scholarly journals Contributions of Clouds, Surface Albedos, and Mixed-Phase Ice Nucleation Schemes to Arctic Radiation Biases in CAM5

2014 ◽  
Vol 27 (13) ◽  
pp. 5174-5197 ◽  
Author(s):  
Jason M. English ◽  
Jennifer E. Kay ◽  
Andrew Gettelman ◽  
Xiaohong Liu ◽  
Yong Wang ◽  
...  
Keyword(s):  
Radiant Energy ◽  
Cloud Amount ◽  
Ice Nucleation ◽  
Radiative Flux ◽  
Mixed Phase ◽  
Surface Radiation ◽  
Nucleation Theory ◽  
The Arctic ◽  
Radiation Balance ◽  
Ice Nuclei

The Arctic radiation balance is strongly affected by clouds and surface albedo. Prior work has identified Arctic cloud liquid water path (LWP) and surface radiative flux biases in the Community Atmosphere Model, version 5 (CAM5), and reductions to these biases with improved mixed-phase ice nucleation schemes. Here, CAM5 net top-of-atmosphere (TOA) Arctic radiative flux biases are quantified along with the contributions of clouds, surface albedos, and new mixed-phase ice nucleation schemes to these biases. CAM5 net TOA all-sky shortwave (SW) and outgoing longwave radiation (OLR) fluxes are generally within 10 W m−2 of Clouds and the Earth’s Radiant Energy System Energy Balanced and Filled (CERES-EBAF) observations. However, CAM5 has compensating SW errors: Surface albedos over snow are too high while cloud amount and LWP are too low. Use of a new CAM5 Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) lidar simulator that corrects an error in the treatment of snow crystal size confirms insufficient cloud amount in CAM5 year-round. CAM5 OLR is too low because of low surface temperature in winter, excessive atmospheric water vapor in summer, and excessive cloud heights year-round. Simulations with two new mixed-phase ice nucleation schemes—one based on an empirical fit to ice nuclei observations and one based on classical nucleation theory with prognostic ice nuclei—improve surface climate in winter by increasing cloud amount and LWP. However, net TOA and surface radiation biases remain because of increases in midlevel clouds and a persistent deficit in cloud LWP. These findings highlight challenges with evaluating and modeling Arctic cloud, radiation, and climate processes.

scholarly journals Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation

2017 ◽  
Vol 200 ◽  
pp. 165-194 ◽  
Author(s):  
Joseph C. Charnawskas ◽  
Peter A. Alpert ◽  
Andrew T. Lambe ◽  
Thomas Berkemeier ◽  
Rachel E. O’Brien ◽  
...  
Keyword(s):  
Freezing Temperature ◽  
Organic Aerosol ◽  
Ice Nucleation ◽  
Mixed Phase ◽  
Cloud Formation ◽  
Fossil Fuel Combustion ◽  
Soot Particles ◽  
Ice Nuclei ◽  
Deliquescence Relative Humidity ◽  
Homogeneous Freezing

Anthropogenic and biogenic gas emissions contribute to the formation of secondary organic aerosol (SOA). When present, soot particles from fossil fuel combustion can acquire a coating of SOA. We investigate SOA–soot biogenic–anthropogenic interactions and their impact on ice nucleation in relation to the particles’ organic phase state. SOA particles were generated from the OH oxidation of naphthalene, α-pinene, longifolene, or isoprene, with or without the presence of sulfate or soot particles. Corresponding particle glass transition (Tg) and full deliquescence relative humidity (FDRH) were estimated using a numerical diffusion model. Longifolene SOA particles are solid-like and all biogenic SOA sulfate mixtures exhibit a core–shell configuration (i.e.a sulfate-rich core coated with SOA). Biogenic SOA with or without sulfate formed ice at conditions expected for homogeneous ice nucleation, in agreement with respectiveTgand FDRH. α-pinene SOA coated soot particles nucleated ice above the homogeneous freezing temperature with soot acting as ice nuclei (IN). At lower temperatures the α-pinene SOA coating can be semisolid, inducing ice nucleation. Naphthalene SOA coated soot particles acted as ice nuclei above and below the homogeneous freezing limit, which can be explained by the presence of a highly viscous SOA phase. Our results suggest that biogenic SOA does not play a significant role in mixed-phase cloud formation and the presence of sulfate renders this even less likely. However, anthropogenic SOA may have an enhancing effect on cloud glaciation under mixed-phase and cirrus cloud conditions compared to biogenic SOA that dominate during pre-industrial times or in pristine areas.

