scholarly journals Ultrafast imaging of terahertz electric waveforms using quantum dots

2022 ◽  
Vol 11 (1) ◽  
Author(s):  
Moritz B. Heindl ◽  
Nicholas Kirkwood ◽  
Tobias Lauster ◽  
Julia A. Lang ◽  
Markus Retsch ◽  
...  
Keyword(s):  
Electric Fields ◽  
Stark Effect ◽  
Strong Field ◽  
Probe Field ◽  
Ultrafast Imaging ◽  
Strength Limit ◽  
Colloidal Quantum Dot ◽  
Field Excitation ◽  
Field Imaging ◽  
Sub Wavelength

AbstractMicroscopic electric fields govern the majority of elementary excitations in condensed matter and drive electronics at frequencies approaching the Terahertz (THz) regime. However, only few imaging schemes are able to resolve sub-wavelength fields in the THz range, such as scanning-probe techniques, electro-optic sampling, and ultrafast electron microscopy. Still, intrinsic constraints on sample geometry, acquisition speed and field strength limit their applicability. Here, we harness the quantum-confined Stark-effect to encode ultrafast electric near-fields into colloidal quantum dot luminescence. Our approach, termed Quantum-probe Field Microscopy (QFIM), combines far-field imaging of visible photons with phase-resolved sampling of electric waveforms. By capturing ultrafast movies, we spatio-temporally resolve a Terahertz resonance inside a bowtie antenna and unveil the propagation of a Terahertz waveguide excitation deeply in the sub-wavelength regime. The demonstrated QFIM approach is compatible with strong-field excitation and sub-micrometer resolution—introducing a direct route towards ultrafast field imaging of complex nanodevices in-operando.

Application of a numerical-basis-state method to strong-field excitation and ionization of hydrogen atoms

2012 ◽  
Vol 86 (1) ◽  
Author(s):  
Shaohao Chen ◽  
Xiang Gao ◽  
Jiaming Li ◽  
Andreas Becker ◽  
Agnieszka Jaroń-Becker
Keyword(s):  
Strong Field ◽  
Hydrogen Atoms ◽  
State Method ◽  
Field Excitation

scholarly journals Derivative corrections to the Heisenberg-Euler effective action

2021 ◽  
Vol 2021 (9) ◽  
Author(s):  
Felix Karbstein
Keyword(s):  
Electric Fields ◽  
Effective Action ◽  
Vacuum Polarization ◽  
Strong Field ◽  
Background Field ◽  
Polarization Tensor ◽  
Quantum Vacuum ◽  
Electron Positron ◽  
Vacuum Polarization Tensor ◽  
Electron Positron Pair

Abstract We show that the leading derivative corrections to the Heisenberg-Euler effective action can be determined efficiently from the vacuum polarization tensor evaluated in a homogeneous constant background field. After deriving the explicit parameter-integral representation for the leading derivative corrections in generic electromagnetic fields at one loop, we specialize to the cases of magnetic- and electric-like field configurations characterized by the vanishing of one of the secular invariants of the electromagnetic field. In these cases, closed-form results and the associated all-orders weak- and strong-field expansions can be worked out. One immediate application is the leading derivative correction to the renowned Schwinger-formula describing the decay of the quantum vacuum via electron-positron pair production in slowly-varying electric fields.

scholarly journals Piezoelectric Level Splitting in GaInN/GaN Quantum Wells

1999 ◽  
Vol 4 (S1) ◽  
pp. 357-362
Author(s):  
C. Wetzel ◽  
T. Takeuchi ◽  
H. Amano ◽  
I. Akasaki
Keyword(s):  
Quantum Wells ◽  
Electric Fields ◽  
High Performance ◽  
Stark Effect ◽  
Electronic Band Structure ◽  
Multiple Quantum Well ◽  
Multiple Quantum ◽  
Large Set ◽  
Electronic Band ◽  
Level Splitting

Identification of the electronic band structure in AlInGaN heterostructures is the key issue in high performance light emitter and switching devices. In device-typical GaInN/GaN multiple quantum well samples in a large set of variable composition a clear correspondence of transitions in photo- and electroreflection, as well as photoluminescence is found. The effective band offset across the GaN/GaInN/GaN piezoelectric heterointerface is identified and electric fields from 0.23 - 0.90 MV/cm are directly derived. In the bias voltage dependence a level splitting within the well is observed accompanied by the quantum confined Stark effect. We furthermore find direct correspondence of luminescence bands with reflectance features. This indicates the dominating role of piezoelectric fields in the bandstructure of such typical strained layers.

