Soot Particle Measurements in Steady and Unsteady Laminar Diffusion Flames Using Laser-Induced Incandescence

2003 ◽  
Author(s):  
H. Sapmaz ◽  
C. X. Lin ◽  
M. A. Ebadian ◽  
C. Ghenai
Keyword(s):  
Soot Particle ◽  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Volume Fraction ◽  
Pulsation Period ◽  
Laminar Diffusion Flames ◽  
Fuel Flow ◽  
Laser Induced Incandescence ◽  
Sequential Images ◽  
Good Agreement

Laser-Induced Incandescence (LII) is used in this study to measure the soot volume fraction for steady and unsteady laminar ethylene diffusion flames. For the steady flame the soot profiles obtained in this study using LII showed good agreement with those obtained previously using scattering/extinction technique. For the unsteady or flickering flames, we generated very repeatable time-varying diffusion flames by forcing the fuel flow at frequencies between 1–10 Hz. Phase lock images of the soot volume fractions were obtained for different phases between 0° and 360°. The sequential images showed the dynamics of the interactions between the generated vortices in the fuel and the flame. The phase-locked soot images revealed the entire motion process of the soot field during each pulsation period. The results obtained in the course of this study show that the soot emission decreased by lowering the oscillation frequency of the flame.

Two-Dimensional Imaging of Soot Volume Fraction in Pulsed Diffusion Flames by Laser-Induced Incandescence

2006 ◽  
Author(s):  
H. Sapmaz ◽  
C. Ghenai
Keyword(s):  
Flow Rate ◽  
High Speed ◽  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Volume Fraction ◽  
Two Dimensional ◽  
Fuel Flow Rate ◽  
Fuel Flow ◽  
Laser Induced Incandescence ◽  
Pulsed Flames

Laser-Induced Incandescence (LII) is used in this study to measure soot volume fractions in steady and flickering ethylene diffusion flames burning at atmospheric pressure. Better understanding of flickering flame behavior also promises to improve understanding of turbulent combustion systems. A very-high-speed solenoid valve is used to force the fuel flow rate with frequencies between 10 Hz and 200 Hz with the same mean fuel flow rate of steady flame. Periodic flame flickers are captured by two-dimensional phase-locked emission and LII images for eight phases (0°–360°) covering each period. LII spectra scan for minimizing C2 swan band emission and broadband molecular florescence, a calibration procedure using extinction measurements, and corrections for laser extinction and LII signal trapping are carried out towards developing reliable LII for quantitative applications. A comparison between the steady and pulsed flames results and the effect of the oscillation frequency on soot volume fraction for the pulsed flames are presented.

Measurements of Soot Volume Fraction in Pulsed Diffusion Flames by Laser-Induced Incandescence

2006 ◽  
Author(s):  
H. Sapmaz ◽  
C. Ghenai
Keyword(s):  
Flow Rate ◽  
High Speed ◽  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Volume Fraction ◽  
Calibration Procedure ◽  
Fuel Flow Rate ◽  
Fuel Flow ◽  
Laser Induced Incandescence ◽  
Pulsed Flames

Laser-Induced Incandescence (LII) is used in this study to measure soot volume fractions in steady and flickering ethylene diffusion flames burning at atmospheric pressure. Better understanding of flickering flame behavior also promises to improve understanding of turbulent combustion systems. A very-high-speed solenoid valve is used to force the fuel flow rate with frequencies between 10 Hz and 200 Hz with the same mean fuel flow rate of steady flame. Periodic flame flickers are captured by two-dimensional phase-locked emission and LII images for eight phases (0° - 360°) covering each period. LII spectra scan for minimizing C2 swan band emission and broadband molecular florescence, a calibration procedure using extinction measurements, and corrections for laser extinction and LII signal trapping are carried out towards developing reliable LII for quantitative applications. A comparison between the steady and pulsed flames results and the effect of the oscillation frequency on soot volume fraction for the pulsed flames are presented.

scholarly journals The influence of aliphatics on soot inception modelling

2021 ◽  
Author(s):  
Nemanja Ceranic
Keyword(s):  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Formation ◽  
Fluid Dynamic ◽  
Soot Volume Fraction ◽  
Surface Reactivity ◽  
Complex Nature ◽  
Laminar Diffusion Flames ◽  
Laminar Diffusion ◽  
Polycyclic Aromatic