scholarly journals Brief Overview of Ice Nucleation

Molecules ◽  
2021 ◽  
Vol 26 (2) ◽  
pp. 392
Author(s):  
Nobuo Maeda
Keyword(s):  
Molecular Level ◽  
Ice Nucleation ◽  
Nucleation Theory ◽  
Classical Nucleation Theory ◽  
Radiation Balance ◽  
Feature Article ◽  
Aircraft Wings ◽  
Food Engineering ◽  
Research Activities ◽  
Important Field

The nucleation of ice is vital in cloud physics and impacts on a broad range of matters from the cryopreservation of food, tissues, organs, and stem cells to the prevention of icing on aircraft wings, bridge cables, wind turbines, and other structures. Ice nucleation thus has broad implications in medicine, food engineering, mineralogy, biology, and other fields. Nowadays, the growing threat of global warming has led to intense research activities on the feasibility of artificially modifying clouds to shift the Earth’s radiation balance. For these reasons, nucleation of ice has been extensively studied over many decades and rightfully so. It is thus not quite possible to cover the whole subject of ice nucleation in a single review. Rather, this feature article provides a brief overview of ice nucleation that focuses on several major outstanding fundamental issues. The author’s wish is to aid early researchers in ice nucleation and those who wish to get into the field of ice nucleation from other disciplines by concisely summarizing the outstanding issues in this important field. Two unresolved challenges stood out from the review, namely the lack of a molecular-level picture of ice nucleation at an interface and the limitations of classical nucleation theory.

Intercomparison of Bulk Cloud Microphysics Schemes in Mesoscale Simulations of Springtime Arctic Mixed-Phase Stratiform Clouds

2006 ◽  
Vol 134 (7) ◽  
pp. 1880-1900 ◽  
Author(s):  
H. Morrison ◽  
J. O. Pinto
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Heat Budget ◽  
Cloud Microphysics ◽  
Ice Nucleation ◽  
Mixed Phase ◽  
Precipitation Rate ◽  
The Arctic ◽  
Ice Clouds ◽  
Complex Scheme

Abstract A persistent, weakly forced, horizontally extensive mixed-phase boundary layer cloud observed on 4–5 May 1998 during the Surface Heat Budget of the Arctic Ocean (SHEBA)/First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment–Arctic Clouds Experiment (FIRE–ACE) is modeled using three different bulk microphysics parameterizations of varying complexity implemented into the polar version of the fifth-generation Pennsylvania State University–National Center for Atmospheric Research Mesoscale Model (MM5). The two simpler schemes predict mostly ice clouds and very little liquid water, while the complex scheme is able to reproduce the observed persistence and horizontal extent of the mixed-phase stratus deck. This mixed-phase cloud results in radiative warming of the surface, the development of a cloud-topped, surface-based mixed layer, and an enhanced precipitation rate. In contrast, the optically thin ice clouds predicted by the simpler schemes lead to radiative cooling of the surface, a strong diurnal cycle in the boundary layer structure, and very weak precipitation. The larger surface precipitation rate using the complex scheme is partly balanced by an increase in the turbulent flux of water vapor from the surface to the atmosphere. This enhanced vapor flux is attributed to changes in the surface and boundary layer characteristics induced by the cloud itself, although cloud–surface interactions appear to be exaggerated in the model compared with reality. The prediction of extensive mixed-phase stratus by the complex scheme is also associated with increased surface pressure and subsidence relative to the other simulations. Sensitivity tests show that the detailed treatment of ice nucleation and prediction of snow particle number concentration in the complex scheme suppresses ice particle concentration relative to the simpler schemes, reducing the vapor deposition rate (for given values of bulk ice mass and ice supersaturation) and leading to much greater amounts of liquid water and mixed-phase cloudiness. These results suggest that the treatments of ice nucleation and the snow intercept parameter in the simpler schemes, which are based upon midlatitude observations, are inadequate for simulating the weakly forced mixed-phase clouds endemic to the Arctic.

