Prediction of Packed Catalyst Bed Stress and Load for Radial Flow Reactors

Author(s):  
Mingxin Zhao ◽  
Pedro Vargas

For the radial flow reactor with a packed catalyst bed, the pressure drop in radial direction will affect bed support stress and load condition significantly. Increased fines due to catalyst attrition during operation will increase the radial pressure drop. For an extreme case, the entire catalyst bed could be pushed inward and pinned to the reactor’s perforated center screen, potentially causing the internal components to be overly stressed by the excessive load. Understanding the impact of radial pressure drop to bed stress and load distribution is very important for reactor internals design and operation. In this study, a generic packed catalyst bed for a radial flow reactor is analytically modeled and examined for stress and load by a classical granular solid material model, i.e., Janssen’s theory, which is further modified to include the pressure drop effects for a radial flow reactor. Interactions between bed stress, load, and radial pressure drop are explored. The critical condition is derived.

Author(s):  
David Zhao ◽  
Mingxin Zhao

Abstract Pressure drop in a radial flow reactor occurs when process flow crosses the packed catalyst bed installed between the two concentric perforated screens during operation. This pressure drop generates the lateral bed stress against the reactor’s perforated screens to shift. The pressure drop will further grow as catalyst attrition increases in production. For an outward radial flow, the pressure drop may exert higher stresses to the outer screen as the packed bed is pushed toward it. An extreme case is when the entire catalyst bed could be pinned to the outer screen of the reactor by enough pressure drop. This could cause the internal components to be overly stressed on the excessive bed load, for which the components might not have been designed adequately. Predicting how radial pressure drop impacts the bed stress and shifts the load distribution is important in preventing mechanical failure during operation. In this study, an analytical model is derived based on Janssen’s theory, a classical semi-empirical granular solid material model, to examine a generic packed catalyst bed in an outward radical flow reactor. A modification to Janssen’s theory is introduced to include pressure drop in order to explore its effects on bed stress and load. The critical condition is derived.


2020 ◽  
Vol 10 (3) ◽  
pp. 1080 ◽  
Author(s):  
Qian Yu ◽  
Wim Brilman

Direct air capture (DAC) of CO2 can address CO2 emissions from distributed sources and produce CO2 from air virtually anywhere that it is needed. In this paper, the performance of a new radial flow reactor (RFR) for CO2 adsorption from ambient air is reported. The reactor uses a supported amine sorbent and is operated in a batch mode of operation or semi-continuously, respectively without or with sorbent circulation. The radial flow reactor, containing 2 kg of the adsorbent, is successfully scaled up from the experimental results obtained with a fixed bed reactor using only 1 g of the adsorbent. In the batch operation mode, the sorbent in the annular space of the RFR is regenerated in situ. With sorbent circulation, the RFR is loaded and unloaded batchwise and only used as an adsorber. A sorbent batch loaded with CO2 is transported to and regenerated in an external (fluid bed) regenerator. The RFR unit is characterized by a low contacting energy (0.7–1.5 GJ/ton-CO2) and a relatively short adsorption time (24–43 min) compared to other DAC processes using the same types of sorbents. The contactor concept is ready for further scale-up and continuous application.


AIChE Journal ◽  
1987 ◽  
Vol 33 (10) ◽  
pp. 1747-1750 ◽  
Author(s):  
A. L. López de Ramos ◽  
F. F. Pironti

AIChE Journal ◽  
2002 ◽  
Vol 48 (3) ◽  
pp. 617-624 ◽  
Author(s):  
B. Marwaha ◽  
D. Luss

1990 ◽  
Vol 45 (8) ◽  
pp. 2169-2176 ◽  
Author(s):  
D. Suter ◽  
A. Bartroli ◽  
F. Schneider ◽  
D.W.T. Rippin ◽  
E.J. Newson

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