescence to derive soot volume fractions after suitable calibration. This results in ensemble averaged as well as instantaneous soot distributions. Beyond pressure, parameters under study were the equivalence ratio, thermal power and amount of oxidation air. Latter could be injected radially into the combustor downstream of the main reaction zone through holes in the combustion chamber posts. Combustion air was introduced through a dual swirl injector whose two flow rates were controlled separately. The split of those air flows provided an additional parameter variation. Nominal power of the operating points was approximately 10 kW/bar leading to a maximum power of roughly 50 kW, not including oxidation air.


Author(s):  
Christoph Hassa ◽  
Ulrich Meier ◽  
Johannes Heinze ◽  
Eggert Magens ◽  
Michael Schroll ◽  
...  

Two RR Lean Direct Injection (LDI) injector versions with different amounts of pilot swirl were investigated. Experiments, performed at elevated pressure and temperature, corresponding to engine conditions at idle include Mie scattering. LII and absorption measurements are used for soot concentration within the primary zone. The soot emission at the outlet is measured by an SMPS instrument. These experimental studies are complemented with PIV measurements. The acquired data allows evaluation of the combustion process from the liquid phase, followed by evaporation, reaction and finally soot production with high spatial resolution. The change of swirl produced rather moderate changes in the flow field, nevertheless qualitative changes in the fuel placement were observed. Starting from there, differences in heat release and soot formation can be explained, which lead to larger changes of soot emission. These observations show that a good knowledge of the interaction of gas and liquid phase is necessary to predict the occurrence of behavioral changes in the operating regime.


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