Solar irradiance, air pollution and temperature changes in the Arctic

1995 ◽  
Vol 352 (1699) ◽  
pp. 247-258 ◽  
Keyword(s):  
Air Pollution ◽  
Spatial Distribution ◽  
Solar Irradiance ◽  
Early Spring ◽  
Surface Radiation ◽  
The Arctic ◽  
Radiation Balance ◽  
Temperature Changes ◽  
Global Irradiance ◽  
Arctic Haze

A highly significant decrease in the annual sums of global irradiance reaching the surface of the Arctic, averaging 0.36 W m -2 per year, was derived from an analysis of 389 complete years of measurement, beginning in 1950, at 22 pyranometer stations within the Arctic Circle. The smaller data base of radiation balance measurements available showed a much smaller and statistically non-significant change. Reductions in global irradiance were most frequent in the early spring months and in the western sectors of the Arctic, coinciding with the seasonal and spatial distribution of the incursions of polluted air which give rise to the Arctic Haze. Irradiance measured in Antarctica during the same period showed a similar and more widespread decline despite the lower concentrations of pollutants. A marked increase in the surface radiation balance was recorded. Possible reasons for these interpolar anomalies and their consequences for temperature change are discussed.

scholarly journals The Changing Energy Balance of the Polar Regions in a Warmer Climate

2013 ◽  
Vol 26 (10) ◽  
pp. 3112-3129 ◽  
Author(s):  
Lennart Bengtsson ◽  
Kevin I. Hodges ◽  
Symeon Koumoutsaris ◽  
Matthias Zahn ◽  
Paul Berrisford
Keyword(s):  
Polar Region ◽  
Energy Transport ◽  
Climate Model ◽  
Radiant Energy ◽  
Surface Radiation ◽  
The Arctic ◽  
Polar Regions ◽  
Energy Fluxes ◽  
Intergovernmental Panel ◽  
Static Energy

Abstract Energy fluxes for polar regions are examined for two 30-yr periods, representing the end of the twentieth and twenty-first centuries, using data from high-resolution simulations with the ECHAM5 climate model. The net radiation to space for the present climate agrees well with data from the Clouds and the Earth’s Radiant Energy System (CERES) over the northern polar region but shows an underestimation in planetary albedo for the southern polar region. This suggests there are systematic errors in the atmospheric circulation or in the net surface energy fluxes in the southern polar region. The simulation of the future climate is based on the Intergovernmental Panel on Climate Change (IPCC) A1B scenario. The total energy transport is broadly the same for the two 30-yr periods, but there is an increase in the moist energy transport on the order of 6 W m−2 and a corresponding reduction in the dry static energy. For the southern polar region the proportion of moist energy transport is larger and the dry static energy correspondingly smaller for both periods. The results suggest a possible mechanism for the warming of the Arctic that is discussed. Changes between the twentieth and twenty-first centuries in the northern polar region show the net ocean surface radiation flux in summer increases ~18 W m−2 (24%). For the southern polar region the response is different as there is a decrease in surface solar radiation. It is suggested that this is caused by changes in cloudiness associated with the poleward migration of the storm tracks.

scholarly journals Modeling of Aircraft Measurements of Ice Crystal Concentration in the Arctic and a Parameterization for Mixed-Phase Cloud

2017 ◽  
Vol 74 (11) ◽  
pp. 3799-3814 ◽  
Author(s):  
Songmiao Fan ◽  
Daniel A. Knopf ◽  
Andrew J. Heymsfield ◽  
Leo J. Donner
Keyword(s):  
Nucleation Rate ◽  
Large Scale ◽  
Weather Forecasting ◽  
Ice Nucleation ◽  
Mixed Phase ◽  
The Arctic ◽  
Dust Particles ◽  
Aircraft Measurements ◽  
Ice Crystal ◽  
Phase Partitioning

Abstract In this study, two parameterizations of ice nucleation rate on dust particles are used in a parcel model to simulate aircraft measurements of ice crystal number concentration Ni in the Arctic. The parcel model has detailed microphysics for droplet and ice nucleation, growth, and evaporation with prescribed vertical air velocities. Three dynamic regimes are considered, including large-scale ascent, cloud-top generating cells, and their combination. With observed meteorological conditions and aerosol concentrations, the parcel model predicts the number concentrations of size-resolved ice crystals, which may be compared to aircraft measurements. Model results show rapid changes with height/time in relative humidity, Ni, and thermodynamic phase partitioning, which is not resolved in current climate and weather forecasting models. Parameterizations for ice number and nucleation rate in mixed-phase stratus clouds are thus developed based on the parcel model results to represent the time-integrated effect of some microphysical processes in large-scale models.

