Abstract. Black carbon (BC) is the most important light-absorbing aerosol in the atmosphere. However, sources of atmospheric BC aerosols are largely
uncertain, making it difficult to assess its influence on radiative forcing
and climate change. In this study, year-round light-absorption observations
were conducted during 2014 using an aethalometer in Xiamen, a coastal city in Southeast China. Source apportionment of BC was performed and temporal
variations in BC sources were characterized based on both light absorption
measurements and a source-oriented air quality model. The annual average
concentrations of BC from fossil fuel (BCff) and biomass burning
(BCbb) by the aethalometer method were 2932 ± 1444 ng m−3 and 1340 ± 542 ng m−3, contributing 66.7 % and 33.3 % to
total BC, respectively. A sensitivity analysis was performed with different
absorption Ångström exponent (AAE) values of fossil fuel combustion (αff) and biomass burning (αbb), suggesting that
the aethalometer method was more sensitive to changes in αbb than αff. BCbb contribution exhibited a clear diurnal cycle, with the highest level (37.9 %) in the evening rush hour and a seasonal pattern with the maximum (39.9 %) in winter. Conditional probability
function (CPF) analysis revealed the large biomass-burning contributions were accompanied by east-northeasterly and northerly winds. Backward
trajectory indicated that air masses from North and East–Central China were associated with larger biomass-burning contributions. Potential source contribution function (PSCF) and concentration-weighted trajectory (CWT)
suggested that North and East–Central China and Southeast Asia were potential sources of both BCff and BCbb. The source-oriented modeling results showed that transportation, residential and open biomass
burning accounting for 45.3 %, 30.1 % and 17.6 % were the major BC
sources. Among the three fuel catalogs, liquid fossil fuel (46.5 %) was
the largest source, followed by biomass burning (32.6 %) and coal
combustion (20.9 %). Source contributions of fossil fuel combustion and
biomass burning identified by the source-oriented model were 67.4 % and
32.6 %, respectively, close to those obtained by the aethalometer method. The findings provide solid support for controlling fossil fuel sources to limit the impacts of BC on climate change and environmental degradation in
the relatively clean region in China.