scholarly journals Empirical age spectra for the midlatitude lower stratosphere from in situ observations of CO2: Quantitative evidence for a subtropical “barrier” to horizontal transport

2001 ◽  
Vol 106 (D10) ◽  
pp. 10257-10274 ◽  
Author(s):  
A. E. Andrews ◽  
K. A. Boering ◽  
S. C. Wofsy ◽  
B. C. Daube ◽  
D. B. Jones ◽  
...  
2016 ◽  
Vol 16 (18) ◽  
pp. 12273-12286 ◽  
Author(s):  
Sergey M. Khaykin ◽  
Jean-Pierre Pommereau ◽  
Emmanuel D. Riviere ◽  
Gerhard Held ◽  
Felix Ploeger ◽  
...  

Abstract. High-resolution in situ balloon measurements of water vapour, aerosol, methane and temperature in the upper tropical tropopause layer (TTL) and lower stratosphere are used to evaluate the processes affecting the stratospheric water budget: horizontal transport (in-mixing) and hydration by cross-tropopause overshooting updrafts. The obtained in situ evidence of these phenomena are analysed using satellite observations by Aura MLS (Microwave Limb Sounder) and CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) together with trajectory and transport modelling performed using CLaMS (Chemical Lagrangian Model of the Stratosphere) and HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) model. Balloon soundings were conducted during March 2012 in Bauru, Brazil (22.3° S) in the frame of the TRO-Pico campaign for studying the impact of convective overshooting on the stratospheric water budget. The balloon payloads included two stratospheric hygrometers: FLASH-B (Fluorescence Lyman-Alpha Stratospheric Hygrometer for Balloon) and Pico-SDLA instrument as well as COBALD (Compact Optical Backscatter Aerosol Detector) sondes, complemented by Vaisala RS92 radiosondes. Water vapour vertical profiles obtained independently by the two stratospheric hygrometers are in excellent agreement, ensuring credibility of the vertical structures observed. A signature of in-mixing is inferred from a series of vertical profiles, showing coincident enhancements in water vapour (of up to 0.5 ppmv) and aerosol at the 425 K (18.5 km) level. Trajectory analysis unambiguously links these features to intrusions from the Southern Hemisphere extratropical stratosphere, containing more water and aerosol, as demonstrated by MLS and CALIPSO global observations. The in-mixing is successfully reproduced by CLaMS simulations, showing a relatively moist filament extending to 20° S. A signature of local cross-tropopause transport of water is observed in a particular sounding, performed on a convective day and revealing water vapour enhancements of up to 0.6 ppmv as high as the 404 K (17.8 km) level. These are shown to originate from convective overshoots upwind detected by an S-band weather radar operating locally in Bauru. The accurate in situ observations uncover two independent moisture pathways into the tropical lower stratosphere, which are hardly detectable by space-borne sounders. We argue that the moistening by horizontal transport is limited by the weak meridional gradients of water, whereas the fast convective cross-tropopause transport, largely missed by global models, can have a substantial effect, at least at a regional scale.


Author(s):  
Sergey M. Khaykin ◽  
Jean-Pierre Pommereau ◽  
Emmanuel D. Riviere ◽  
Gerhard Held ◽  
Felix Ploeger ◽  
...  