scholarly journals Possible roles of ice nucleation mode and ice nuclei depletion in the extended lifetime of Arctic mixed-phase clouds

2005 ◽  
Vol 32 (18) ◽  
pp. n/a-n/a ◽  
Author(s):  
Hugh Morrison ◽  
Matthew D. Shupe ◽  
James O. Pinto ◽  
Judith A. Curry
Keyword(s):  
Ice Nucleation ◽  
Mixed Phase ◽  
Nucleation Mode ◽  
Ice Nuclei ◽  
Mixed Phase Clouds

scholarly journals Depositional ice nucleation onto hydrated NaCl particles: a new mechanism for ice formation in the troposphere

2011 ◽  
Vol 11 (8) ◽  
pp. 23139-23167 ◽  
Author(s):  
M. E. Wise ◽  
K. J. Baustian ◽  
T. Koop ◽  
M. A. Freedman ◽  
E. J. Jensen ◽  
...  
Keyword(s):  
Marine Boundary Layer ◽  
Aerosol Particles ◽  
Ice Nucleation ◽  
Sea Salt ◽  
Ice Formation ◽  
Radiation Balance ◽  
Atmospheric Conditions ◽  
Hydrated Form ◽  
Sea Salt Aerosol ◽  
Ice Nuclei

Abstract. Sea-salt aerosol particles (SSA) are ubiquitous in the marine boundary layer and over coastal areas. Therefore SSA have ability to directly and indirectly affect the Earth's radiation balance. The influence SSA have on climate is related to their water uptake and ice nucleation characteristics. In this study, optical microscopy coupled with Raman spectroscopy was used to detect the formation of an NaCl hydrate that could form under atmospheric conditions. NaCl(s) particles deliquesced at the well established value of 75.7 ± 2.5 % RH. NaCl(aq) particles effloresced to a mixture of hydrated and non-hydrated particles at temperatures between 236 and 252 K. The aqueous particles effloresced into the non-hydrated form at temperatures warmer than 252 K. At temperatures colder than 236 K all particles effloresced into the hydrated form. The deliquescence relative humidities (DRH) of hydrated NaCl(s) particles ranged from 76.6 to 93.2 % RH. Based on the measured DRH and efflorescence relative humidities (ERH), we estimate crystalline NaCl particles could be in the hydrated form 40–80 % of the time in the troposphere. Additionally, the ice nucleating abilities of NaCl(s) and hydrated NaCl(s) were determined at temperatures ranging from 221 to 238 K. NaCl(s) particles depositionally nucleated ice at an average Sice value of 1.11 ± 0.07. Hydrated NaCl(s) particles depositionally nucleated ice at an average Sice value of 1.02 ± 0.04. When a mixture of hydrated and anhydrous NaCl(s) particles was present in the same sample, ice preferentially nucleated on the hydrated particles 100 % of the time. While both types of particles are efficient ice nuclei, hydrated NaCl(s) particles are better ice nuclei than NaCl(s) particles.

scholarly journals The potential influence of Asian and African mineral dust on ice, mixed-phase and liquid water clouds

2010 ◽  
Vol 10 (18) ◽  
pp. 8649-8667 ◽  
Author(s):  
A. Wiacek ◽  
T. Peter ◽  
U. Lohmann
Keyword(s):  
Liquid Water ◽  
Mineral Dust ◽  
Dust Emission ◽  
Ice Nucleation ◽  
Transport Processes ◽  
Mixed Phase ◽  
Ice Clouds ◽  
Cloud Processing ◽  
Ice Nuclei ◽  
Mixed Phase Clouds

