Vertical distribution of H2O in the stratosphere as determined by UV fluorescence in-situ measurements

1978 ◽  
Vol 5 (12) ◽  
pp. 1017-1020 ◽  
Author(s):  
Jean-Loup Bertaux ◽  
Alain Delannoy
2021 ◽  
Author(s):  
Mikhail Yu. Arshinov ◽  
Boris Belan ◽  
Denis Davydov ◽  
Artem Kozlov ◽  
Alexandr Fofonov

<p>The Arctic is warming much faster than other regions of the globe. In 2020, temperature anomalies in the Russian Arctic reached unprecedented high levels. The atmospheric composition in this key region still remains insufficiently studied that makes difficult predicting future climate change.</p><p>In September 2020, an extensive aircraft campaign was conducted to document the tropospheric composition over the Russian Arctic. The Optik Tu-134 research aircraft was equipped with instruments to carry out in-situ measurements of trace gases and aerosols, as well as with a lidar for profiling of aerosol backscatter. The aircraft flew over a vast area from Arkhangelsk to Anadyr. Six measurement flights with changing altitudes from 0.2 to 9.0 m were conducted over the waters of the Barents, Kara, Laptev, East Siberian, Chukchi, and Bering Seas. The weather was unusually warm for this period of the year, surface air temperatures were above 0°C through the campaign.</p><p>Here, we present the results of in-situ measurements of the vertical distribution of aerosol number concentrations in a wide range of sizes. A modified diffusional particle sizer (DPS) consisted of the Novosibirsk-type eight-stage screen diffusion battery connected to the TSI condensation particle counter Model 3756 was used to determine the number size distribution of particles between 0.003 mm and 0.2 mm (20 size bins). Distribution of particles in the size range from 0.25 µm to 32 µm (31 size bins) was measured by means of the Grimm aerosol spectrometer Model 1.109.</p><p>The flights over Barents and Kara Seas were predominantly performed under clear sky or partly cloudy weather conditions. Number size distributions were wide representing particles of almost all aerosol fractions. When flying in the upper troposphere with a constant altitude over these seas, some cases of enhanced concentrations of nucleation and Aitken mode particles comparable to ones in the lower troposphere were recorded, suggesting in situ new particle formation was likely to be taking place via gas-to-particle conversion aloft.</p><p>East of the Kara Sea, flights were conducted under mostly cloudy conditions resulting in a lower median aerosol number concentration and narrower size distributions.</p><p>This work was supported by the Russian Foundation for Basic Research (Grant No. 19-05-50024).</p>


2005 ◽  
Vol 62 (4) ◽  
pp. 1093-1117 ◽  
Author(s):  
Jacek Chowdhary ◽  
Brian Cairns ◽  
Michael I. Mishchenko ◽  
Peter V. Hobbs ◽  
Glenn F. Cota ◽  
...  

Abstract The extensive set of measurements performed during the Chesapeake Lighthouse and Aircraft Measurements for Satellites (CLAMS) experiment provides a unique opportunity to evaluate aerosol retrievals over the ocean from multiangle, multispectral photometric, and polarimetric remote sensing observations by the airborne Research Scanning Polarimeter (RSP) instrument. Previous studies have shown the feasibility of retrieving particle size distributions and real refractive indices from such observations for visible wavelengths without prior knowledge of the ocean color. This work evaluates the fidelity of the aerosol retrievals using RSP measurements during the CLAMS experiment against aerosol properties derived from in situ measurements, sky radiance observations, and sun-photometer measurements, and further extends the scope of the RSP retrievals by using a priori information about the ocean color to constrain the aerosol absorption and vertical distribution. It is shown that the fine component of the aerosol observed on 17 July 2001 consisted predominantly of dirty sulfatelike particles with an extinction optical thickness of several tenths in the visible, an effective radius of 0.15 ± 0.025 μm and a single scattering albedo of 0.91 ± 0.03 at 550 nm. Analyses of the ocean color and sky radiance observations favor the lower boundary of aerosol single scattering albedo, while in situ measurements favor its upper boundary. Both analyses support the polarimetric retrievals of fine-aerosol effective radius and the consequent spectral variation in extinction optical depth. The estimated vertical distribution of this aerosol component depends on assumptions regarding the water-leaving radiances and is consistent with the top of the aerosol layer being close to the aircraft height (3500 m), with the bottom of the layer being between 2.7 km and the surface. The aerosol observed on 17 July 2001 also contained coarse-mode particles. Comparison of RSP data with sky radiance and in situ measurements suggests that this component consists of nonspherical particles with an effective radius in excess of 1 μm, and with the extinction optical depth being much less than one-tenth at 550 nm.


2019 ◽  
Author(s):  
Michael Stukel ◽  
Thomas Kelly

Thorium-234 (234Th) is a powerful tracer of particle dynamics and the biological pump in the surface ocean; however, variability in carbon:thorium ratios of sinking particles adds substantial uncertainty to estimates of organic carbon export. We coupled a mechanistic thorium sorption and desorption model to a one-dimensional particle sinking model that uses realistic particle settling velocity spectra. The model generates estimates of 238U-234Th disequilibrium, particulate organic carbon concentration, and the C:234Th ratio of sinking particles, which are then compared to in situ measurements from quasi-Lagrangian studies conducted on six cruises in the California Current Ecosystem. Broad patterns observed in in situ measurements, including decreasing C:234Th ratios with depth and a strong correlation between sinking C:234Th and the ratio of vertically-integrated particulate organic carbon (POC) to vertically-integrated total water column 234Th, were accurately recovered by models assuming either a power law distribution of sinking speeds or a double log normal distribution of sinking speeds. Simulations suggested that the observed decrease in C:234Th with depth may be driven by preferential remineralization of carbon by particle-attached microbes. However, an alternate model structure featuring complete consumption and/or disaggregation of particles by mesozooplankton (e.g. no preferential remineralization of carbon) was also able to simulate decreasing C:234Th with depth (although the decrease was weaker), driven by 234Th adsorption onto slowly sinking particles. Model results also suggest that during bloom decays C:234Th ratios of sinking particles should be higher than expected (based on contemporaneous water column POC), because high settling velocities minimize carbon remineralization during sinking.


2013 ◽  
Vol 24 (3) ◽  
pp. 147
Author(s):  
Ming LI ◽  
Qinghua YANG ◽  
Jiechen ZHAO ◽  
Lin ZHANG ◽  
Chunhua LI ◽  
...  

1995 ◽  
Vol 31 (7) ◽  
pp. 51-59 ◽  
Author(s):  
Ian Guymer ◽  
Rob O'Brien

Previously, the design of sewer systems has been limited to studies of their hydraulic characteristics, in particular the ability of the system to convey the maximum discharge. Greater environmental awareness has necessitated that new designs, and some existing schemes, are assessed to determine the environmental load which the scheme will deliver to any downstream component. This paper describes a laboratory programme which has been designed to elucidate the effects of manholes on the longitudinal dispersion of solutes. A laboratory system is described, which allows in situ measurements to be taken of the concentration of a fluorescent solute tracer, both up- and down-stream of a surcharged manhole junction. Results are presented from a preliminary series of studies undertaken for a single manhole geometry over a range of discharges, with varying levels of surcharge. Results are presented showing the variation of travel time, change in second moment of the distribution and of a dispersion factor with surcharge, assuming a Taylor approach and determining the dispersion factor using a ‘change in moment’ method. The effect of the stored volume within the manhole is clearly evident. The limitations and the applicability of this approach are discussed.


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