scholarly journals Terahertz Field Confinement in Nonlinear Metamaterials and Near-Field Imaging

Photonics ◽  
2019 ◽  
Vol 6 (1) ◽  
pp. 22 ◽  
Author(s):  
George Keiser ◽  
Pernille Klarskov
Keyword(s):  
Terahertz Radiation ◽  
Terahertz Spectroscopy ◽  
Near Field ◽  
Terahertz Imaging ◽  
Imaging Systems ◽  
Near Field Imaging ◽  
Nonlinear Metamaterials ◽  
Terahertz Devices ◽  
Field Imaging ◽  
Sub Wavelength

This article reviews recent advances in terahertz science and technology that rely on confining the energy of incident terahertz radiation to small, very sub-wavelength sized regions. We focus on two broad areas of application for such field confinement: metamaterial-based nonlinear terahertz devices and terahertz near-field microscopy and spectroscopy techniques. In particular, we focus on field confinement in: terahertz nonlinear absorbers, metamaterial enhanced nonlinear terahertz spectroscopy, and in sub-wavelength terahertz imaging systems.

scholarly journals Piezoelectric Level Splitting in GaInN/GaN Quantum Wells

1998 ◽  
Vol 537 ◽  
Author(s):  
C. Wetzel ◽  
T. Takeuchi ◽  
H. Amano ◽  
I. Akasaki
Keyword(s):  
Quantum Wells ◽  
Electric Fields ◽  
High Performance ◽  
Stark Effect ◽  
Electronic Band Structure ◽  
Multiple Quantum Well ◽  
Multiple Quantum ◽  
Large Set ◽  
Electronic Band ◽  
Level Splitting

AbstractIdentification of the electronic band structure in AlInGaN heterostructures is the key issue in high performance light emitter and switching devices. In device-typical GaInN/GaN multiple quantum well samples in a large set of variable composition a clear correspondence of transitions in photo- and electroreflection, as well as photoluminescence is found. The effective band offset across the GaN/GaInN/GaN piezoelectric heterointerface is identified and electric fields from 0.23 - 0.90 MV/cm are directly derived. In the bias voltage dependence a level splitting within the well is observed accompanied by the quantum confined Stark effect. We furthermore find direct correspondence of luminescence bands with reflectance features. This indicates the dominating role of piezoelectric fields in the bandstructure of such typical strained layers.

scholarly journals Supramolecular Stark Effect in Host-Guest Complexes via Charge Density Analysis

2014 ◽  
Vol 70 (a1) ◽  
pp. C674-C674
Author(s):  
Sajesh Thomas ◽  
Rebecca Fuller ◽  
Alexandre Sobolev ◽  
Philip Schauer ◽  
Simon Grabowsky ◽  
...  
Keyword(s):  
Electric Field ◽  
Charge Density ◽  
Electric Fields ◽  
Active Sites ◽  
Stark Effect ◽  
Dipole Moments ◽  
Covalent Bonds ◽  
Guest Molecules ◽  
Density Mapping ◽  
Density Analysis

The effect of an electric field on the vibrational spectra, the Vibrational Stark Effect (VSE), has been utilized extensively to probe the local electric field in the active sites of enzymes [1, 2]. For this reason, the electric field and consequent polarization effects induced by a supramolecular host system upon its guest molecules attain special interest due to the implications for various biological processes. Although the host-guest chemistry of crown ether complexes and clathrates is of fundamental importance in supramolecular chemistry, many of these multicomponent systems have yet to be explored in detail using modern techniques [3]. In this direction, the electrostatic features associated with the host-guest interactions in the inclusion complexes of halogenated acetonitriles and formamide with 18-crown-6 host molecules have been analyzed in terms of their experimental charge density distribution. The charge density models provide estimates of the molecular dipole moment enhancements which correlate with the simulated values of dipole moments under electric field. The accurate electron density mapping using the multipole formalism also enable the estimation of the electric field experienced by the guest molecules. The electric field vectors thus obtained were utilized to estimate the vibrational stark effect in the nitrile (-C≡N) and carbonyl (C=O) stretching frequencies of the guest molecules via quantum chemical calculations in gas phase. The results of these calculations indicate remarkable elongation of C≡N and C=O bonds due to the electric fields. The electronic polarization in these covalent bonds induced by the field manifests as notable red shifts in their characteristic vibrational frequencies. These results derived from the charge densities are further supported by FT-IR experiments and thus establish the significance of a phenomenon that could be termed as the "supramolecular Stark effect" in crystal environment.

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