Abstract. This modelling study explores the availability of mineral dust particles as ice nuclei for interactions with ice, mixed-phase and liquid water clouds, also tracking the particles' history of cloud-processing. We performed 61 320 one-week forward trajectory calculations originating near the surface of major dust emitting regions in Africa and Asia using high-resolution meteorological analysis fields for the year 2007. Dust-bearing trajectories were assumed to be those coinciding with known dust emission seasons, without explicitly modelling dust emission and deposition processes. We found that dust emissions from Asian deserts lead to a higher potential for interactions with high ice clouds, despite being the climatologically much smaller dust emission source. This is due to Asian regions experiencing significantly more ascent than African regions, with strongest ascent in the Asian Taklimakan desert at ~25%, ~40% and 10% of trajectories ascending to 300 hPa in spring, summer and fall, respectively. The specific humidity at each trajectory's starting point was transported in a Lagrangian manner and relative humidities with respect to water and ice were calculated in 6-h steps downstream, allowing us to estimate the formation of liquid, mixed-phase and ice clouds. Downstream of the investigated dust sources, practically none of the simulated air parcels reached conditions of homogeneous ice nucleation (T≲−40 °C) along trajectories that have not experienced water saturation first. By far the largest fraction of cloud forming trajectories entered conditions of mixed-phase clouds, where mineral dust will potentially exert the biggest influence. The majority of trajectories also passed through atmospheric regions supersaturated with respect to ice but subsaturated with respect to water, where so-called "warm ice clouds" (T≳−40 °C) theoretically may form prior to supercooled water or mixed-phase clouds. The importance of "warm ice clouds" and the general influence of dust in the mixed-phase cloud region are highly uncertain due to both a considerable scatter in recent laboratory data from ice nucleation experiments, which we briefly review in this work, and due to uncertainties in sub-grid scale vertical transport processes unresolved by the present trajectory analysis. For "classical" cirrus-forming temperatures (T≲−40 °C), our results show that only mineral dust ice nuclei that underwent mixed-phase cloud-processing, most likely acquiring coatings of organic or inorganic material, are likely to be relevant. While the potential paucity of deposition ice nuclei shown in this work dimishes the possibility of deposition nucleation, the absence of liquid water droplets at T≲−40 °C makes the less explored contact freezing mechanism (involving droplet collisions with bare ice nuclei) highly inefficient. These factors together indicate the necessity of further systematic studies of immersion mode ice nucleation on mineral dust suspended in atmospherically relevant coatings.

scholarly journals Cloud_cci AVHRR-PM dataset version 3: 35 year climatology of global cloud and radiation properties

2019 ◽  
Author(s):  
Martin Stengel ◽  
Stefan Stapelberg ◽  
Oliver Sus ◽  
Stephan Finkensieper ◽  
Benjamin Würzler ◽  
...  
Keyword(s):  
Radiant Energy ◽  
Energy System ◽  
Global Scale ◽  
Radiative Flux ◽  
Surface Radiation ◽  
Digital Object Identifier ◽  
Cloud Detection ◽  
Cloud Properties ◽  
Global Quality ◽  
Ice Water

Abstract. We present version 3 of the Cloud_cci AVHRR-PM dataset which contains a comprehensive set of cloud and radiative flux properties on a global scale covering the period of 1982 to 2016. The properties were retrieved from Advanced Very High Resolution Radiometer (AVHRR) measurements recorded by the afternoon (post meridiem, PM) satellites of the National Oceanic and Atmospheric Administration (NOAA) Polar Operational Environmental Satellites (POES) missions. The cloud properties in version 3 are of improved quality compared with the precursor dataset version 2, providing better global quality scores for cloud detection, cloud phase and ice water path based on validation results against A-Train sensors. Furthermore, the parameter set was extended by a suite of broadband radiative flux properties. They were calculated by combining the retrieved cloud properties with thermodynamic profiles from reanalysis and surface properties. The flux properties comprise upwelling and downwelling, shortwave and longwave broadband fluxes at the surface (bottom-of-atmosphere - BOA) and top-of-atmosphere (TOA). All fluxes were determined at AVHRR pixel level for all-sky and clear-sky conditions, which will particularly facilitate the assessment of the cloud radiative effect at BOA and TOA in future studies. Validation of the BOA downwelling fluxes against the Baseline Surface Radiation Network (BSRN) show a very good agreement. This is supported by comparisons of multi-annual mean maps with NASA's Clouds and the Earth's Radiant Energy System (CERES) products for all fluxes at BOA and TOA. The Cloud_cci AVHRR-PM version 3 dataset allows for a large variety of climate applications that build on cloud properties, radiative flux properties and/or the link between them. For the presented Cloud_cci AVHRR-PMv3 dataset a Digital Object Identifier has been issued: https://doi.org/10.5676/DWD/ESA_Cloud_cci/AVHRR-PM/V003 (Stengel et al., 2019).

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