Formation of Soot in Ethylene-Air Partially Premixed Flames Over a Wide Range of Premixedness

Author(s):  
Aritra Chakraborty ◽  
Satya R. Chakravarthy

This paper reports an investigation of soot formation in ethylene-air partially premixed flames over a wide range of premixedness. An axisymmetric co-flow configuration is chosen to establish partially premixed flames from the fully non-premixed to fully premixed conditions. Reducing the fuel flow rate as a percentage of the maximum from the core stream and supplying the same to the annular stream leads to stratification of the reactant concentrations. The thermal power, overall equivalence ratio, and the average velocity in the both streams are maintained constant under all conditions. The soot volume fraction is estimated by light attenuation method, and laser induced incandescence is performed to map the soot distribution in the flow field. The soot volume fraction is observed to exhibit a ‘S’-type trend as the conditions are traversed from near the premixed to the non-premixed regimes. That is, when traversing from the non-premixed to near-premixed regime, below 60% fuel flow rate in core, the soot volume fraction drops drastically. The onset of sooting in the partially premixed flames is clearly seen to be at the tip of the rich-premixed flame branch of their triple flame structure, which advances upstream towards the base of the flame as the premixing is reduced. The ‘S’-type variation is clearly the effect of partial premixing, more specifically due to the presence of the lean premixed flame branch of the triple flame. Laser induced incandescence intensities are insufficient to capture the upstream advance of the soot onset with decreased premixedness. So, a quick and inexpensive technique to isolate soot luminescence through flame imaging is presented in the paper involving quasi-simultaneous imaging with a 650 nm and a BG-3 filter using a normal color camera.

2017 ◽  
Vol 139 (12) ◽  
Author(s):  
Aritra Chakraborty ◽  
Satya R. Chakravarthy

This paper reports an investigation of soot formation in ethylene–air partially premixed flames (PPFs) over a wide range of premixedness. An axisymmetric co-flow configuration is chosen to establish PPFs from the fully nonpremixed to fully premixed conditions. Reducing the fuel flow rate as a percentage of the maximum from the core stream and supplying the same to the annular stream leads to stratification of the reactant concentrations. The thermal power, overall equivalence ratio, and the average velocity in both the streams are maintained constant under all conditions. The soot volume fraction is estimated by light attenuation method, and laser-induced incandescence (LII) is performed to map the soot distribution in the flow field. The soot volume fraction is observed to exhibit an “S”-type trend as the conditions are traversed from near the premixed to the nonpremixed regimes. That is, when traversing from the nonpremixed to near-premixed regime, below 60% fuel flow rate in core, the soot volume fraction drops drastically. The onset of sooting in the PPFs is clearly seen to be at the tip of the rich-premixed flame (RPF) branch of their triple flame structure, which advances upstream toward the base of the flame as the premixing is reduced. The S-type variation is clearly the effect of partial premixing, more specifically due to the presence of the lean premixed flame (LPF) branch of the triple flame. LII intensities are insufficient to capture the upstream advance of the soot onset with decreased premixedness. So, a quick and inexpensive technique to isolate soot luminescence through flame imaging is presented in the paper involving quasi-simultaneous imaging with a 650 nm and a BG-3 filter using a normal color camera.


Author(s):  
H. Sapmaz ◽  
C. Ghenai

Laser-Induced Incandescence (LII) is used in this study to measure soot volume fractions in steady and flickering ethylene diffusion flames burning at atmospheric pressure. Better understanding of flickering flame behavior also promises to improve understanding of turbulent combustion systems. A very-high-speed solenoid valve is used to force the fuel flow rate with frequencies between 10 Hz and 200 Hz with the same mean fuel flow rate of steady flame. Periodic flame flickers are captured by two-dimensional phase-locked emission and LII images for eight phases (0°–360°) covering each period. LII spectra scan for minimizing C2 swan band emission and broadband molecular florescence, a calibration procedure using extinction measurements, and corrections for laser extinction and LII signal trapping are carried out towards developing reliable LII for quantitative applications. A comparison between the steady and pulsed flames results and the effect of the oscillation frequency on soot volume fraction for the pulsed flames are presented.


Author(s):  
H. Sapmaz ◽  
C. Ghenai

Laser-Induced Incandescence (LII) is used in this study to measure soot volume fractions in steady and flickering ethylene diffusion flames burning at atmospheric pressure. Better understanding of flickering flame behavior also promises to improve understanding of turbulent combustion systems. A very-high-speed solenoid valve is used to force the fuel flow rate with frequencies between 10 Hz and 200 Hz with the same mean fuel flow rate of steady flame. Periodic flame flickers are captured by two-dimensional phase-locked emission and LII images for eight phases (0° - 360°) covering each period. LII spectra scan for minimizing C2 swan band emission and broadband molecular florescence, a calibration procedure using extinction measurements, and corrections for laser extinction and LII signal trapping are carried out towards developing reliable LII for quantitative applications. A comparison between the steady and pulsed flames results and the effect of the oscillation frequency on soot volume fraction for the pulsed flames are presented.


