scholarly journals Unveiling the Coupling of Single Metallic Nanoparticles to Whispering-Gallery Microcavities

Nano Letters ◽  
2021 ◽  
Author(s):  
Yves Auad ◽  
Cyrille Hamon ◽  
Marcel Tencé ◽  
Hugo Lourenço-Martins ◽  
Vahagn Mkhitaryan ◽  
...  
Author(s):  
Maurizio Manzo ◽  
Ryan Schwend

Whispering gallery mode (WGM) resonators exhibit high quality factor Q and a small mode volume; they usually exhibit high resolution when used as sensors. The light trapped inside a polymeric micro-cavity travels through total internal reflection generating the whispering gallery modes (WGMs). A laser or a lamp is used to power the microlaser by using a laser dye embedded within the resonator. The excited fluorescence of the dye couples with the optical modes. The optical modes (laser modes) are seen as sharp peaks in the emission spectrum with the aid of an optical interferometer. The position of these optical modes is sensitive to any change in the morphology of the resonator. However, the laser threshold of these microlasers is of few hundreds of microjoules per square centimeter (fluence) usually. In addition, the excitation wavelength’s light powering the device must be smaller than the microlasers size. When metallic nanoparticles are added to the microlaser, the excited surface plasmon couples with the emission spectrum of the laser dye. Therefore, the fluorescence of the dye can be enhanced by this coupling; this in turn, lowers the power threshold of the microlaser. Also, due to a plasmonic effect, it is possible to use smaller microlasers. In addition, a new sensing modality is enabled based on the variation of the optical modes’ amplitude with the change in the morphology’s microlaser. This opens a new avenue of low power consumption microlasers and photonics multiplexed biosensors.


Author(s):  
Maurizio Manzo ◽  
Ryan Schwend

Whispering gallery mode (WGM) resonators exhibit a high quality factor Q and a small mode volume; they usually exhibit high resolution when used as sensors. The light trapped inside a polymeric microcavity travels through total internal reflection generating the WGMs. A laser or a lamp is used to power the microlaser by using a laser dye embedded within the resonator. The excited fluorescence of the dye couples with the optical modes. The optical modes (laser modes) are seen as sharp peaks in the emission spectrum with the aid of an optical interferometer. The position of these optical modes is sensitive to any change in the morphology of the resonator. However, the laser threshold of these microlasers is of few hundreds of microjoules per square centimeter (fluence) usually. In addition, the excitation wavelength's light powering the device must be smaller than the microlasers size. When metallic nanoparticles are added to the microlaser, the excited surface plasmon couples with the emission spectrum of the laser dye. Therefore, the fluorescence of the dye can be enhanced by this coupling; this in turn, lowers the power threshold of the microlaser. Also, due to a plasmonic effect, it is possible to use smaller microlasers. In addition, a new sensing modality is enabled based on the variation of the optical modes' amplitude with the change in the morphology's microlaser. This opens a new avenue of low power consumption microlasers and photonics multiplexed biosensors.


2007 ◽  
Vol 32 (2-3) ◽  
pp. 123-126
Author(s):  
Y.-R. Nowicki-Bringuier ◽  
J. Claudon ◽  
C. Böckler ◽  
S. Reitzenstein ◽  
M. Kamp ◽  
...  

2020 ◽  
Vol 92 (2) ◽  
pp. 20101
Author(s):  
Behnam Kheyraddini Mousavi ◽  
Morteza Rezaei Talarposhti ◽  
Farshid Karbassian ◽  
Arash Kheyraddini Mousavi

Metal-assisted chemical etching (MACE) is applied for fabrication of silicon nanowires (SiNWs). We have shown the effect of amorphous sheath of SiNWs by treating the nanowires with SF6 and the resulting reduction of absorption bandwidth, i.e. making SiNWs semi-transparent in near-infrared (IR). For the first time, by treating the fabricated SiNWs with copper containing HF∕H2O2∕H2O solution, we have generated crystalline nanowires with broader light absorption spectrum, up to λ = 1 μm. Both the absorption and photo-luminescence (PL) of the SiNWs are observed from visible to IR wavelengths. It is found that the SiNWs have PL at visible and near Infrared wavelengths, which may infer presence of mechanisms such as forbidden gap transitions other can involvement of plasmonic resonances. Non-radiative recombination of excitons is one of the reasons behind absorption of SiNWs. Also, on the dielectric metal interface, the absorption mechanism can be due to plasmonic dissipation or plasmon-assisted generation of excitons in the indirect band-gap material. Comparison between nanowires with and without metallic nanoparticles has revealed the effect of nanoparticles on absorption enhancement. The broader near IR absorption, paves the way for applications like hyperthermia of cancer while the optical transition in near IR also facilitates harvesting electromagnetic energy at a broad spectrum from visible to IR.


1990 ◽  
Vol 160 (1) ◽  
pp. 157 ◽  
Author(s):  
Vladimir B. Braginskii ◽  
V.S. Il'chenko ◽  
M.L. Gorodetskii

2009 ◽  
Vol E92-C (12) ◽  
pp. 1504-1511 ◽  
Author(s):  
Thi Huong TRAN ◽  
Yuanfeng SHE ◽  
Jiro HIROKAWA ◽  
Kimio SAKURAI ◽  
Yoshinori KOGAMI ◽  
...  

2017 ◽  
Vol 13 (2) ◽  
pp. 4671-4677 ◽  
Author(s):  
A. M. Abdelghany ◽  
A.H. Oraby ◽  
Awatif A Hindi ◽  
Doaa M El-Nagar ◽  
Fathia S Alhakami

Bimetallic nanoparticles of silver (Ag) and gold (Au) were synthesized at room temperature using Curcumin. Reduction process of silver and gold ions with different molar ratios leads to production of different nanostructures including alloys and core-shells. Produced nanoparticles were characterized simultaneously with FTIR, UV/vis. spectroscopy, transmission electron microscopy (TEM), and Energy-dispersive X-ray (EDAX). UV/vis. optical absorption spectra of as synthesized nanoparticles reveals presence of surface palsmon resonance (SPR) of both silver at (425 nm) and gold at (540 nm) with small shift and broadness of gold band after mixing with resucing and capping agent in natural extract which suggest presence of bimetallic nano structure (Au/Ag). FTIR and EDAX data approve the presence of bimetallic nano structure combined with curcumin extract. TEM micrographs shows that silver and gold can be synthesized separately in the form of nano particles using curcumin extract. Synthesis of gold nano particles in presence of silver effectively enhance and control formation of bi-metallic structure.


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