scholarly journals Evidence of horizontal and vertical transport of water in the Southern Hemisphere tropical tropopause layer (TTL) from high-resolution balloon observations

2016 ◽  
Vol 16 (18) ◽  
pp. 12273-12286 ◽  
Author(s):  
Sergey M. Khaykin ◽  
Jean-Pierre Pommereau ◽  
Emmanuel D. Riviere ◽  
Gerhard Held ◽  
Felix Ploeger ◽  
...  
Keyword(s):  
High Resolution ◽  
Water Vapour ◽  
Southern Hemisphere ◽  
Water Budget ◽  
Lower Stratosphere ◽  
Vertical Profiles ◽  
Tropical Tropopause Layer ◽  
Horizontal Transport ◽  
Tropical Tropopause

Abstract. High-resolution in situ balloon measurements of water vapour, aerosol, methane and temperature in the upper tropical tropopause layer (TTL) and lower stratosphere are used to evaluate the processes affecting the stratospheric water budget: horizontal transport (in-mixing) and hydration by cross-tropopause overshooting updrafts. The obtained in situ evidence of these phenomena are analysed using satellite observations by Aura MLS (Microwave Limb Sounder) and CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) together with trajectory and transport modelling performed using CLaMS (Chemical Lagrangian Model of the Stratosphere) and HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) model. Balloon soundings were conducted during March 2012 in Bauru, Brazil (22.3° S) in the frame of the TRO-Pico campaign for studying the impact of convective overshooting on the stratospheric water budget. The balloon payloads included two stratospheric hygrometers: FLASH-B (Fluorescence Lyman-Alpha Stratospheric Hygrometer for Balloon) and Pico-SDLA instrument as well as COBALD (Compact Optical Backscatter Aerosol Detector) sondes, complemented by Vaisala RS92 radiosondes. Water vapour vertical profiles obtained independently by the two stratospheric hygrometers are in excellent agreement, ensuring credibility of the vertical structures observed. A signature of in-mixing is inferred from a series of vertical profiles, showing coincident enhancements in water vapour (of up to 0.5 ppmv) and aerosol at the 425 K (18.5 km) level. Trajectory analysis unambiguously links these features to intrusions from the Southern Hemisphere extratropical stratosphere, containing more water and aerosol, as demonstrated by MLS and CALIPSO global observations. The in-mixing is successfully reproduced by CLaMS simulations, showing a relatively moist filament extending to 20° S. A signature of local cross-tropopause transport of water is observed in a particular sounding, performed on a convective day and revealing water vapour enhancements of up to 0.6 ppmv as high as the 404 K (17.8 km) level. These are shown to originate from convective overshoots upwind detected by an S-band weather radar operating locally in Bauru. The accurate in situ observations uncover two independent moisture pathways into the tropical lower stratosphere, which are hardly detectable by space-borne sounders. We argue that the moistening by horizontal transport is limited by the weak meridional gradients of water, whereas the fast convective cross-tropopause transport, largely missed by global models, can have a substantial effect, at least at a regional scale.

scholarly journals Evidence of horizontal and vertical transport of water in the Southern Hemisphere Tropical Tropopause Layer (TTL) from high-resolution balloon observations

2016 ◽  
pp. 1-15
Author(s):  
Sergey M. Khaykin ◽  
Jean-Pierre Pommereau ◽  
Emmanuel D. Riviere ◽  
Gerhard Held ◽  
Felix Ploeger ◽  
...  
Keyword(s):  
High Resolution ◽  
Water Vapour ◽  
Southern Hemisphere ◽  
Water Budget ◽  
Lower Stratosphere ◽  
Vertical Profiles ◽  
Tropical Tropopause Layer ◽  
Horizontal Transport ◽  
Tropical Tropopause