Author(s):  
Andrew J. Lock ◽  
Alejandro Briones ◽  
Suresh K. Aggarwal ◽  
Ishwar K. Puri ◽  
Uday G. Hegde

The suppression of fires and flames is an important area of interest for both terrestrial and space based applications. In this investigation we elucidate the relative efficacy of fuel and air stream inert diluents for suppressing laminar partially premixed flames. A comparison of the effects of fuel and air stream dilution are also made with other fuels. Both counterflow and coflow flames are investigated, with both normal and zerogravity conditions considered for coflow flames. Simulations are conducted for both the counterflow and coflow flames, while experimental observations are made on the coflowing flames. With fuel or air stream dilution, coflow flames are observed to move downstream from the burner after overcoming initial heat transfer coupling. Further increases in diluent result in increases in the flame liftoff height until blow off occurs. The flame liftoff height and the critical volume fraction of extinguishing agent at blow out vary with both equivalence ratio and with the stream in which diluents are introduced. Nonpremixed methane-air flames are more difficult to extinguish than partially premixed flames with fuel stream dilution; whereas, partially premixed methane-air flames are more resistant to extinction than nonpremixed flames with air stream dilution. This difference in efficacy of the fuel and air stream dilution is attributed to the action of the diluent. In leaner partially premixed flames with fuel stream dilution and richer partially premixed flames with air stream dilution the effect of the diluent is to replace the deficient reactant in the system, thus starving the flame. In leaner partially premixed flames with air stream dilution and richer partially premixed flames with fuel stream dilution the effect of the diluent is purely thermal in that it absorbs heat from the flame, until combustion may no longer be sustained. The dilution effect is more effective than the thermal effect. When gravity is eliminated from the 2-D flame the liftoff height decreases and the critical volume fraction of diluent for blow off is also decreased.


Author(s):  
Fengshan Liu ◽  
Kevin A. Thomson ◽  
Gregory J. Smallwood

Investigation of the effect of oxygen addition to fuel on the visible flame appearance and soot formation characteristics of laminar diffusion flames is important to gain comprehensive understanding of gas-phase combustion chemistry and its interaction with soot chemistry. This paper reports experimental results of oxygen addition to fuel on the visible flame height and soot volume fraction distributions in axisymmetric coflow laminar ethylene and propane diffusion flames at atmospheric flames. The carbon flow rate was maintained constant in all the experiments. Although many experimental studies have been conducted in the literature in this topic, the present investigation aimed at providing spatially resolved soot volume fraction distributions over the entire range of oxygen addition from no oxygen addition up to the point of flashback while keeping the carbon mass flow rate constant. The level of oxygen added to fuel right before flashback is about 45% (the percentage of oxygen addition is always by volume in this study) of the fuel flow rate in the ethylene flame and 300% of the fuel flow rate in the propane flame. As the added oxygen amount to ethylene increases, the visible flame height first increases. When the added oxygen flow rate is about 13% of the fuel flow rate, the flame becomes smoking, i.e., soot escapes from the flame tip. When the oxygen flow rate reaches about 42% of the fuel flow rate, the flame stops smoking. When oxygen was added to propane, the visible flame height linearly decreases with increasing the amount of oxygen. These very different effects of oxygen addition to ethylene and propane indicate that oxygen plays a drastically different role in the chemical pathways leading to soot formation in ethylene and propane flames. Distributions of soot volume fractions in these flames were measured using a 2D light attenuation technique coupled with the Abel inversion. The present study provides valuable experimental data for validating soot models.


2020 ◽  
Vol 126 (12) ◽  
Author(s):  
Manu Mannazhi ◽  
Per-Erik Bengtsson

AbstractTwo-dimensional laser-induced incandescence (LII) measurements usually involve the use of a cylindrical lens to illuminate the planar region of interest. This creates a varying laser fluence and sheet width in the imaged flame region which could lead to large uncertainties in the quantification of the 2D LII signals into soot volume fraction distributions. To investigate these effects, 2D LII measurements using a wide range of laser pulse energies were performed on a premixed flat ethylene–air flame while employing a cylindrical lens to focus the laser sheet. Using shorter focal length of the focusing lens resulted in larger variation of the LII signal profiles across the flame. A heat – and – mass – transfer - based LII model was also used to simulate the measurements and good agreement was found. The ratio between focal length (FL) and image length (IL) was introduced as a useful parameter for estimating the bias in estimated soot volume fractions across the flame. The general recommendation is to maximize this FL/IL ratio in an experiment, which in practice means the use of a long focal length lens. Furthermore, the best choices of laser fluence and detection gate width are discussed based on results from these simulations.


2003 ◽  
Author(s):  
H. Sapmaz ◽  
C. X. Lin ◽  
M. A. Ebadian ◽  
C. Ghenai

Laser-Induced Incandescence (LII) is used in this study to measure the soot volume fraction for steady and unsteady laminar ethylene diffusion flames. For the steady flame the soot profiles obtained in this study using LII showed good agreement with those obtained previously using scattering/extinction technique. For the unsteady or flickering flames, we generated very repeatable time-varying diffusion flames by forcing the fuel flow at frequencies between 1–10 Hz. Phase lock images of the soot volume fractions were obtained for different phases between 0° and 360°. The sequential images showed the dynamics of the interactions between the generated vortices in the fuel and the flame. The phase-locked soot images revealed the entire motion process of the soot field during each pulsation period. The results obtained in the course of this study show that the soot emission decreased by lowering the oscillation frequency of the flame.


AIAA Journal ◽  
2002 ◽  
Vol 40 (11) ◽  
pp. 2289-2297 ◽  
Author(s):  
Hongshe Xue ◽  
Suresh K. Aggarwal

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