scholarly journals Methane Generation from Anthracite by Fungi and Methanogen Mixed Flora Enriched from Produced Water Associated with the Qinshui Basin in China

ACS Omega ◽  
2021 ◽  
Author(s):  
Qing Han ◽  
Hongguang Guo ◽  
Jinlong Zhang ◽  
Zaixing Huang ◽  
Michael Allan Urynowicz ◽  
...  
Keyword(s):  
Produced Water ◽  
Methane Generation ◽  
Qinshui Basin

scholarly journals Biogeochemistry and the associated redox signature of co-produced water from coalbed methane wells in the Shizhuangnan block in the southern Qinshui Basin, China

2020 ◽  
Vol 38 (4) ◽  
pp. 1034-1053
Author(s):  
Yang Li ◽  
Shuheng Tang ◽  
Songhang Zhang ◽  
Zhaodong Xi ◽  
Pengfei Wang
Keyword(s):  
Coalbed Methane ◽  
Produced Water ◽  
Dissolved Inorganic Carbon ◽  
Gas Production ◽  
Redox Conditions ◽  
Effective Parameters ◽  
Production Rates ◽  
Qinshui Basin ◽  
Southern Qinshui Basin ◽  
Biogeochemical Parameters

To meet the global energy demands, the exploitation of coalbed methane has received increasing attention. Biogeochemical parameters of co-produced water from coalbed methane wells were performed in the No. 3 coal seam in the Shizhuangnan block of the southern Qinshui Basin (China). These biogeochemical parameters were firstly utilized to assess coal reservoir environments and corresponding coalbed methane production. A high level of Na+ and HCO3– and deuterium drift were found to be accompanied by high gas production rates, but these parameters are unreliable to some extent. Dissolved inorganic carbon (DIC) isotopes δ13CDIC from water can be used to distinguish the environmental redox conditions. Positive δ13CDIC values within a reasonable range suggest reductive conditions suitable for methanogen metabolism and were accompanied by high gas production rates. SO42–, NO3– and related isotopes affected by various bacteria corresponding to various redox conditions are considered effective parameters to identify redox states and gas production rates. Importantly, the combination of δ13CDIC and SO42– can be used to evaluate gas production rates and predict potentially beneficial areas. The wells with moderate δ13CDIC and negligible SO42– represent appropriate reductive conditions, as observed in most high and intermediate production wells. Furthermore, the wells with highest δ13CDIC and negligible SO42– exhibit low production rates, as the most reductive environments were too strict to extend pressure drop funnels.

scholarly journals Biogeochemistry and Water–Rock Interactions of Coalbed Methane Co-Produced Water in the Shizhuangnan Block of the Southern Qinshui Basin, China

Water ◽  
2019 ◽  
Vol 12 (1) ◽  
pp. 130
Author(s):  
Yang Li ◽  
Shuheng Tang ◽  
Songhang Zhang ◽  
Zhaodong Xi ◽  
Pengfei Wang
Keyword(s):  
16S Rrna ◽  
Water Samples ◽  
Coalbed Methane ◽  
Produced Water ◽  
Major Ions ◽  
16S Rrna Sequencing ◽  
Qinshui Basin ◽  
Isotopic Compositions ◽  
Rrna Sequencing ◽  
Southern Qinshui Basin

Coalbed methane is a major unconventional resource that has been exploited commercially for decades in the southern Qinshui Basin of China. The hydrogeochemical characteristics of coal reservoir water play a key role in the exploration and development of coalbed methane resources. In view of this, a detailed study was performed on coalbed methane co-produced water collected from the Shizhuangnan block to assess water–rock interactions and biogeochemical processes. Water samples were analyzed to establish major ions, isotopic compositions and perform 16S rRNA sequencing. Results suggest that the hydrochemistry was controlled by water–rock processes and that methane was consumed by sulfate reduction through calculation. Meanwhile, the isotopic compositions of water samples indicated that they had a predominantly meteoric origin and were influenced by microbial activity. The 16S rRNA sequencing results of bacteria and archaea provide an important foundation for understanding the activity of sulfate-reducing bacteria and methanogens at different hydraulic heads, which was consistent with isotopic analysis. Carbonates containing calcite and dolomite were found to be distributed at different hydraulic head due to the biogeochemical characteristics and associated water–rock interactions.

scholarly journals Fluorescence Characteristics of Coalbed Methane Produced Water and Its Influence on Freshwater Bacteria in the South Qinshui Basin, China

2021 ◽  
Vol 18 (24) ◽  
pp. 12921
Author(s):  
Tao Jin ◽  
Qingjun Meng ◽  
Xiangdong Li ◽  
Lai Zhou
Keyword(s):  
Coalbed Methane ◽  
Produced Water ◽  
Quality Analysis ◽  
Chemical Production ◽  
Qinshui Basin ◽  
Factor Method ◽  
Freshwater Bacteria ◽  
Fluorescence Characteristics ◽  
Parallel Factor ◽  
Method Analysis

Production of coalbed methane (CBM) resources commonly requires using hydraulic fracturing and chemical production well additives. Concern exists for the existence of chemical compounds in CBM produced water, due to the risk of environmental receptor contamination. In this study, parallel factor method analysis (PARAFAC), fluorescence index, and the fluorescence area integral methods were used to analyse the properties of CBM produced water sampled from Shizhuang Block (one of the most active CBM-producing regions in the Qinshui Basin). A culture experiment was designed to determine the effect of discharged CBM produced water on microorganisms in freshwater. Water quality analysis shows the hydrochemistry of most water samples as Na-HCO3 type produced water of CBM appears as a generally weak alkaline (pH 8.69 ± 0.185) with high salinity, high alkalinity, and a high chemical oxygen demand (COD) value. Three individual components were identified by using parallel factor method analysis as humic-like components (C1), fulvic-like components (C2), and amino acid-like substances (C3). The fluorescence characteristic index comprehensively explains that the fluorescent substances in CBM produced water has the characteristics of a low degree of humification and a high recent self-generating source. The region integration results of characteristic peaks show that tyrosine-like and tryptophan-like materials account for more than 67% of fluorescent substances in CBM produced water. The addition of produced water from coalbed methane promotes the growth of freshwater bacteria, and this process is accompanied by the decrease of the proportion of fulvic acid, humic acid, and the increase of the proportion of soluble microbial metabolites. This paper proposes a convenient method for organic matter identification of CBM produced water and provides some theoretical support and reference for the improvement of CBM water treatment and utilization.

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