Colocalization of Light Harvesting and Catalytic Units in ‘Soft’ Coordination Polymer Hydrogel toward Visible-Light Driven Photocatalytic Hydrogen Production

Author(s):  
Parul Verma ◽  
Ashish Singh ◽  
Faruk Ahamed Rahimi ◽  
Tapas Kumar Maji

Colocalization of essential molecular components in the solvated soft supramolecular assembly towards realizing visible-light-driven hydrogen evolution would be an exciting approach for sustainable energy by generating clean solar fuel. In...

2020 ◽  
Vol 8 (42) ◽  
pp. 21968-21972
Author(s):  
Debabrata Samanta ◽  
Manish Kumar ◽  
Sugandha Singh ◽  
Parul Verma ◽  
Kamal K. Kar ◽  
...  

A donor–acceptor coordination polymer (TPA-Zn) was synthesized by Zn(ii)-assisted self-assembly of an in situ generated triphenylamine (TPA) cored tristerpyridine ligand.


2014 ◽  
Vol 50 (14) ◽  
pp. 1731-1734 ◽  
Author(s):  
Zheng Wang ◽  
Jungang Hou ◽  
Chao Yang ◽  
Shuqiang Jiao ◽  
Hongmin Zhu

Three-dimensional MoS2–CdS–γ-TaON hollow nanostructures as novel photocatalysts were firstly synthesized via a facile hydrothermal method and they exhibit a high photocatalytic hydrogen production rate without a noble metal.


2017 ◽  
Vol 1 (3) ◽  
pp. 548-554 ◽  
Author(s):  
Xiangqing Li ◽  
Honglei Xu ◽  
Qiang Luo ◽  
Shizhao Kang ◽  
Lixia Qin ◽  
...  

The noble metal-free CuxNiy bimetallic nanoalloy decorated graphene nanohybrids (CuxNiy/G) exhibited a higher photocatalytic activity for hydrogen production. It provides a new and cheaper noble-metal-free graphene-based photocatalyst system for visible light-driven photocatalytic hydrogen evolution.


RSC Advances ◽  
2019 ◽  
Vol 9 (56) ◽  
pp. 32674-32682 ◽  
Author(s):  
Shanshan Li ◽  
Chun Hu ◽  
Yannan Peng ◽  
Zhihong Chen

Integration of a nanostructure design with a sub-bandgap enhances the photocatalytic H2 production activity of g-C3N4via facilitating separation of photogenerated charges while simultaneously increasing the active sites and light harvesting ability.


2020 ◽  
Vol 10 (15) ◽  
pp. 5298-5305
Author(s):  
Xuanxuan Yang ◽  
Yu Guo ◽  
Yongbing Lou ◽  
Jinxi Chen

The reaction mechanism of O-MoS2/Mn0.5Cd0.5S for photocatalytic hydrogen evolution is put forward and the satisfactory hydrogen production rate of the optimized composite is superior to most of the Mn–Cd–S based catalysts reported.


2021 ◽  
Author(s):  
Nageshwarrao Chanda ◽  
Koteshwar Devulapally ◽  
Spandana Gonuguntla ◽  
Sreedhar Bojja ◽  
Ujjwal Pal ◽  
...  

Here, we report the fine-tuned Donor-π-Acceptor concept based Zinc-porphyrin sensitized TiO2 photocatalyst for photochemical hydrogen evolution application. The newly designed system showed unprecedented photocatalytic activity. The molecular structure comprises of...


2018 ◽  
Vol 20 (23) ◽  
pp. 5266-5270 ◽  
Author(s):  
Jinfang Wang ◽  
Hongyu Mou ◽  
Rong Li ◽  
Yan Li ◽  
Debao Wang ◽  
...  

A solution processing strategy for V2VI3chalcogenides with a deep eutectic solvent for visible light photocatalytic hydrogen evolution is described here.


2017 ◽  
Vol 53 (68) ◽  
pp. 9430-9433 ◽  
Author(s):  
Ji-Tong Yin ◽  
Zhe Li ◽  
Yong Cai ◽  
Qian-Feng Zhang ◽  
Wei Chen

Ultrathin graphitic carbon nitride nanosheets with exceptional visible-light-driven photocatalytic hydrogen evolution efficiency are prepared via a facile secondary calcination approach.


RSC Advances ◽  
2015 ◽  
Vol 5 (83) ◽  
pp. 67742-67751 ◽  
Author(s):  
Felix Niefind ◽  
John Djamil ◽  
Wolfgang Bensch ◽  
Bikshandarkoil R. Srinivasan ◽  
Ilya Sinev ◽  
...  

An amorphous molybdenum sulfide based composite has been synthesized at room temperature applying a kinetically controlled reaction. The new material exhibits an extraordinary performance in the visible light driven hydrogen evolution reaction.


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