scholarly journals Source Apportionment with Site Specific Source Profiles

1991 ◽  
Vol 41 (3) ◽  
pp. 294-305 ◽  
Author(s):  
David M. Glover ◽  
Philip K. Hopke ◽  
Stephen J. Vermette ◽  
Sheldon Landsberger ◽  
Daniel R. D’Auben
2019 ◽  
Vol 12 (10) ◽  
pp. 5475-5501 ◽  
Author(s):  
Judith C. Chow ◽  
Junji Cao ◽  
L.-W. Antony Chen ◽  
Xiaoliang Wang ◽  
Qiyuan Wang ◽  
...  

Abstract. Smoke from laboratory chamber burning of peat fuels from Russia, Siberia, the USA (Alaska and Florida), and Malaysia representing boreal, temperate, subtropical, and tropical regions was sampled before and after passing through a potential-aerosol-mass oxidation flow reactor (PAM-OFR) to simulate intermediately aged (∼2 d) and well-aged (∼7 d) source profiles. Species abundances in PM2.5 between aged and fresh profiles varied by several orders of magnitude with two distinguishable clusters, centered around 0.1 % for reactive and ionic species and centered around 10 % for carbon. Organic carbon (OC) accounted for 58 %–85 % of PM2.5 mass in fresh profiles with low elemental carbon (EC) abundances (0.67 %–4.4 %). OC abundances decreased by 20 %–33 % for well-aged profiles, with reductions of 3 %–14 % for the volatile OC fractions (e.g., OC1 and OC2, thermally evolved at 140 and 280 ∘C). Ratios of organic matter (OM) to OC abundances increased by 12 %–19 % from intermediately aged to well-aged smoke. Ratios of ammonia (NH3) to PM2.5 decreased after intermediate aging. Well-aged NH4+ and NO3- abundances increased to 7 %–8 % of PM2.5 mass, associated with decreases in NH3, low-temperature OC, and levoglucosan abundances for Siberia, Alaska, and Everglades (Florida) peats. Elevated levoglucosan was found for Russian peats, accounting for 35 %–39 % and 20 %–25 % of PM2.5 mass for fresh and aged profiles, respectively. The water-soluble organic carbon (WSOC) fractions of PM2.5 were over 2-fold higher in fresh Russian peat (37.0±2.7 %) than in Malaysian (14.6±0.9 %) peat. While Russian peat OC emissions were largely water-soluble, Malaysian peat emissions were mostly water-insoluble, with WSOC ∕ OC ratios of 0.59–0.71 and 0.18–0.40, respectively. This study shows significant differences between fresh and aged peat combustion profiles among the four biomes that can be used to establish speciated emission inventories for atmospheric modeling and receptor model source apportionment. A sufficient aging time (∼7 d) is needed to allow gas-to-particle partitioning of semi-volatilized species, gas-phase oxidation, and particle volatilization to achieve representative source profiles for regional-scale source apportionment.


2018 ◽  
Vol 56 (2C) ◽  
pp. 88-95 ◽  
Author(s):  
Do Thi Nhu Ngoc

Volatile organic compounds (VOCs) are atmospheric pollutants of concern because of the health effect including carcinogenic risk of some of their species and the contribution in the formation of tropospheric ozone. The levels of VOCs in Hanoi were demonstrated to be higher than neighboring countries by previous research. The ozone potential formation (OFP) of VOCs was also some folds higher than others. Among transportation sources, VOCs were proved to be mainly emitted from motorbikes. The contribution percentages of transportation and other sources such as industrial, biomass burning sources are still remained unknown. In this research we applied chemical mass balance (CMB) receptor modelling to determine VOCs source apportionment. One week VOCs observation data at Hanoi University of Science and Technology in June 2017 was applied for investigation. Fourteen VOC species among 55 of which were applied for CMB modelling. Transportation and biomass burning source profiles were developed by monitoring in this study. Four other source profiles, namely gasoline evaporation, industrial production, cooking and paint that were compiled or calculated from previous studies. The results showed that the main sources of VOCs were vehicular emission, biomass burning, and gasoline evaporation contributing 37 %, 21 % and 20 % for VOCs levels, respectively. Other sources contributed for the leftover. The results can support to initiate policy for future control of VOCs.


Author(s):  
Anna Bokowa ◽  
Carlos Diaz ◽  
Jacek Koziel ◽  
Michael McGinley ◽  
Jennifer Barclay ◽  
...  

When it comes to air pollution complaints, odours are often the most significant contributor. Sources of odour emissions range from natural to anthropogenic. Mitigation of odour can be challenging, multifaceted, site-specific, and is often confounded by its complexity—defined by existing (or non-existing) environmental laws, public ordinances, and socio-economic considerations. The objective of this paper is to review and summarize odour legislation in selected European countries (France, Germany, Austria, Hungary, United Kingdom, Spain, The Netherlands, Italy, Belgium), North America (USA and Canada), South America (Chile and Colombia), as well as Oceania (Australia and New Zealand) and Asia (Japan, China). Many countries have incorporated odour controls into their legislation. However, odour-related assessment criteria tend to be highly variable between countries, individual states, provinces and even counties and towns. Legislation ranges from (1) no specific mention in environmental legislation that regulates pollutants which are known to have an odour impact to (2) extensive details about odour source testing, odour dispersion modeling, ambient odour monitoring, (3) setback distances, (4) process operations, and (5) odour control technologies and procedures. Agricultural operations are one specific source of odour emissions in rural and suburban areas and a model example of such complexities. Management of agricultural odour emissions is important because of the dense consolidation of animal feeding operations and the advance of housing development into rural areas. Overall, there is a need for continued survey, review, development, and adjustment of odour legislation that considers sustainable development, environmental stewardship, and socio-economic realities, all of which are amenable to a just, site-specific, and sector-specific application.


2015 ◽  
Vol 15 (4) ◽  
pp. 746-752 ◽  
Author(s):  
S. Six ◽  
T. Diez ◽  
B. Van Limbergen ◽  
L. Keustermans

Around 70% of the drinking water produced by De Watergroep (a Belgian public water company) is extracted from 83 groundwater pumping sites. To control the risks that endanger the drinking water supply and for the groundwater extracted to be as pure as possible, a risk-based approach for the protection of the catchment areas is developed, as part of the water safety plans. The approach consists of three steps: first, the compilation of a site-specific source file, second, the performance of a risk analysis for every catchment area, and third, the development of a monitoring strategy and action plans. The general goals are to lower the level of purification and to enhance the sustainability of groundwater extraction. The listed benefits make it worthwhile to implement this approach, despite the uncertainties.


2016 ◽  
Vol 219 ◽  
pp. 821-828 ◽  
Author(s):  
Tianqi Cai ◽  
James J. Schauer ◽  
Wei Huang ◽  
Dongqing Fang ◽  
Jing Shang ◽  
...  

Author(s):  
Ningning Zhang ◽  
Mazhan Zhuang ◽  
Jie Tian ◽  
Pengshan Tian ◽  
Jieru Zhang ◽  
...  

1999 ◽  
Vol 30 ◽  
pp. S455-S456
Author(s):  
Pen-Chi Chiang ◽  
Yu-Chun Chiang ◽  
Chu-Fang Wang ◽  
Sheng-Chi Chang

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