scholarly journals Characterizing decoherence rates of a superconducting qubit by direct microwave scattering

2021 ◽  
Vol 7 (1) ◽  
Author(s):  
Yong Lu ◽  
Andreas Bengtsson ◽  
Jonathan J. Burnett ◽  
Emely Wiegand ◽  
Baladitya Suri ◽  
...  
Keyword(s):  
Transmission Line ◽  
Radiative Decay ◽  
Incoherent Scattering ◽  
Decay Rates ◽  
Superconducting Qubit ◽  
Time Resolved ◽  
Microwave Scattering ◽  
Pure Dephasing ◽  
Order Of Magnitude ◽  
Dephasing Rate

AbstractWe experimentally investigate a superconducting qubit coupled to the end of an open transmission line, in a regime where the qubit decay rates to the transmission line and to its own environment are comparable. We perform measurements of coherent and incoherent scattering, on- and off-resonant fluorescence, and time-resolved dynamics to determine the decay and decoherence rates of the qubit. In particular, these measurements let us discriminate between non-radiative decay and pure dephasing. We combine and contrast results across all methods and find consistent values for the extracted rates. The results show that the pure dephasing rate is one order of magnitude smaller than the non-radiative decay rate for our qubit. Our results indicate a pathway to benchmark decoherence rates of superconducting qubits in a resonator-free setting.

scholarly journals Effect of the Substitution Position on the Electronic and Solvatochromic Properties of Isocyanoaminonaphthalene (ICAN) Fluorophores

Molecules ◽  
2019 ◽  
Vol 24 (13) ◽  
pp. 2434 ◽  
Author(s):  
Sándor Lajos Kovács ◽  
Miklós Nagy ◽  
Péter Pál Fehér ◽  
Miklós Zsuga ◽  
Sándor Kéki
Keyword(s):  
Radiative Decay ◽  
Fluorescence Emission ◽  
Solvent Polarity ◽  
Decay Rates ◽  
Quantum Yields ◽  
Time Resolved Fluorescence ◽  
Solvatochromic Shift ◽  
Fluorescence Emission Spectra ◽  
Time Resolved ◽  
Donor And Acceptor

The properties of 1,4-isocyanoaminonaphthalene (1,4-ICAN) and 2,6-isocyanoaminonaphthalene (2,6-ICAN) isomers are discussed in comparison with those of 1,5-isocyanoaminonaphthalene (1,5-ICAN), which exhibits a large positive solvatochromic shift similar to that of Prodan. In these isocyanoaminonaphthalene derivatives, the isocyano and the amine group serve as the donor and acceptor moieties, respectively. It was found that the positions of the donor and the acceptor groups in these naphthalene derivatives greatly influence the Stokes and solvatochromic shifts, which decrease in the following order: 1,5-ICAN > 2,6-ICAN > 1,4-ICAN. According to high-level quantum chemical calculations, this order is well correlated with the charge transfer character of these compounds upon excitation. Furthermore, unlike 1,5-ICAN, the 1,4-ICAN and 2,6-ICAN isomers showed relatively high quantum yields in water, that were determined to be 0.62 and 0.21, respectively. In addition, time-resolved fluorescence experiments revealed that both the radiative and non-radiative decay rates for these three ICAN isomers varied unusually with the solvent polarity parameter ET(30). The explanations of the influence of the solvent polarity on the resulting steady-state and time-resolved fluorescence emission spectra are also discussed.

scholarly journals Quantum efficiency, purity and stability of a tunable, narrowband microwave single-photon source

2021 ◽  
Vol 7 (1) ◽  
Author(s):  
Yong Lu ◽  
Andreas Bengtsson ◽  
Jonathan J. Burnett ◽  
Baladitya Suri ◽  
Sankar Raman Sathyamoorthy ◽  
...  
Keyword(s):  
Transmission Line ◽  
Quantum Efficiency ◽  
Radiative Decay ◽  
Single Photon ◽  
Photon Emission ◽  
Single Photons ◽  
Single Photon Source ◽  
Emission Channel ◽  
Pure Dephasing ◽  
Photon Source

