Leach Rates of High Level Waste and Spent Fuel. - Limiting Rates as Determined By Backfill and Bedrock Conditions.

1981 ◽  
Vol 11 ◽  
Author(s):  
Ivars Neretnieks

The release rate of radionuclides from a degraded canister containing radioactive waste is controlled by diffusion through the backfill and by diffusion into the water flowing past the canister. In low porosity low permeability bedrock like the Swedish granites the amount of water which can be contaminated may be very small. Two sample cases are calculated. One uses the conditions for a repository for vitrified high level waste, the other applies to a repository for spent fuel. The small amount of water which can carry the waste in combination with the low solubilities for the major longlived actinides limit the release rate from the repositories to very small values.

Author(s):  
Marnix Braeckeveldt ◽  
Luc Ooms ◽  
Gustaaf Geenen

Abstract The BR3 reactor (10.5 MWe) at the Nuclear Research Center SCK•CEN was the first PWR plant installed in Europe and has been shut down in 1987. The BR3 reactor is from 1989 in a decommissioning stage and most of the spent fuel is presently still stored in the deactivation pool of the BR3 plant and has to be evacuated. The BR3 was used as a test-reactor for new fuel types and assemblies (Mixed Oxide (MOX) fuel, fuel rods containing burnable poison (Gd2O3) and other types of fuels). Some fuel rods, having undergone a destructive analysis, are stored in different laboratories at the SCK•CEN. In total, the BR3 spent fuel comprises the equivalent of almost 200 fuel assemblies corresponding to some 5000 fuel rods. Beside the spent BR3 fuel, a limited number of spent fuel rods, with equivalent characteristics as the BR3 fuel but irradiated in research reactors outside Belgium and stored in other buildings at the SCK•CEN nuclear site, were added to the inventory of spent fuel to be evacuated. Various options such as reprocessing and intermediate storage awaiting final disposal were evaluated against criteria as available techniques, safety, waste production and overall costs. Finally the option of an AFR (away-from-reactor) intermediate dry storage of the BR3 and other spent fuel in seven CASTOR BR3® casks was adopted. As the SCK•CEN declared this spent fuel as radioactive waste, NIRAS/ONDRAF, the Belgian radioactive waste management agency became directly involved and the decision was taken to construct a small building at the Belgoprocess nuclear site for storing the CASTOR BR3® casks. Loading at the SCK•CEN followed by transport to Belgoprocess and storage is scheduled to take place at the end of 2001. The CASTOR BR3® cask weighing some 25 tonnes, consists of a monolithic body and has two independent lids with metal seals guaranteeing the long term leak-tightness of the cask. The CASTOR BR3® cask is designed for transport and the intermediate storage of at least 50 years. Although a defect of the leaktightness of a CASTOR BR3® cask is very unlikely to occur, an intervention scenario had to be developed. As no pool is present at the Belgoprocess nuclear site to unload the fuel, an innovative procedure is developed that consists of transferring the basket, containing the spent fuel, into another CASTOR BR3® cask. This operation can be performed in the hot cell of the existing storage building for high level waste at the Belgoprocess site.


Author(s):  
Jacques Delay ◽  
Jiri Slovak ◽  
Raymond Kowe

The Implementing Geological Disposal of Radioactive Waste Technology Platform (IGD-TP) was launched in November 2009 to tackle the remaining research, development and demonstration (RD&D) challenges with a view to fostering the implementation of geological disposal programmes for high-level and long-lived waste in Europe. The IGD-TP’s Vision is that “by 2025, the first geological disposal facilities for spent fuel, high-level waste and other long-lived radioactive waste will be operating safely in Europe”. Aside from most of European waste management organisations, the IGD-TP now has 110 members covering most of the RD&D actors in the field of implementing geological disposal of radioactive waste in Europe. The IGD-TP Strategic Research Agenda (SRA), that defines shared RD&D priorities with an important cooperative added value, is used as a basis for the Euratom programme. It provides a vehicle to emphasise RD&D and networking activities that are important for establishing safety cases and fostering disposal implementation. As the IGD-TP brings together the national organisations which have a mandate to implement geological disposal and act as science providers, its SRA also ensures a balance between fundamental science, implementation-driven RD&D and technological demonstration. The SRA is in turn supported by a Deployment Plan (DP) for the Joint Activities to be carried out by the Technology Platform with its members and participants. The Joint Activities were derived from the individual SRA Topics and prioritized and assigned a timeline for their implementation. The deployment scheme of the activities is updated on a yearly basis.