High-resolution in situ balloon measurements of water vapour, aerosol, methane and temperature in the upper Tropical Tropopause Layer (TTL) and lower stratosphere are used to evaluate the processes controlling the stratospheric water budget: horizontal transport (inmixing) and hydration by cross-tropopause overshooting updrafts. The obtained in situ evidences of these phenomena are analyzed using satellite observations by Aura MLS (Microwave Limb Sounder) and CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) together with trajectory and transport modeling performed using CLaMS (Chemical Lagrangian Model of the Stratosphere) and HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model. <br><br> Balloon soundings were conducted during March 2012 in Bauru, Brazil (22.3°&thinsp;S) in the frame of the TRO-Pico campaign for studying the impact of convective overshooting on the stratospheric water budget. The balloon payloads included two stratospheric hygrometers: FLASH-B (Fluorescence Lyman-Alpha Stratospheric Hygrometer for Balloon) and Pico-SDLA instrument as well as COBALD (Compact Optical Backscatter Aerosol Detector) sondes, complemented by Vaisala RS-92 radiosondes. Water vapour vertical profiles obtained independently by the two stratospheric hygrometers are in excellent agreement, ensuring credibility of the vertical structures observed. <br><br> A signature of in-mixing is inferred from a series of vertical profiles, showing coincident enhancements in water vapour and aerosol at the 425&thinsp;K (18.5&thinsp;km) level. Trajectory analysis unambiguously links these features to intrusions from the Southern Hemisphere extra-tropical stratosphere, containing more water and aerosol, as demonstrated by MLS and CALIPSO global observations. The in-mixing is successfully reproduced by CLaMS simulations, showing a relatively moist filament extending to 20&thinsp;S°. A signature of local cross-tropopause transport of water is observed in a particular sounding, performed on a convective day and revealing water vapour enhancements of up to 0.6&thinsp;ppmv as high as the 404&thinsp;K (17.8&thinsp;km) level. These are shown to originate from convective overshoots upwind detected by an S-band weather radar operating locally in Bauru. <br><br> The accurate in situ observations uncover two independent moisture pathways into the tropical lower stratosphere, whose manifestations are hardly detectable by space-borne sounders. We argue that the moistening by horizontal transport is limited by the weak meridional gradients of water, whereas the fast convective cross-tropopause transport, largely missed by global models, can have a substantial effect, at least at a regional scale.

scholarly journals Representation of Vertical Atmospheric Structures by Radio Occultation Observations in the Upper Troposphere and Lower Stratosphere: Comparison to High-Resolution Radiosonde Profiles

2019 ◽  
Vol 36 (4) ◽  
pp. 655-670 ◽  
Author(s):  
Zhen Zeng ◽  
Sergey Sokolovskiy ◽  
William S. Schreiner ◽  
Doug Hunt
Keyword(s):  
High Resolution ◽  
Radio Occultation ◽  
Lower Stratosphere ◽  
Small Scale ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Low Latitudes ◽  
Observational Noise ◽  
Horizontal Inhomogeneity ◽  
Cold Point

AbstractGlobal positioning system (GPS) radio occultation (RO) is capable of retrieving vertical profiles of atmospheric parameters with high resolution (<100 m), which can be achieved in spherically symmetric atmosphere. Horizontal inhomogeneity of real atmosphere results in representativeness errors of retrieved profiles. In most cases these errors increase with a decrease of vertical scales of atmospheric structures and may not allow one to fully utilize the physical resolution of RO. Also, GPS RO–retrieved profiles are affected by observational noise of different types, which, in turn, affect the representation of small-scale atmospheric structures. This study investigates the effective resolution and optimal smoothing of GPS RO–retrieved temperature profiles using high-pass filtering and cross correlation with collocated high-resolution radiosondes. The effective resolution is a trade-off between representation of real atmospheric structures and suppression of observational noise, which varies for different latitudes (15°S–75°N) and altitudes (10–27 km). Our results indicate that at low latitudes the effective vertical resolution is about 0.2 km near the tropical tropopause layer and about 0.5 km in the lower stratosphere. The best resolution of 0.1 km is at the cold-point tropical tropopause. The effective resolutions at the midlatitudes are slightly worse than at low latitudes, varying from ~0.2 to 0.6 km. At high latitudes, the effective resolutions change notably with altitude from ~0.2 km at 10–15 km to ~1.4 km at 22–27 km. Our results suggest that the atmospheric inhomogeneity plays an important role in the representation of the vertical atmospheric structures by RO measurements.

scholarly journals Convective hydration in the tropical tropopause layer during the StratoClim aircraft campaign: pathway of an observed hydration patch