AbstractWe demonstrate an on-demand source of microwave single photons with 71–99% intrinsic quantum efficiency. The source is narrowband (300 kHz) and tuneable over a 600 MHz range around 5.2 GHz. Such a device is an important element in numerous quantum technologies and applications. The device consists of a superconducting transmon qubit coupled to the open end of a transmission line. A π-pulse excites the qubit, which subsequently rapidly emits a single photon into the transmission line. A cancellation pulse then suppresses the reflected π-pulse by 33.5 dB, resulting in 0.005 photons leaking into the photon emission channel. We verify strong antibunching of the emitted photon field and determine its Wigner function. Non-radiative decay and 1/f flux noise both affect the quantum efficiency. We also study the device stability over time and identify uncorrelated discrete jumps of the pure dephasing rate at different qubit frequencies on a time scale of hours, which we attribute to independent two-level system defects in the device dielectrics, dispersively coupled to the qubit. Our single-photon source with only one input port is more compact and scalable compared to standard implementations.

scholarly journals Helmet Phthalocyaninato Iron Complex as a Primary Drier for Alkyd Paints

Materials ◽  
2021 ◽  
Vol 14 (5) ◽  
pp. 1220
Author(s):  
Jan Honzíček ◽  
Eliška Matušková ◽  
Štěpán Voneš ◽  
Jaromír Vinklárek
Keyword(s):  
Catalytic Performance ◽  
Mechanical Tests ◽  
Iron Complex ◽  
Kinetic Measurements ◽  
Time Resolved ◽  
Strong Activity ◽  
Vis Spectroscopy ◽  
Order Of Magnitude ◽  
Transparent Coatings ◽  
Time Resolved Infrared Spectroscopy

This study describes the catalytic performance of an iron(III) complex bearing a phthalocyaninato-like ligand in two solvent-borne and two high-solid alkyd binders. Standardized mechanical tests revealed strong activity, which appeared in particular cases at concentrations about one order of magnitude lower than in the case of cobalt(II) 2-ethylhexanoate, widespread used in paint-producing industry. The effect of the iron(III) compound on autoxidation process, responsible for alkyd curing, was quantified by kinetic measurements by time-resolved infrared spectroscopy and compared with several primary driers. Effect of the drier concentration on coloration of transparent coatings was determined by UV–Vis spectroscopy.

Radiative decay rates in LaF3:Dy3+

1979 ◽  
Vol 63 (1) ◽  
pp. 90-92 ◽  
Author(s):  
H. Jagannath ◽  
A. Sivaram ◽  
D. Ramachandra Rao ◽  
P. Venkateswarlu
Keyword(s):  
Radiative Decay ◽  
Decay Rates

SELF-TRAPPED EXCITONS IN ORTHORHOMBIC SnBr2

2001 ◽  
Vol 15 (28n30) ◽  
pp. 4009-4012 ◽  
Author(s):  
Y. YAMASAKI ◽  
N. OHNO
Keyword(s):  
Time Dependence ◽  
Low Temperatures ◽  
Luminescence Band ◽  
Radiative Decay ◽  
Time Resolved ◽  
Tunneling Recombination ◽  
Exciton Region ◽  
Time Resolved Photoluminescence ◽  
Stokes Shifts ◽  
2.5 Ev Luminescence

Luminescence properties of SnBr 2 have been studied to reveal the photo-excited exciton relaxation process. Two types of luminescence with large Stokes shifts are found at low temperatures; the 2.2-eV luminescence band produced under the photo-excitation in the first exciton region, and the 2.5-eV luminescence band stimulated by photons with energies above the bandgap. The time-resolved photoluminescence measurements have revealed that the 2.2-eV luminescence comprises fast (1.2 μs) and slow (6.4 μs) exponential decay components, whereas the 2.5-eV luminescence shows the time dependence of I(t)∞ t-0.9. These results suggest that the former band is attributed to the radiative decay of self-trapped excitons, and the latter band would originate from tunneling recombination of holes with the STEL as in the case of lead halides.

