scholarly journals A Radial Flow Contactor for Ambient Air CO2 Capture

2020 ◽  
Vol 10 (3) ◽  
pp. 1080 ◽  
Author(s):  
Qian Yu ◽  
Wim Brilman

Direct air capture (DAC) of CO2 can address CO2 emissions from distributed sources and produce CO2 from air virtually anywhere that it is needed. In this paper, the performance of a new radial flow reactor (RFR) for CO2 adsorption from ambient air is reported. The reactor uses a supported amine sorbent and is operated in a batch mode of operation or semi-continuously, respectively without or with sorbent circulation. The radial flow reactor, containing 2 kg of the adsorbent, is successfully scaled up from the experimental results obtained with a fixed bed reactor using only 1 g of the adsorbent. In the batch operation mode, the sorbent in the annular space of the RFR is regenerated in situ. With sorbent circulation, the RFR is loaded and unloaded batchwise and only used as an adsorber. A sorbent batch loaded with CO2 is transported to and regenerated in an external (fluid bed) regenerator. The RFR unit is characterized by a low contacting energy (0.7–1.5 GJ/ton-CO2) and a relatively short adsorption time (24–43 min) compared to other DAC processes using the same types of sorbents. The contactor concept is ready for further scale-up and continuous application.

2017 ◽  
Vol 11 (1) ◽  
pp. 16-25 ◽  
Author(s):  
Rebecca Faschian ◽  
Ilyas Eren ◽  
Steven Minden ◽  
Ralf Pörtner

Fixed-bed processes, where cells are immobilized within macroporous carriers, are a promising alternative to processes with suspended cells. A scale-up concept is presented in order to evaluate the performance as part of process design of fixed-bed processes. Therefore,Lactococcus lactiscultivation in chemostat and batch mode was compared to fixed bed cultures on three different scales, the smallest being the downscaledMultifermwith 10 mL fixed bed units, the second a 100 mL fixed-bed reactor and the third a pilot scale reactor with 1 L fixed bed volume. As expected, the volume specific lactate productivity of all cultivations was dependent on dilution rate. In suspension chemostat culture a maximum of 2.3 g·L-1·h-1was reached. Due to cell retention in the fixed-beds, productivity increased up to 8.29 g·L-1·h-1at a dilution rate of D = 1.16 h-1(corresponding to 2.4·µmax) on pilot scale. For all fixed bed cultures a common spline was obtained indicating a good scale-up performance.


1985 ◽  
Vol 50 (10) ◽  
pp. 2122-2133 ◽  
Author(s):  
Jindřich Zahradník ◽  
Marie Fialová ◽  
Jan Škoda ◽  
Helena Škodová

An experimental study was carried out aimed at establishing a data base for an optimum design of a continuous flow fixed-bed reactor for biotransformation of ammonium fumarate to L-aspartic acid catalyzed by immobilized cells of the strain Escherichia alcalescens dispar group. The experimental program included studies of the effect of reactor geometry, catalytic particle size, and packed bed arrangement on reactor hydrodynamics and on the rate of substrate conversion. An expression for the effective reaction rate was derived including the effect of mass transfer and conditions of the safe conversion-data scale-up were defined. Suggestions for the design of a pilot plant reactor (100 t/year) were formulated and decisive design parameters of such reactor were estimated for several variants of problem formulation.


2013 ◽  
Vol 11 (1) ◽  
pp. 19-30 ◽  
Author(s):  
Xingxing Cheng ◽  
Xiaotao T. Bi

Abstract A NOx adsorption kinetic model including NO oxidation and adsorption was developed. The NOx and O2 adsorption experimental data from a fixed bed were found to be fitted well to the Freundlich type isotherm. An axial dispersion adsorption model was then developed to simulate the breakthrough curve for NOx adsorption in the fixed bed. The model parameters including mass transfer coefficient and axial dispersion coefficient were fitted from the NOx breakthrough curves measured in a fixed bed. This model can be used for design and scale-up of fixed bed NOx adsorption columns. It can also be extended for the modeling of NOx adsorption in the annulus region of the circulating fluidized bed reactor for catalytic reduction of NOx.


AIChE Journal ◽  
1987 ◽  
Vol 33 (10) ◽  
pp. 1747-1750 ◽  
Author(s):  
A. L. López de Ramos ◽  
F. F. Pironti

2008 ◽  
Vol 17 (1) ◽  
pp. 59-63 ◽  
Author(s):  
Haitao Liu ◽  
Xiaolai Wang ◽  
Dexin Yang ◽  
Runxiong Gao ◽  
Zhonglai Wang ◽  
...  

AIChE Journal ◽  
2002 ◽  
Vol 48 (3) ◽  
pp. 617-624 ◽  
Author(s):  
B. Marwaha ◽  
D. Luss

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