High-resolution in situ balloon measurements of water vapour, aerosol, methane and temperature in the upper Tropical Tropopause Layer (TTL) and lower stratosphere are used to evaluate the processes controlling the stratospheric water budget: horizontal transport (inmixing) and hydration by cross-tropopause overshooting updrafts. The obtained in situ evidences of these phenomena are analyzed using satellite observations by Aura MLS (Microwave Limb Sounder) and CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) together with trajectory and transport modeling performed using CLaMS (Chemical Lagrangian Model of the Stratosphere) and HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model. <br><br> Balloon soundings were conducted during March 2012 in Bauru, Brazil (22.3°&thinsp;S) in the frame of the TRO-Pico campaign for studying the impact of convective overshooting on the stratospheric water budget. The balloon payloads included two stratospheric hygrometers: FLASH-B (Fluorescence Lyman-Alpha Stratospheric Hygrometer for Balloon) and Pico-SDLA instrument as well as COBALD (Compact Optical Backscatter Aerosol Detector) sondes, complemented by Vaisala RS-92 radiosondes. Water vapour vertical profiles obtained independently by the two stratospheric hygrometers are in excellent agreement, ensuring credibility of the vertical structures observed. <br><br> A signature of in-mixing is inferred from a series of vertical profiles, showing coincident enhancements in water vapour and aerosol at the 425&thinsp;K (18.5&thinsp;km) level. Trajectory analysis unambiguously links these features to intrusions from the Southern Hemisphere extra-tropical stratosphere, containing more water and aerosol, as demonstrated by MLS and CALIPSO global observations. The in-mixing is successfully reproduced by CLaMS simulations, showing a relatively moist filament extending to 20&thinsp;S°. A signature of local cross-tropopause transport of water is observed in a particular sounding, performed on a convective day and revealing water vapour enhancements of up to 0.6&thinsp;ppmv as high as the 404&thinsp;K (17.8&thinsp;km) level. These are shown to originate from convective overshoots upwind detected by an S-band weather radar operating locally in Bauru. <br><br> The accurate in situ observations uncover two independent moisture pathways into the tropical lower stratosphere, whose manifestations are hardly detectable by space-borne sounders. We argue that the moistening by horizontal transport is limited by the weak meridional gradients of water, whereas the fast convective cross-tropopause transport, largely missed by global models, can have a substantial effect, at least at a regional scale.


2019 ◽  
Author(s):  
Zhipeng Qu ◽  
Yi Huang ◽  
Paul A. Vaillancourt ◽  
Jason N. S. Cole ◽  
Jason A. Milbrandt ◽  
...  

Abstract. Stratospheric water vapor (SWV) is a climatically important atmospheric constituent due to its impacts on the radiation budget and atmospheric chemical composition. Despite the important role of SWV in the climate system, the processes controlling the distribution and variation of water vapor in the upper troposphere and lower stratosphere (UTLS) are not well understood. In order to better understand the mechanism of transport of water vapor through the tropopause, this study uses the high resolution Global Environmental Multiscale model of the Environment and Climate Change Canada, to simulate a lower stratosphere moistening event over North America. Satellite remote sensing and aircraft in situ observations are used to evaluate the quality of model simulation. The main focus of this study is to evaluate the processes that influence the lower stratosphere water vapor budget, particularly the direct water vapor transport and the moistening due to the ice sublimation. In the high-resolution simulations with horizontal grid-spacing less than 2.5 km, it is found that the main contribution to lower-stratospheric moistening is the upward transport caused by the breaking of gravity waves. In contrast, for the lower-resolution simulation with horizontal grid-spacing of 10 km, the lower-stratospheric moistening is dominated by the sublimation of ice. In comparison with the aircraft in situ observations, the high-resolution simulations predict well the water vapor content in the UTLS, while the lower resolution simulation over-estimates the water vapor content. This overestimation is associated with the overly abundant ice in the UTLS along with too-high sublimation rate in the lower stratosphere. The results of this study affirm the strong influence of overshooting convection on the lower-stratospheric water vapor and highlight the importance of both dynamics and microphysics in simulating the water vapor distribution in the UTLS region.


2020 ◽  
Author(s):  
Susan S. Kulawik ◽  
John R. Worden ◽  
Vivienne H. Payne ◽  
Dejian Fu ◽  
Steve C. Wofsy ◽  
...  