2019 ◽  
Vol 19 (18) ◽  
pp. 11803-11820 ◽  
Author(s):  
Keun-Ok Lee ◽  
Thibaut Dauhut ◽  
Jean-Pierre Chaboureau ◽  
Sergey Khaykin ◽  
Martina Krämer ◽  
...  
Keyword(s):  
Water Vapour ◽  
Lower Stratosphere ◽  
Asian Summer Monsoon ◽  
Great Part ◽  
The South ◽  
Water Vapour Content ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Water Vapour Concentration ◽  
Ice Content

Abstract. The source and pathway of the hydration patch in the TTL (tropical tropopause layer) that was measured during the Stratospheric and upper tropospheric processes for better climate predictions (StratoClim) field campaign during the Asian summer monsoon in 2017 and its connection to convective overshoots are investigated. During flight no. 7, two remarkable layers are measured in the TTL, namely (1) the moist layer (ML) with a water vapour content of 4.8–5.7 ppmv in altitudes of 18–19 km in the lower stratosphere and (2) the ice layer (IL) with ice content up to 1.9 eq. ppmv (equivalent parts per million by volume) in altitudes of 17–18 km in the upper troposphere at around 06:30 UTC on 8 August to the south of Kathmandu (Nepal). A Meso-NH convection-permitting simulation succeeds in reproducing the characteristics of the ML and IL. Through analysis, we show that the ML and IL are generated by convective overshoots that occurred over the Sichuan Basin about 1.5 d before. Overshooting clouds develop at altitudes up to 19 km, hydrating the lower stratosphere of up to 20 km with 6401 t of water vapour by a strong-to-moderate mixing of the updraughts with the stratospheric air. A few hours after the initial overshooting phase, a hydration patch is generated, and a large amount of water vapour (above 18 ppmv) remains at even higher altitudes up to 20.5 km while the anvil cloud top descends to 18.5 km. At the same time, a great part of the hydrometeors falls shortly, and the water vapour concentration in the ML and IL decreases due to turbulent diffusion by mixing with the tropospheric air, ice nucleation, and water vapour deposition. As the hydration patch continues to travel toward the south of Kathmandu, tropospheric tracer concentration increases up to ∼30 % and 70 % in the ML and IL, respectively. The air mass in the layers becomes gradually diffused, and it has less and less water vapour and ice content by mixing with the dry tropospheric air.

scholarly journals Isentropic advection and convective lifting of water vapor in the UT – LS as observed over Brazil (22° S) in February 2004 by in situ high-resolution measurements of H<sub>2</sub>O, CH<sub>4</sub>, O<sub>3</sub> and temperature

2006 ◽  
Vol 6 (6) ◽  
pp. 12469-12501 ◽  
Author(s):  
G. Durry ◽  
N. Huret ◽  
A. Hauchecorne ◽  
V. Marecal ◽  
J.-P. Pommereau ◽  
...  
Keyword(s):  
High Resolution ◽  
Convective Transport ◽  
Thin Layers ◽  
Potential Contribution ◽  
Laser Sensor ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Diode Laser Spectrometer ◽  
Cold Point

Abstract. The micro-SDLA balloonborne diode laser spectrometer was flown twice from Bauru (22° S, Brazil) in February 2004 during HIBISCUS to yield in situ H2O measurements in the Upper Troposphere (UT) and Lower Stratosphere (LS) and in particular in the Tropical Tropopause Layer (TTL). The overall TTL was found warmer (with a subsaturated cold point near –79°C) and the LS moister compared to former measurements obtained in tropical oceanic conditions. The use of specific balloons with a slow descent, combined with the high-resolution of the laser sensor, allowed us to observe in situ in the UT, the TTL and the LS several thin layers correlated on H2O, CH4, O3, temperature and PV. A component of these layers is associated with the isentropic transport into the UT- LS of extratropical stratospheric air masses. Moreover, the examination of temperature and tracer (CH4, O3) profiles gives insights on the potential contribution of convective transport of H2O in the TTL.

scholarly journals Impact of tropical land convection on the water vapour budget in the Tropical Tropopause Layer

