Molecular Design Opening Two Emission Pathways for High Efficiency and Long Lifetime in Thermally Activated Delayed Fluorescent Organic Light-Emitting Diodes

Author(s):  
Ha Lim Lee ◽  
Kyung Hyung Lee ◽  
Jun Yeob Lee ◽  
Ho Jung Lee

High efficiency and long lifetime thermally activated delayed fluorescent (TADF) organic light-emitting diodes (OLEDs) were developed using a novel molecular design with two emission pathways for high photoluminescence quantum yield...

2020 ◽  
Vol 8 (15) ◽  
pp. 5265-5272 ◽  
Author(s):  
Ji Han Kim ◽  
Kyung Hyung Lee ◽  
Jun Yeob Lee

Yellow thermally activated delayed fluorescence materials were synthesized using two types of acceptors of 2,4,6-triphenylpyrimidine-5-carbonitrile and 4-(3-cyanophenyl)-2,6-diphenylpyrimidine-5-carbonitrile combined with a strong donor.


Author(s):  
Shantaram Kothavale ◽  
Won Jae Chung ◽  
Jun Yeob Lee

Molecular design approach for the simultaneous achievement of high efficiency and long lifetime in the long wavelength region.


2021 ◽  
Vol 15 (3) ◽  
pp. 208-215 ◽  
Author(s):  
Soon Ok Jeon ◽  
Kyung Hyung Lee ◽  
Jong Soo Kim ◽  
Soo-Ghang Ihn ◽  
Yeon Sook Chung ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Maria Vasilopoulou ◽  
Abd. Rashid bin Mohd Yusoff ◽  
Matyas Daboczi ◽  
Julio Conforto ◽  
Anderson Emanuel Ximim Gavim ◽  
...  

AbstractBlue organic light-emitting diodes require high triplet interlayer materials, which induce large energetic barriers at the interfaces resulting in high device voltages and reduced efficiencies. Here, we alleviate this issue by designing a low triplet energy hole transporting interlayer with high mobility, combined with an interface exciplex that confines excitons at the emissive layer/electron transporting material interface. As a result, blue thermally activated delay fluorescent organic light-emitting diodes with a below-bandgap turn-on voltage of 2.5 V and an external quantum efficiency (EQE) of 41.2% were successfully fabricated. These devices also showed suppressed efficiency roll-off maintaining an EQE of 34.8% at 1000 cd m−2. Our approach paves the way for further progress through exploring alternative device engineering approaches instead of only focusing on the demanding synthesis of organic compounds with complex structures.


2019 ◽  
Vol 7 (40) ◽  
pp. 12695-12703 ◽  
Author(s):  
Ji Seon Jang ◽  
Ha Lim Lee ◽  
Kyung Hyung Lee ◽  
Jun Yeob Lee

Pyrimidine-5-carbonitrile was developed as an electrostatic potential managing and strong acceptor moiety of thermally activated delayed fluorescent (TADF) emitters for high efficiency and long lifetime in devices.


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