Soot models have been investigated for several decades and many fundamental models exist that prescribe soot formation in agreement with experiments and theories. However, due to the complex nature of soot formation, not all pathways have been fully characterized. This work has numerically studied the influence that aliphatic based inception models have on soot formation for coflow laminar diffusion flames. CoFlame is the in-house parallelized FORTRAN code that was used to conduct this research. It solves the combustion fluid dynamic conservation equations for a variety of coflow laminar diffusion flames. New soot inception models have been developed for specific aliphatics in conjunction with polycyclic aromatic hydrocarbon based inception. The purpose of these models was not to be completely fundamental in nature, but more so a proof-of-concept in that an aliphatic based mechanism could account for soot formation deficiencies that exist with just PAH based inception. The aliphatic based inception models show potential to enhance predicative capability by increasing the prediction of the soot volume fraction along the centerline without degrading the prediction along the pathline of maximum soot. Additionally, the surface reactivity that was used to achieve these results lied closer in the range of numerically derived optimal values as compared to the surface reactivity that was needed to match peak soot concentrations without the aliphatic based inception models.

scholarly journals A Numerical Investigation on Soot Formation From Laminar Diffusion Flames of Ethylene/Methane Mixture

2008 ◽  
Author(s):  
Hongsheng Guo ◽  
Stephanie Trottier ◽  
Matthew R. Johnson ◽  
Gregory J. Smallwood
Keyword(s):  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Formation ◽  
Soot Volume Fraction ◽  
Fuel Mixture ◽  
Methyl Radical ◽  
Laminar Diffusion Flames ◽  
Laminar Diffusion ◽  
Methane Mixture ◽  
Phase Chemistry

The sooting propensity of laminar diffusion flames employing ethylene/methane mixture fuel is investigated by numerical simulation. Detailed gas phase chemistry and moments method are used to describe the chemical reaction process and soot particle dynamics, respectively. The numerical model captures the primary features experimentally observed previously. At constant temperatures of air and fuel mixture, both maximum soot volume fraction and soot yield monotonically decrease with increasing the fraction of carbon from methane in the fuel mixture. However, when the temperatures of air and fuel mixture are preheated so that the adiabatic temperatures of all flames are same, the variation of the maximum soot yield becomes higher than what would be expected from a linear combination of the flames of pure ethylene and pure methane, showing a synergistic phenomenon in soot formation. Further analysis of the details of the numerical results suggests that the synergistic phenomenon is caused by the combined effects of the variations in the concentrations of acetylene (C2H2) and methyl radical (CH3). When the fraction of carbon from methane in fuel mixture increases, the concentration of C2H2 monotonically decreases, whereas that of methyl radical increases, resulting in a synergistic phenomenon in the variation of propargyl (C3H3) radical concentration due to the reactions C2H2 + CH3 = PC3H4 + H and PC3H4 + H = C3H3 + H2. This synergistic phenomenon causes a qualitatively similar variation trend in the concentration of pyrene (A4) owing to the reaction paths C3H3 → A1 (benzene) → A2 (naphthalene) → A3 (phenanthrene) → A4. Consequently, the synergistic effect occurs for soot inception and PAH condensation rates, leading to the synergistic phenomenon in soot yield. The similar synergistic phenomenon is not observed in the variation of peak soot volume fraction, since the maximum surface growth rate monotonically decreases, as the fraction of carbon from methane in fuel mixture increases.

Formation of Soot in Ethylene-Air Partially Premixed Flames Over a Wide Range of Premixedness

2017 ◽  
Author(s):  
Aritra Chakraborty ◽  
Satya R. Chakravarthy
Keyword(s):  
Volume Fraction ◽  
Premixed Flames ◽  
Soot Volume Fraction ◽  
Premixed Flame ◽  
Fuel Flow Rate ◽  
Fuel Flow ◽  
Wide Range ◽  
Partially Premixed Flames ◽  
Laser Induced Incandescence ◽  
Partially Premixed

This paper reports an investigation of soot formation in ethylene-air partially premixed flames over a wide range of premixedness. An axisymmetric co-flow configuration is chosen to establish partially premixed flames from the fully non-premixed to fully premixed conditions. Reducing the fuel flow rate as a percentage of the maximum from the core stream and supplying the same to the annular stream leads to stratification of the reactant concentrations. The thermal power, overall equivalence ratio, and the average velocity in the both streams are maintained constant under all conditions. The soot volume fraction is estimated by light attenuation method, and laser induced incandescence is performed to map the soot distribution in the flow field. The soot volume fraction is observed to exhibit a ‘S’-type trend as the conditions are traversed from near the premixed to the non-premixed regimes. That is, when traversing from the non-premixed to near-premixed regime, below 60% fuel flow rate in core, the soot volume fraction drops drastically. The onset of sooting in the partially premixed flames is clearly seen to be at the tip of the rich-premixed flame branch of their triple flame structure, which advances upstream towards the base of the flame as the premixing is reduced. The ‘S’-type variation is clearly the effect of partial premixing, more specifically due to the presence of the lean premixed flame branch of the triple flame. Laser induced incandescence intensities are insufficient to capture the upstream advance of the soot onset with decreased premixedness. So, a quick and inexpensive technique to isolate soot luminescence through flame imaging is presented in the paper involving quasi-simultaneous imaging with a 650 nm and a BG-3 filter using a normal color camera.

