scholarly journals Investigation of the Phonon Spectra in CdSe/CdS Nanoplatelets by Raman Spectroscopy

2021 ◽  
Vol 2015 (1) ◽  
pp. 012076
Author(s):  
N.N. Kurus ◽  
A.G. Milekhin ◽  
R.B. Vasiliev ◽  
B.M. Saidzhonov ◽  
K.V. Anikin ◽  
...  

Abstract We report the phonon spectra of core/shell CdSe/CdS nanoplatelets with different shell thicknesses studied using Raman scattering. The nanoplatelets are rectangular colloidal nanocrystals, with thicknesses of core and shell layers of a few nanometers. The Raman spectra show features corresponding to the dominating longitudinal optical (LO) and surface optical (SO) phonon modes of the CdSe core in CdS shell located in the frequency regions of 200-210 and 250-290 cm-1, respectively. As the shell thickness increases, the phonon modes reveal a frequency shift and a change in intensity. The frequency shift associated with a change in the stress state in the core and shell, as well as with confinement effects is discussed. The phonon mode intensities are determined by the thickness of the shell and the proximity to resonant Raman scattering conditions.

2007 ◽  
Vol 21 (17) ◽  
pp. 2989-3000
Author(s):  
XIANG-FU ZHAO ◽  
CUI-HONG LIU

The scattering intensity (SI) for an electron resonant Raman scattering (ERRS) process in a free-standing semiconductor quantum wire of cylindrical geometry associated with bulk longitudinal optical (LO) phonon modes or the surface optical (SO) phonon modes is calculated for T=0 K . The Fröhlich interaction is considered to illustrate the theory for a GaAs system. Electron states are confined within a free-standing quantum wire (FSW). Single parabolic conduction and valence bands are assumed. The selection rules are studied. Numerical results and a discussion are also presented for various radii of the cylindrical quantum wires.


1997 ◽  
Vol 468 ◽  
Author(s):  
D. Behr ◽  
R. Niebuhr ◽  
H. Obloh ◽  
J. Wagner ◽  
K. H. Bachem ◽  
...  

ABSTRACTWe report on resonant Raman scattering in Al0.15Ga0.85N/GaN single quantum wells (QWs) and AlxGa1-xN/GaN/lnyGa1-yN heterostructures. By choosing appropriate excitation conditions we could probe selectively the GaN quantum well or the Al0.15Ga0.85N barrier of Al0.15Ga0.85N/GaN single quantum wells. For the InxGa1-xN material system a linear frequency shift of the E2- and A1(LO) phonon mode to lower frequencies was found with increasing In content. The shift was determined to -0.79cm-1 per % In content for the A,(LO) phonon frequency. Resonant excitation of AlxGa1-xN/GaN/InyGa1-YN heterostructures enabled us to detect phonon signals from the InxGa1-xN layer in the heterostructure and to determine its In content.


1990 ◽  
Vol 42 (17) ◽  
pp. 11325-11334 ◽  
Author(s):  
W. Limmer ◽  
H. Leiderer ◽  
K. Jakob ◽  
W. Gebhardt ◽  
W. Kauschke ◽  
...  

1973 ◽  
Vol 13 (2) ◽  
pp. 209-213 ◽  
Author(s):  
G.D. Holah ◽  
J.S. Webb ◽  
R.B. Dennis ◽  
C.R. Pidgeon

1977 ◽  
Vol 24 (9) ◽  
pp. 607-609 ◽  
Author(s):  
J. Windscheif ◽  
H. Stolz ◽  
W. von der Osten

2007 ◽  
Vol 1053 ◽  
Author(s):  
Stefan Werner ◽  
Patrick Zimmer ◽  
André Strittmatter ◽  
Axel Hoffmann

ABSTRACTThe carrier-phonon interaction in self-organized In(Ga)As/GaAs quantum dots is investigated under resonant excitation of the ground-state transition. Different phonon-coupled processes are observed. The distinction between Raman scattering and hot-luminescence process has been resolved by time-dependent photoluminescence measurements. The quantum dot LO (33.8 meV) as well as an interface (36.5 meV) phonon mode is observed by resonant Raman scattering. For the QD LO phonon mode, a very short radiative lifetime of 10 ps was found.


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