Abstract. We evaluate the uncertainties of methane optimal estimation retrievals from single footprint thermal infrared observations from the Atmospheric Infrared Sounder (AIRS). These retrievals are primarily sensitive to atmospheric methane in the mid-troposphere through the lower stratosphere (~2 to ~17 km). We compare to in situ observations made from aircraft during the Hiaper Pole to Pole Observations (HIPPO), the NASA Atmospheric Tomography Mission (ATom) campaigns, and from the NOAA ESRL aircraft network, between the surface and 5–13 km, across a range of years, latitudes between 60 S to 80 N, and over land and ocean. After a global, pressure dependent bias correction, we find that the land and ocean have similar biases and that the reported observation error (combined measurement and interference errors) of ~27  ppb is consistent with the standard deviation between aircraft and individual AIRS observations. A single measurement has measurement (noise related) uncertainty of ~17 ppb, a ~20 ppb uncertainty from radiative interferences (e.g. from water, temperature, etc.), and ~ 30 ppb due to smoothing error, which is partially removed when making comparisons to in situ measurements or models in a way that account for this regularization. We estimate a 16 ppb validation error because the aircraft typically did not measure methane at altitudes where the AIRS measurements have some sensitivity, e.g. the stratosphere. Daily averaged AIRS measurements of at least 9 observations over spatio-temporal domains of


2020 ◽  
Vol 20 (4) ◽  
pp. 2143-2159 ◽  
Author(s):  
Zhipeng Qu ◽  
Yi Huang ◽  
Paul A. Vaillancourt ◽  
Jason N. S. Cole ◽  
Jason A. Milbrandt ◽  
...  

Abstract. Stratospheric water vapour (SWV) is a climatically important atmospheric constituent due to its impacts on the radiation budget and atmospheric chemical composition. Despite the important role of SWV in the climate system, the processes controlling the distribution and variation in water vapour in the upper troposphere and lower stratosphere (UTLS) are not well understood. In order to better understand the mechanism of transport of water vapour through the tropopause, this study uses the high-resolution Global Environmental Multiscale model of the Environment and Climate Change Canada to simulate a lower stratosphere moistening event over North America. Satellite remote sensing and aircraft in situ observations are used to evaluate the quality of model simulation. The main focus of this study is to evaluate the processes that influence the lower stratosphere water vapour budget, particularly the direct water vapour transport and the moistening due to the ice sublimation. In the high-resolution simulations with horizontal grid spacing of less than 2.5 km, it is found that the main contribution to lower stratospheric moistening is the upward transport caused by the breaking of gravity waves. In contrast, for the lower-resolution simulation with horizontal grid spacing of 10 km, the lower stratospheric moistening is dominated by the sublimation of ice. In comparison with the aircraft in situ observations, the high-resolution simulations predict the water vapour content in the UTLS well, while the lower-resolution simulation overestimates the water vapour content. This overestimation is associated with the overly abundant ice in the UTLS along with a sublimation rate that is too high in the lower stratosphere. The results of this study affirm the strong influence of overshooting convection on the lower stratospheric water vapour and highlight the importance of both dynamics and microphysics in simulating the water vapour distribution in the UTLS region.


1999 ◽  
Vol 104 (D21) ◽  
pp. 26705-26714 ◽  
Author(s):  
R. M. Stimpfle ◽  
R. C. Cohen ◽  
G. P. Bonne ◽  
P. B. Voss ◽  
K. K. Perkins ◽  
...  

1995 ◽  
Vol 100 (D2) ◽  
pp. 3065 ◽  
Author(s):  
D. W. Fahey ◽  
E. R. Keim ◽  
E. L. Woodbridge ◽  
R. S. Gao ◽  
K. A. Boering ◽  
...  

2020 ◽  
Author(s):  
Christian Rolf ◽  
Felix Plöger ◽  
Martina Krämer ◽  
Martin Riese