Author(s):  
Pierre Van Iseghem ◽  
Jan Marivoet

This paper discusses the impact of the parameter values used for the transport of radionuclides from high-level radioactive waste to the far-field on the long-term safety of a proposed geological disposal in the Boom Clay formation in Belgium. The methodology of the Safety Assessment is explained, and the results of the Safety Assessment for vitrified high-level waste and spent fuel are presented. The radionuclides having the strongest impact on the dose-to-man for both HLW glass and spent fuel are 79Se, 129I, 126Sn, 36Cl, and 99Tc. Some of them are volatile during the vitrification process, other radionuclides are activation products, and for many of them there is no accurate information on their inventory in the waste form. The hypotheses in the selection of the main parameter values are further discussed, together with the status of the R&D on one of the main dose contributing radionuclides (79Se).


2016 ◽  
Vol 722 ◽  
pp. 59-65
Author(s):  
Markéta Kočová ◽  
Zdeňka Říhová ◽  
Jan Zatloukal

Nowadays manipulation and depositing of high-level radioactive waste has become the most important issue, which needs to be solved. High-level radioactive waste consists mainly of spent fuel elements from nuclear power plants, which cannot be deposited for long time in surface repositories in the same way as it is possible in case of low and medium level radioactive waste. The most effective and safe solution in longer time horizon seems to be deep geological repository of high level waste. In this process of deposition, large amount of specific conditions needs to be taken into account while designing the whole underground complex, because the materials and structures must fulfil all necessary requirements. Then adequate safety will be ensured.


2003 ◽  
Vol 807 ◽  
Author(s):  
L. H. Johnson ◽  
J. W. Schneider ◽  
Piet Zuidema ◽  
P. Gribi ◽  
G. Mayer ◽  
...  

ABSTRACTNagra (the Swiss National Cooperative for the Disposal of Radioactive Waste) has completed a study to determine the suitability of Opalinus Clay as a host rock for a repository for spent fuel (SF), high-level waste from reprocessing (HLW) and long-livedintermediate-level waste (ILW). The proposed siting area is in the Zürcher Weinland region of Northern Switzerland. A repository at this site is shown to provide sufficient safety for a spectrum of assessment cases that is broad enough to cover all reasonable possibilities for the evolution of the system. Furthermore, the system is robust; i.e. remaining uncertainties do not put safety in question.


2015 ◽  
Vol 79 (6) ◽  
pp. 1591-1597 ◽  
Author(s):  
R. Kowe ◽  
J. Delay ◽  
M. Hammarström ◽  
T. Beattie ◽  
M. Palmu

AbstractThe Implementing Geological Disposal of Radioactive Waste Technology Platform (IGD-TP) was launched in November 2009 to facilitate international cooperation in common areas of research, development and demonstration (RD&D) with a view to advancing the implementation of geological disposal facilities for spent fuel, high-level and other long-lived waste in Europe.The IGD-TP's Vision is that “by 2025, the first geological disposal facilities for spent fuel, high-level waste and other long-lived radioactive waste will be operating safely in Europe”. Aside from most European waste management organisations, the IGD-TP currently has 124 members covering most of the RD&D actors in the field of implementing geological disposal of radioactive waste in Europe.Five years after its inception, the IGD-TP has been shown to play a leading role in coordinating joint actions for RD&D in radioactive waste geological disposal programmes. The work of the platform takes into account differences between the timing and challenges for the respective waste management programmes. Following implementation of Posiva's geological disposal facility in Finland it is expected that within the next 5 years the construction of the Swedish and French geological disposal facilities will commence. Within IGD-TP, the SecIGD2 project whose remit is “Coordination and Support Action under the 7th Framework programme” aims at supporting, at the European level, the networking and structuring of RD&D programmes and competences in countries with less advanced geological disposal programmes, including those in the new European Union Member States. Furthermore, the SecIGD2 supports the development and coordination of the necessary competences to meet the Vision 2025 as a part of the platform's Competence Maintenance, Education and Training (CMET) working group.