scholarly journals Experimental and theoretical radiative decay rates for highly excited ruthenium atomic levels and the solar abundance of ruthenium

2009 ◽  
Vol 396 (4) ◽  
pp. 2124-2132 ◽  
Author(s):  
V. Fivet ◽  
P. Quinet ◽  
P. Palmeri ◽  
É. Biémont ◽  
M. Asplund ◽  
...  
Keyword(s):  
Radiative Decay ◽  
Decay Rates ◽  
Solar Abundance

scholarly journals Radial diffusion modeling with empirical lifetimes: comparison with CRRES observations

2005 ◽  
Vol 23 (4) ◽  
pp. 1467-1471 ◽  
Author(s):  
Y. Y. Shprits ◽  
R. M. Thorne ◽  
G. D. Reeves ◽  
R. Friedel
Keyword(s):  
Diffusion Model ◽  
Radiation Effects ◽  
Outer Zone ◽  
Recovery Phase ◽  
Decay Rates ◽  
Radial Diffusion ◽  
Main Phase ◽  
Relativistic Electrons ◽  
Storm Main Phase ◽  
Order Of Magnitude

Abstract. A time dependent radial diffusion model is used to quantify the competing effects of inward radial diffusion and losses on the distribution of the outer zone relativistic electrons. The rate of radial diffusion is parameterized by Kp with the loss time as an adjustable parameter. Comparison with HEEF data taken over 500 Combined Release and Radiation Effects Satellite (CRRES) orbits indicates that 1-MeV electron lifetimes near the peak of the outer zone are less than a day during the storm main phase and few days under less disturbed conditions. These values are comparable to independent estimates of the storm time loss rate due to scattering by EMIC waves and chorus emission, and also provide an acceptable representation of electron decay rates following the storm time injection. Although our radial diffusion model, with data derived lifetimes, is able to simulate many features of the variability of outer zone fluxes and predicts fluxes within one order of magnitude accuracy for most of the storms and L values, it fails to reproduce the magnitude of flux changes and the gradual build up of fluxes observed during the recovery phase of many storms. To address these differences future modeling should include an additional local acceleration source and also attempt to simulate the pronounced loss of electrons during the main phase of certain storms.

High-energy X-ray diffuse scattering

2009 ◽  
Vol 42 (3) ◽  
pp. 392-400 ◽  
Author(s):  
I. B. Ramsteiner ◽  
A. Schöps ◽  
H. Reichert ◽  
H. Dosch ◽  
V. Honkimäki ◽  
...  
Keyword(s):  
Multiple Scattering ◽  
Diffuse Scattering ◽  
Binary Systems ◽  
High Energy ◽  
Absorption Length ◽  
Time Resolved ◽  
X Ray ◽  
Order Of Magnitude ◽  
Extinction Length ◽  
Scattering Volume

Diffuse X-ray scattering has been an important tool for understanding the atomic structure of binary systems for more than 50 years. The majority of studies have used laboratory-based sources providing 8 keV photons or synchrotron radiation with similar energies. Diffuse scattering is weak, with the scattering volume determined by the X-ray absorption length. In the case of 8 keV photons, this is not significantly different from the typical extinction length for Bragg scattering. If, however, one goes to energies of the order of 100 keV the scattering volume for the diffuse scattering increases up to three orders of magnitude while the extinction length increases by only one order of magnitude. This leads to a gain of two orders of magnitude in the relative intensity of the diffuse scattering compared with the Bragg peaks. This gain, combined with the possibility of recording the intensity from an entire plane in reciprocal space using a two-dimensional X-ray detector, permits time-resolved diffuse scattering studies in many systems. On the other hand, diffraction features that are usually neglected, such as multiple scattering, come into play. Four types of multiple scattering phenomena are discussed, and the manner in which they appear in high-energy diffraction experiments is considered.

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