&lt;p&gt;Water vapor is one of the most important greenhouse gases in the Earth&amp;#8217;s atmosphere. Due to the high sensitivity of atmospheric radiative forcing to changes in greenhouse gases in the cold upper troposphere and lower stratosphere (UTLS) region, even small variations in water vapor in the lower LS are an important source of the decadal variability of the surface temperature. This implies the need for a detailed understanding of the observed water vapor variability in the UTLS and their underlying processes.&lt;/p&gt;&lt;p&gt;Isentropic transport of water vapor due to planetary waves and their breaking provides a mechanism for bringing moist tropical tropospheric air into the dry lower extra-tropical stratosphere (exLS, see e.g. McIntyre and Palmer, 1983). Uplifted moist air masses by the Asian and American monsoons at the sub-tropical jet generate maximum water vapor concentrations in the summer/fall season. This water vapor maximum coincides with a maximum in planetary wave breaking in the northern hemisphere lower stratosphere and thus subsequent horizontal poleward transport. This transport serves as the dominant pathway to moisten the exLS in boreal summer (e.g. Ploeger et al., 2013 , Rolf et al. 2018).&lt;/p&gt;&lt;p&gt;We investigate this transport pathway with measurements to better understand the water vapor distribution and their annual cycle in the exLS. Here, we use in-situ measurements of water vapor obtained with the FISH instrument (Fast In-situ Stratospheric Hygrometer) during the aircraft field campaigns TACTS in August/ September 2012 and WISE in September/October 2017. Water vapor observations with the AURA MLS satellite instrument encompassing the entire exLS are used to put the temporal and spatial limited in-situ observations into a larger perspective. A very good agreement between the median of the in-situ water vapor distribution and the satellite observation is found, which shows that the in-situ observations are representative for the water vapor distribution of the exLS. Isentropic transport is shown to be dependent on the planetary wave activity by using the divergence of the Eliassen-Palm flux. Together with an extensive backward trajectory analysis we show that the isentropic transport is the dominant pathway of moistening the exLS up to 420 K potential temperature.&lt;/p&gt;&lt;p&gt;&lt;strong&gt;References&lt;/strong&gt;&lt;/p&gt;&lt;ul&gt;&lt;li&gt; &lt;p&gt;McIntyre, M. E., and T. N. Palmer (1983), Breaking planetary waves in the stratosphere, Nature, 305, 593-600.&lt;/p&gt; &lt;/li&gt; &lt;li&gt; &lt;p&gt;Ploeger, F., G&amp;#252;nther, G., Konopka, P., Fueglistaler, S., M&amp;#252;ller, R., Hoppe, C., Kunz, A., Spang, R., Groo&amp;#223;, J.&amp;#8208;U., and Riese, M. ( 2013), Horizontal water vapor transport in the lower stratosphere from subtropics to high latitudes during boreal summer, &lt;em&gt;J. Geophys. Res. Atmos.&lt;/em&gt;, 118, 8111&amp;#8211; 8127, doi:&lt;span&gt;&lt;/span&gt;.&lt;/p&gt; &lt;/li&gt; &lt;li&gt; &lt;p&gt;Rolf, C., Vogel, B., Hoor, P., Afchine, A., G&amp;#252;nther, G., Kr&amp;#228;mer, M., M&amp;#252;ller, R., M&amp;#252;ller, S., Spelten, N., and Riese, M.: Water vapor increase in the lower stratosphere of the Northern Hemisphere due to the Asian monsoon anticyclone observed during the TACTS/ESMVal campaigns, Atmos. Chem. Phys., 18, 2973&amp;#8211;2983, https://doi.org/10.5194/acp-18-2973-2018, 2018.&lt;/p&gt; &lt;/li&gt; &lt;/ul&gt;


Author(s):  
T. Marieb ◽  
J. C. Bravman ◽  
P. Flinn ◽  
D. Gardner ◽  
M. Madden

Electromigration and stress voiding have been active areas of research in the microelectronics industry for many years. While accelerated testing of these phenomena has been performed for the last 25 years[1-2], only recently has the introduction of high voltage scanning electron microscopy (HVSEM) made possible in situ testing of realistic, passivated, full thickness samples at high resolution.With a combination of in situ HVSEM and post-testing transmission electron microscopy (TEM) , electromigration void nucleation sites in both normal polycrystalline and near-bamboo pure Al were investigated. The effect of the microstructure of the lines on the void motion was also studied.The HVSEM used was a slightly modified JEOL 1200 EX II scanning TEM with a backscatter electron detector placed above the sample[3]. To observe electromigration in situ the sample was heated and the line had current supplied to it to accelerate the voiding process. After testing lines were prepared for TEM by employing the plan-view wedge technique [6].


2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Sze Hoon Gan ◽  
Zarinah Waheed ◽  
Fung Chen Chung ◽  
Davies Austin Spiji ◽  
Leony Sikim ◽  
...  

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