2013 ◽  
Vol 103 (21) ◽  
pp. 211116 ◽  
Author(s):  
Kevin D. Heylman ◽  
Randall H. Goldsmith

Author(s):  
Haiyong Quan ◽  
Zhixiong (James) Guo

Laser energy transfer and molecule-radiation interaction in optical microcavity devices are characterized. The device is operated at whispering-gallery modes, and consists of a microcavity and a micro-waveguide coupled by a sub-micrometer air-gap. Emphases are placed on the influences of microcavity size and waveguide compatibility on the energy transfer and storage capability, on the interactions of foreign molecules with the evanescent radiation field surrounding a resonant microcavity. An optimal gap is found for the considered device configuration where maximum energy storage is achieved. This optimal gap is dependent on the resonance mode as well as the morphology. The Q factor increases exponentially with increasing gap and saturates as the gap approaches the optical wavelength. The influence of molecules attachment is demonstrated and the potential in molecular detection is discussed.


2019 ◽  
Vol 16 (3) ◽  
pp. 211-219 ◽  
Author(s):  
Bernard Gelloz ◽  
Kouichiro Murata ◽  
Toshiyuki Ohta ◽  
Mher Ghulinyan ◽  
Lorenzo Pavesi ◽  
...  

Author(s):  
Qi-Fan Yang ◽  
Xu Yi ◽  
Ki Youl Yang ◽  
Kerry J. Vahala

Optik ◽  
2018 ◽  
Vol 165 ◽  
pp. 168-173 ◽  
Author(s):  
Francis Segovia-Chaves ◽  
Herbert Vinck-Posada

MRS Advances ◽  
2018 ◽  
Vol 3 (59) ◽  
pp. 3465-3470 ◽  
Author(s):  
Jonathan D B Van Schenck ◽  
Gregory Giesbers ◽  
Akash Kannegulla ◽  
Li-Jing Cheng ◽  
John E. Anthony ◽  
...  

AbstractPolarization-dependent absorption spectra of two functionalized derivatives of fluorinated anthradithiophene, diF TES-ADT and diF TDMS-ADT, were studied in the crystal phase using a Holstein-like Hamiltonian. For both molecules, the primary contribution to the lowest energy absorption was found to be the S0-S1 excitonic transition perturbed by an intermolecular coupling of 15 meV for both TES and TDMS. A secondary contribution, consistent with that from charge-transfer states, was also found. Additionally, absorption spectra were analysed when crystals were placed inside of optical microcavities formed by two metal mirrors. Cavities exhibited a primary absorption peak determined to be an enhanced absorption from the lowest-energy S0-S1 transition.


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