Scattering Processes with the Emission of Longitudinal Optical Phonons in the Landau Level System In GaAs/AlGaAs Quantum Well

The scattering processes of longitudinal optical phonons in GaAs/AlGaAs quantum wells in a quantizing magnetic field are considered. The time of intrasubband scattering between Landau levels is calculated by using Fermi's golden rule. The dependence of the scattering rate on the magnitude of the magnetic field has been shown and the magnetic field can suppress scattering processes on longitudinal optical phonons. It is found that the scattering time depends linearly on the width of the quantum well.

Silicene dynamic optical response in the presence of external electric and exchange fields

We investigate the dynamic optical transition of monolayer silicene in the presence of external electric and exchange fields within the low-energy tight-binding model. Applying external electric and exchange fields breaks the silicene band structure spin and valley degeneracies. Three phases of silicene corresponding to different strengths of perpendicular electric field with respect to the spin-orbit coupling (∆z < ∆so, ∆z = ∆so and ∆z > ∆so) are considered. We obtain the spinand valley-dependent optical responses to the incoming circularly polarized light using the Kubo formula. We show and discuss how the magnitude and direction of the transverse and longitudinal optical responses of such a system change with the electric and exchange fields. Our calculations suggest that the intraband part of the longitudinal optical response as well as the initial point of the interband part have strong dependencies on the exchange field. Furthermore, we show that one of the spin subbands plays a dominant role in the response to polarized light. Depending on the type of incident light polarization, the dominant subband may change. Our results shed light on the relation between silicene dynamic optical responses and externally applied fields.

Optical Pulling Using Chiral Metalens as a Photonic Probe

Optical pulling forces, which can pull objects in the source direction, have emerged as an intensively explored field in recent years. Conventionally, optical pulling forces exerted on objects can be achieved by tailoring the properties of an electromagnetic field, the surrounding environment, or the particles themselves. Recently, the idea of applying conventional lenses or prisms as photonic probes has been proposed to realize an optical pulling force. However, their sizes are far beyond the scope of optical manipulation. Here, we design a chiral metalens as the photonic probe to generate a robust optical pulling force. The induced pulling force exerted on the metalens, characterized by a broadband spectrum over 0.6 μm (from 1.517 to 2.117 μm) bandwidth, reached a maximum value of −83.76 pN/W. Moreover, under the illumination of incident light with different circular polarization states, the longitudinal optical force acting on the metalens showed a circular dichroism response. This means that the longitudinal optical force can be flexibly tuned from a pulling force to a pushing force by controlling the polarization of the incident light. This work could pave the way for a new advanced optical manipulation technique, with potential applications ranging from contactless wafer-scale fabrication to cell assembly and even course control for spacecraft.

Complex energies of the coherent longitudinal optical phonon–plasmon coupled mode according to dynamic mode decomposition analysis

In a dissipative quantum system, we report the dynamic mode decomposition (DMD) analysis of damped oscillation signals. We used a reflection-type pump-probe method to observe time-domain signals, including the coupled modes of long-lived longitudinal optical phonons and quickly damped plasmons (LOPC) at various pump powers. The Fourier transformed spectra of the observed damped oscillation signals show broad and asymmetric modes, making it difficult to evaluate their frequencies and damping rates. We then used DMD to analyze the damped oscillation signals by precisely determining their frequencies and damping rates. We successfully identified the LOPC modes. The obtained frequencies and damping rates were shown to depend on the pump power, which implies photoexcited carrier density. We compared the pump-power dependence of the frequencies and damping rates of the LOPC modes with the carrier density dependence of the complex eigen-energies of the coupled modes by using the non-Hermitian phenomenological effective Hamiltonian. Good agreement was obtained between the observed and calculated dependences, demonstrating that DMD is an effective alternative to Fourier analysis which often fails to estimate effective damping rates.

Mapping propagation of collective modes in Bi2Se3 and Bi2Te2.2Se0.8 topological insulators by near-field terahertz nanoscopy

Near-field microscopy discloses a peculiar potential to explore novel quantum state of matter at the nanoscale, providing an intriguing playground to investigate, locally, carrier dynamics or propagation of photoexcited modes as plasmons, phonons, plasmon-polaritons or phonon-polaritons. Here, we exploit a combination of hyperspectral time domain spectroscopy nano-imaging and detectorless scattering near-field optical microscopy, at multiple terahertz frequencies, to explore the rich physics of layered topological insulators as Bi2Se3 and Bi2Te2.2Se0.8, hyperbolic materials with topologically protected surface states. By mapping the near-field scattering signal from a set of thin flakes of Bi2Se3 and Bi2Te2.2Se0.8 of various thicknesses, we shed light on the nature of the collective modes dominating their optical response in the 2-3 THz range. We capture snapshots of the activation of transverse and longitudinal optical phonons and reveal the propagation of sub-diffractional hyperbolic phonon-polariton modes influenced by the Dirac plasmons arising from the topological surface states and of bulk plasmons, prospecting new research directions in plasmonics, tailored nanophotonics, spintronics and quantum technologies.

Investigation of the Phonon Spectra in CdSe/CdS Nanoplatelets by Raman Spectroscopy

We report the phonon spectra of core/shell CdSe/CdS nanoplatelets with different shell thicknesses studied using Raman scattering. The nanoplatelets are rectangular colloidal nanocrystals, with thicknesses of core and shell layers of a few nanometers. The Raman spectra show features corresponding to the dominating longitudinal optical (LO) and surface optical (SO) phonon modes of the CdSe core in CdS shell located in the frequency regions of 200-210 and 250-290 cm-1, respectively. As the shell thickness increases, the phonon modes reveal a frequency shift and a change in intensity. The frequency shift associated with a change in the stress state in the core and shell, as well as with confinement effects is discussed. The phonon mode intensities are determined by the thickness of the shell and the proximity to resonant Raman scattering conditions.

Spin photonics: from transverse spin to photonic skyrmions

Spin angular momentum associated with circular polarization is a fundamental and important aspect of photons both in classical and quantum optics. The interaction of this optical spin with matter and structures results in many intriguing optical effects and state-of-the-art applications covered under the emerging subject of spin optics. Distinct from longitudinal optical spin along the mean wavevector, transverse spin, the corresponding vector of which is perpendicular to the mean wavevector, prevails and plays a significant role in confined electromagnetic waves such as focused beams, guided waves, and evanescent waves. In the optical near-field, these transverse spins are generated owing to the spatial variation of the kinetic momentum of confined electromagnetic waves, where the spin and orbital angular momenta are strongly coupled, leading to many interesting topological spin structures and properties. Several reviews on optical transverse spins have been published in recent years in which their concepts and the various configurations producing them were introduced systematically. Here, we introduce in this review the underlying physics and dynamics of transverse spin and the resultant topological structures and properties such as the photonic skyrmions and merons. We term this sub-area ‘spin photonics’, its scope being to cover the design and research of spin structures in strongly confined electromagnetic fields with unique properties and applications. The concepts and framework reviewed have importance in optics, topological photonics, metrology, and quantum technologies and may be used to extend spin-dynamics concepts to fluidic, acoustic, and gravitational waves.