2013 ◽  
Vol 13 (12) ◽  
pp. 33055-33087
Author(s):  
F. Carminati ◽  
P. Ricaud ◽  
J.-P. Pommereau ◽  
E. Rivière ◽  
S. Khaykin ◽  
...  
Keyword(s):  
Water Vapour ◽  
Diurnal Cycle ◽  
Lower Stratosphere ◽  
Regional Scale ◽  
Maritime Continent ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Geographical Variations ◽  
Water Vapour Concentration ◽  
Ice Water

Abstract. The tropical deep overshooting convection is known to be most intense above continental areas such as South America, Africa and the maritime continent. However, its impact on the Tropical Tropopause Layer (TTL) at global scale remains debated. In our analysis, we use the 8 yr Microwave Limb Sounder (MLS) water vapour (H2O), cloud ice water content (IWC) and temperature datasets from 2005 to date, to highlight the interplays between these parameters and their role in the water vapour variability in the TTL, separately in the northern and southern tropics. The water vapour concentration is displaying a systematic diurnal cycle with a night-time peak in the tropical Upper Troposphere (pressure ≥146 hPa) and the opposite in the TTL (121 to 68 hPa) and the tropical Lower Stratosphere (pressure ≤56 hPa), of larger amplitude above continents than continental-oceanic areas such as the maritime continent or full oceanic areas such as the Western Pacific. In addition, the amplitude of the diurnal cycle is found systematically larger (5–10%) in the southern than in the northern tropics during their respective summer, indicative of a more vigorous convective intensity in the south. Using a regional scale approach, we investigate the geographical variations of mechanisms linked to the H2O variability. In summary, the MLS water vapour, ice water cloud and temperature observations are demonstrating a clear contribution of TTL and lower stratosphere moistening by ice crystals overshooting updrafts over land tropical regions and the much greater efficiency of the process in the Southern Hemisphere.

scholarly journals A Reel-Down Instrument System for Profile Measurements of Water Vapor, Temperature, Clouds and Aerosol Beneath Constant Altitude Scientific Balloons

2020 ◽  
Author(s):  
Lars E. Kalnajs ◽  
Sean M. Davis ◽  
J. Douglas Goetz ◽  
Terry Deshler ◽  
Sergey Khaykin ◽  
...  
Keyword(s):  
Water Vapor ◽  
High Resolution ◽  
Stratospheric Ozone ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Long Duration ◽  
Constant Altitude ◽  
And Control ◽  
Vapor Temperature

Abstract. The Tropical Tropopause Layer (14–18.5 km) is the gateway for most air entering the stratosphere, and therefore processes within this layer have an outsized influence in determining global stratospheric ozone and water vapor concentrations. Despite the importance of this layer there are few in situ measurements with the necessary detail to resolve the fine scale processes within this region. Here, we introduce a novel platform for high resolution in situ profiling that lowers and retracts a suspended instrument package beneath drifting long duration balloons in the tropics. During a 100-day circumtropical flight, the instrument collected over 100 two-kilometer profiles of temperature, water vapor and aerosol at one-meter resolution, yielding unprecedented geographic sampling and vertical resolution. The instrument system integrates proven sensors for water vapor, temperature, pressure and cloud and aerosol particles with an innovative mechanical reeling and control system. A technical evaluation of the system performance demonstrated the feasibility of this new measurement platform for future missions with minor modifications. Six instruments planned for two upcoming field campaigns are expected to provide over 4000 profiles through the TTL, quadrupling the number of high-resolution aircraft and balloon profiles collected to date. These and future measurements will provide the necessary resolution to diagnose the importance of competing mechanisms for the transport of water vapor across the TTL.

scholarly journals Diagnostics of the Tropical Tropopause Layer from in-situ observations and CCM data

2009 ◽  
Vol 9 (3) ◽  
pp. 11659-11698
Author(s):  
E. Palazzi ◽  
F. Fierli ◽  
F. Cairo ◽  
C. Cagnazzo ◽  
G. Di Donfrancesco ◽  
...  
Keyword(s):  
Vertical Structure ◽  
Climate Model ◽  
Joint Analysis ◽  
Vertical Profiles ◽  
Transport Barrier ◽  
Tropical Tropopause Layer ◽  
Mixing Ratios ◽  
Tropical Tropopause ◽  
Scatter Plots

