In situ oxidation of ultrathin Ti3C2Tx MXene modified with crystalline g-C3N4 nanosheets for photocatalytic H2 evolution

Author(s):  
Jingjun Liu ◽  
Haiping Zhou ◽  
Jiajie Fan ◽  
Quanjun Xiang
2018 ◽  
Vol 532 ◽  
pp. 272-279 ◽  
Author(s):  
Ping Wang ◽  
Xiaoqing Yi ◽  
Yanggang Lu ◽  
Huogen Yu ◽  
Jiaguo Yu

2021 ◽  
Author(s):  
Xue Bai ◽  
Bo Liu ◽  
Wei Zhang ◽  
Yang Wang ◽  
Yu Yu ◽  
...  

A porous Cu2O/TiO2 hybrid photocatalyst with n-type Cu2O decorated on the mesoporous TiO2 derived from MIL-125 was designed through the in situ Cu2+ ions reduction strategy. Under UV-vis light irradiation,...


2019 ◽  
Vol 12 (1) ◽  
Author(s):  
Yujie Li ◽  
Lei Ding ◽  
Shujun Yin ◽  
Zhangqian Liang ◽  
Yanjun Xue ◽  
...  

AbstractThe biggest challenging issue in photocatalysis is efficient separation of the photoinduced carriers and the aggregation of photoexcited electrons on photocatalyst’s surface. In this paper, we report that double metallic co-catalysts Ti3C2 MXene and metallic octahedral (1T) phase tungsten disulfide (WS2) act pathways transferring photoexcited electrons in assisting the photocatalytic H2 evolution. TiO2 nanosheets were in situ grown on highly conductive Ti3C2 MXenes and 1T-WS2 nanoparticles were then uniformly distributed on TiO2@Ti3C2 composite. Thus, a distinctive 1T-WS2@TiO2@Ti3C2 composite with double metallic co-catalysts was achieved, and the content of 1T phase reaches 73%. The photocatalytic H2 evolution performance of 1T-WS2@TiO2@Ti3C2 composite with an optimized 15 wt% WS2 ratio is nearly 50 times higher than that of TiO2 nanosheets because of conductive Ti3C2 MXene and 1T-WS2 resulting in the increase of electron transfer efficiency. Besides, the 1T-WS2 on the surface of TiO2@Ti3C2 composite enhances the Brunauer–Emmett–Teller surface area and boosts the density of active site.


2020 ◽  
Vol 10 (7) ◽  
pp. 2221-2230 ◽  
Author(s):  
Chenyang Li ◽  
Mian Fu ◽  
Yan Wang ◽  
Enzhou Liu ◽  
Jun Fan ◽  
...  

The Co2P as co-catalyst was firstly loaded on the 2D microporous structure RP surface by in situ hydrothermal method.


2015 ◽  
Vol 44 (40) ◽  
pp. 17859-17866 ◽  
Author(s):  
Xiao-jing Wang ◽  
Xiao Tian ◽  
Fa-tang Li ◽  
Jun Zhao ◽  
Yu-pei Li ◽  
...  

A Ti species modified g-C3N4 photocatalyst was synthesized via an in situ hydrothermal route and the subsequent low-temperature calcination.


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