2012 ◽  
Vol 76 (8) ◽  
pp. 3475-3482 ◽  
Author(s):  
T. W. Hicks ◽  
S. Watson ◽  
S. Norris ◽  
G. Towler ◽  
D. Reedha ◽  
...  

AbstractThe 2008 UK government White Paper, published as part of the Managing Radioactive Waste Safety programme, identified benefits to disposing of all of the UK's higher activity wastes at the same site. That is, a single geological disposal facility (GDF) could be constructed that consists of a module for low- and intermediate-level waste, and a module for high-level waste and spent fuel.A safety case for a co-located GDF will have to consider the extent to which evolving thermo-hydro-mechanical-chemical and gas (THMCG) conditions in and around one module may affect conditions in the other module, including the extent to which barrier performance and radionuclide migration behaviour could be altered. Several research projects have been undertaken on behalf of Radioactive Waste Management Directorate aimed at understanding and evaluating the THMCG interactions that might occur during the disposal facility operational and post-closure phases.This paper describes research on THMCG interactions between disposal modules based on illustrative GDF designs for different host rock environments. Interactions were evaluated using simple analytical solutions and detailed three-dimensional models. The analyses demonstrated that interactions can be controlled by design constraints.


2012 ◽  
Vol 76 (8) ◽  
pp. 3373-3380 ◽  
Author(s):  
S. Vines ◽  
R. Beard

AbstractIn the UK, radioactive wastes currently planned for disposal in a geological disposal facility (GDF) are intermediate-level waste, some low-level waste and high-level waste. Disposal of other materials, including spent fuel, separated uranium and separated plutonium are also included in the planning of a GDF, if such materials are classified as wastes in the future. This paper gives an overview of the radionuclide behaviour research studies of the Nuclear Decommissioning Authority Radioactive Waste Management Directorate (NDA RWMD). The NDA RWMD's current understanding of the processes that control radionuclide behaviour in groundwater and how the engineered and natural barriers in a GDF would contain radionuclides is presented. Areas requiring further work are also identified.


1983 ◽  
Vol 26 ◽  
Author(s):  
P. W. Levy ◽  
J. A. Kierstead

ABSTRACTVery rough estimates have been made of the total amount, the formation rate and spatial distribution of the Na metal colloid particles induced in rock salt adjacent to four types of radioactive waste canisters. A number of extrapolations were required. Salt immediately adjacent to a lightly shielded, 2.16 kW, high level waste canister could be converted entirely to colloidal Na (and presumably chlorine gas) in 200-400 years. The total Na metal formed will be 250-300 kg. A heavily shielded, 3.3 kW, spent fuel canister will convert roughly 0.3 percent of the salt at the canister surface to colloidal Na and the total sodium metal will be roughly 0.5 kg. Even at the lowest colloid levels the Na metal formed should greatly influence interactions between canisters and the surrounding salt, particularly if brine enters.


1981 ◽  
Vol 6 ◽  
Author(s):  
I-Ming Chou

Rock-salt deposits have been considered as a possible medium for the permanent storage of high-level radioactive wastes and spent fuel. Brine inclusions present in natural salt can migrate toward the waste if the temperature and the temperature gradients in the vicinity of the radioactive waste are large enough. This migration is due to the dissolution of salt at the hot side of the salt-brine interface, ion diffusion through the brine droplet, and the precipitation of salt at the cold side of the salt brine interface.


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