Abstract. A suite of diagnostics is applied to in-situ aircraft measurements and one Chemistry-Climate Model (CCM) data to characterize the vertical structure of the Tropical Tropopause Layer (TTL). The diagnostics are based on the vertical tracers profiles, relative vertical tracers gradients, and tracer-tracer relationships in the tropical Upper Troposphere/Lower Stratosphere (UT/LS), using tropopause coordinates. Observations come from the four tropical campaigns performed from 1998 to 2006 with the research aircraft Geophysica and have been directly compared to the output of the ECHAM5/MESSy CCM. The model vertical resolution in the TTL allows for appropriate comparison with high-resolution aircraft observations and the diagnostics used highlight common TTL features between the model and the observational data. The analysis of the vertical profiles of water vapour, ozone, and nitrous oxide, in both the observations and the model, shows that concentration mixing ratios exhibit a strong gradient change across the tropical tropopause, due to the role of this latter as a transport barrier and that transition between the tropospheric and stratospheric regimes occurs within a finite layer. The use of relative vertical ozone gradients, in addition to the vertical profiles, helps to highlight the region where this transition occurs and allows to give an estimate of its thickness. The analysis of the CO-O3 and H2O-O3 scatter plots and of the Probability Distribution Function (PDF) of the H2O-O3 pair completes this picture as it allows to better distinguish tropospheric and stratospheric regimes that can be identified, first, by their differing chemical composition. The joint analysis and comparison of observed and modelled data allows us to evaluate the capability of the model in reproducing the observed vertical structure of the TTL and its variability, and also to assess whether observations from particular regions on a monthly timescale can be representative of the fine scale mean structure of the Tropical Tropopause Layer.

scholarly journals More evidence for very short-lived substance contribution to stratospheric chlorine inferred from HCl balloon-borne in situ measurements in the tropics

2010 ◽  
Vol 10 (2) ◽  
pp. 397-409 ◽  
Author(s):  
Y. Mébarki ◽  
V. Catoire ◽  
N. Huret ◽  
G. Berthet ◽  
C. Robert ◽  
...  
Keyword(s):  
In Situ Measurements ◽  
Tunable Diode Laser ◽  
Vertical Profiles ◽  
Tropical Tropopause Layer ◽  
Laser Absorption ◽  
Tropical Tropopause ◽  
Product Gas ◽  
Gas Measurements ◽  
The Tropics

Abstract. Volume mixing ratio (vmr) vertical profiles of hydrogen chloride (HCl) are retrieved from in situ measurements performed by a balloon-borne infrared tunable diode laser absorption spectrometer (SPIRALE) during two balloon flights in the tropics (Teresina, Brazil, 5.1° S–42.9° W) in June 2005 and June 2008. HCl vertical profiles obtained from 15 to 31 km are presented and analysed to estimate the contribution of very short-lived substances (VSLS) to total stratospheric chlorine. Both retrieved vertical profiles of HCl from these flights agree very well with each other, with estimated overall uncertainties of 6% on vmr between 23 and 31 km. Upper limits of HCl vmr as low as 20 pptv in June 2008 and 30 pptv in June 2005 are inferred in the upper part of the tropical tropopause layer (TTL). Backward trajectory calculations and such low amounts suggest that the air masses sampled correspond to typical background conditions, i.e. neither influenced by recent tropospheric nor stratospheric air. Taking into account the recently reported VSL source gas measurements obtained in similar conditions (Laube et al., 2008) and the main intermediate degradation product gas COCl2 (Fu et al., 2007), a total VSLS contribution of 85±40 pptv to stratospheric chlorine is inferred. This refines the WMO (2007) estimation of 50 to 100 pptv, which was not taking into account any HCl contribution. In addition, comparisons of HCl measurements between SPIRALE and the Aura MLS satellite instrument in the tropical lower and middle stratosphere lead to a very good agreement. The previous agreement between MLS-deduced upper stratospheric total chlorine content and modelled values including 100 pptv of VSLS (Froidevaux et al., 2006) is thus supported by our present result about the VSLS contribution.

scholarly journals Insight from ozone and water vapour on transport in the tropical tropopause layer (TTL)