scholarly journals Experimental Investigation of Oxygen Addition to Fuel on Soot Formation in Laminar Coflow Diffusion Flames of Ethylene and Propane

2006 ◽  
Author(s):  
Fengshan Liu ◽  
Kevin A. Thomson ◽  
Gregory J. Smallwood
Keyword(s):  
Flow Rate ◽  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Formation ◽  
Soot Volume Fraction ◽  
Oxygen Flow Rate ◽  
Flame Height ◽  
Fuel Flow Rate ◽  
Fuel Flow ◽  
Oxygen Addition

Investigation of the effect of oxygen addition to fuel on the visible flame appearance and soot formation characteristics of laminar diffusion flames is important to gain comprehensive understanding of gas-phase combustion chemistry and its interaction with soot chemistry. This paper reports experimental results of oxygen addition to fuel on the visible flame height and soot volume fraction distributions in axisymmetric coflow laminar ethylene and propane diffusion flames at atmospheric flames. The carbon flow rate was maintained constant in all the experiments. Although many experimental studies have been conducted in the literature in this topic, the present investigation aimed at providing spatially resolved soot volume fraction distributions over the entire range of oxygen addition from no oxygen addition up to the point of flashback while keeping the carbon mass flow rate constant. The level of oxygen added to fuel right before flashback is about 45% (the percentage of oxygen addition is always by volume in this study) of the fuel flow rate in the ethylene flame and 300% of the fuel flow rate in the propane flame. As the added oxygen amount to ethylene increases, the visible flame height first increases. When the added oxygen flow rate is about 13% of the fuel flow rate, the flame becomes smoking, i.e., soot escapes from the flame tip. When the oxygen flow rate reaches about 42% of the fuel flow rate, the flame stops smoking. When oxygen was added to propane, the visible flame height linearly decreases with increasing the amount of oxygen. These very different effects of oxygen addition to ethylene and propane indicate that oxygen plays a drastically different role in the chemical pathways leading to soot formation in ethylene and propane flames. Distributions of soot volume fractions in these flames were measured using a 2D light attenuation technique coupled with the Abel inversion. The present study provides valuable experimental data for validating soot models.

scholarly journals Experimental Study of Soot Volume Fraction Applied in Laminar Diffusion Flames

2013 ◽  
Vol 03 (04) ◽  
pp. 137-141 ◽  
Author(s):  
N. R. Caetano ◽  
F. M. Pereira ◽  
H. A. Vielmo ◽  
F. T. van der Lann
Keyword(s):  
Experimental Study ◽  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Volume Fraction ◽  
Laminar Diffusion Flames ◽  
Laminar Diffusion

scholarly journals The influence of aliphatics on soot inception modelling

2021 ◽  
Author(s):  
Nemanja Ceranic
Keyword(s):  
Volume Fraction ◽  
Diffusion Flames ◽  
Soot Formation ◽  
Fluid Dynamic ◽  
Soot Volume Fraction ◽  
Surface Reactivity ◽  
Complex Nature ◽  
Laminar Diffusion Flames ◽  
Laminar Diffusion ◽  
Polycyclic Aromatic

Soot models have been investigated for several decades and many fundamental models exist that prescribe soot formation in agreement with experiments and theories. However, due to the complex nature of soot formation, not all pathways have been fully characterized. This work has numerically studied the influence that aliphatic based inception models have on soot formation for coflow laminar diffusion flames. CoFlame is the in-house parallelized FORTRAN code that was used to conduct this research. It solves the combustion fluid dynamic conservation equations for a variety of coflow laminar diffusion flames. New soot inception models have been developed for specific aliphatics in conjunction with polycyclic aromatic hydrocarbon based inception. The purpose of these models was not to be completely fundamental in nature, but more so a proof-of-concept in that an aliphatic based mechanism could account for soot formation deficiencies that exist with just PAH based inception. The aliphatic based inception models show potential to enhance predicative capability by increasing the prediction of the soot volume fraction along the centerline without degrading the prediction along the pathline of maximum soot. Additionally, the surface reactivity that was used to achieve these results lied closer in the range of numerically derived optimal values as compared to the surface reactivity that was needed to match peak soot concentrations without the aliphatic based inception models.

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