2011 ◽  
Vol 11 (1) ◽  
pp. 407-419 ◽  
Author(s):  
F. Ploeger ◽  
S. Fueglistaler ◽  
J.-U. Grooß ◽  
G. Günther ◽  
P. Konopka ◽  
...  
Keyword(s):  
Water Vapour ◽  
Potential Temperature ◽  
Transport Processes ◽  
Ozone Production ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
High Bias ◽  
Highly Correlated ◽  
Vertical Ozone

Abstract. We explore the potential of ozone observations to constrain transport processes in the tropical tropopause layer (TTL), and contrast it with insights that can be obtained from water vapour. Global fields from Halogen Occultation Experiment (HALOE) and in-situ observations are predicted using a backtrajectory approach that captures advection, instantaneous freeze-drying and photolytical ozone production. Two different representations of transport (kinematic and diabatic 3-month backtrajectories based on ERA-Interim data) are used to evaluate the sensitivity to differences in transport. Results show that mean profiles and seasonality of both tracers can be reasonably reconstructed. Water vapour predictions are similar for both transport representations, but predictions for ozone are systematically higher for kinematic transport. Compared to global HALOE observations, the diabatic model prediction underestimates the vertical ozone gradient. Comparison of the kinematic prediction with observations obtained during the tropical SCOUT-O3 campaign shows a large high bias above 390 K potential temperature. We show that ozone predictions and vertical dispersion of the trajectories are highly correlated, rendering ozone an interesting tracer for aspects of transport to which water vapour is not sensitive. We show that dispersion and mean upwelling have similar effects on ozone profiles, with slower upwelling and larger dispersion both leading to higher ozone concentrations. Analyses of tropical upwelling based on mean transport characteristics, and model validation have to take into account this ambiguity between tropical ozone production and in-mixing from the stratosphere. In turn, ozone provides constraints on transport in the TTL and lower stratosphere that cannot be obtained from water vapour.

scholarly journals Diagnostics of the Tropical Tropopause Layer from in-situ observations and CCM data

2009 ◽  
Vol 9 (24) ◽  
pp. 9349-9367 ◽  
Author(s):  
E. Palazzi ◽  
F. Fierli ◽  
F. Cairo ◽  
C. Cagnazzo ◽  
G. Di Donfrancesco ◽  
...  
Keyword(s):  
Climate Model ◽  
Regional Scale ◽  
Transport Processes ◽  
Joint Analysis ◽  
Vertical Profiles ◽  
Transport Barrier ◽  
Model Estimate ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause

Abstract. A suite of diagnostics is applied to in-situ aircraft measurements and one Chemistry-Climate Model (CCM) data to characterize the vertical structure of the Tropical Tropopause Layer (TTL). The diagnostics are based on vertical tracer profiles and relative vertical tracer gradients, using tropopause-referenced coordinates, and tracer-tracer relationships in the tropical Upper Troposphere/Lower Stratosphere (UT/LS). Observations were obtained during four tropical campaigns performed from 1999 to 2006 with the research aircraft Geophysica and have been compared to the output of the ECHAM5/MESSy CCM. The model vertical resolution in the TTL (~500 m) allows for appropriate comparison with high-resolution aircraft observations and the diagnostics used highlight common TTL features between the model and the observational data. The analysis of the vertical profiles of water vapour, ozone, and nitrous oxide, in both the observations and the model, shows that concentration mixing ratios exhibit a strong gradient change across the tropical tropopause, due to the role of this latter as a transport barrier and that transition between the tropospheric and stratospheric regimes occurs within a finite layer. The use of relative vertical ozone and carbon monoxide gradients, in addition to the vertical profiles, helps to highlight the region where this transition occurs and allows to give an estimate of its thickness. The analysis of the CO-O3 and H2O-O3 scatter plots and of the Probability Distribution Function (PDF) of the H2O-O3 pair completes this picture as it allows to better distinguish tropospheric and stratospheric regimes that can be identified by their different chemical composition. The joint analysis and comparison of observed and modelled data allows to state that the model can represent the background TTL structure and its seasonal variability rather accurately. The model estimate of the thickness of the interface region between tropospheric and stratospheric regimes agrees well with average values inferred from observations. On the other hand, the measurements can be influenced by regional scale variability, local transport processes as well as deep convection, that can not be captured by the model.

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