scholarly journals Electrical Control of Quantum Emitters in a Van der Waals Heterostructure

Author(s):  
Simon White ◽  
Tieshan Yang ◽  
Nikolai Dontschuk ◽  
Chi Li ◽  
Zaiquan Xu ◽  
...  

Abstract Controlling and manipulating individual quantum systems in solids underpins the growing interest in development of scalable quantum technologies1, 2. Recently, hexagonal boron nitride (hBN) has garnered significant attention in quantum photonic applications due to its ability to host optically stable quantum emitters3-7. However, the large band gap of hBN and the lack of efficient doping inhibits electrical triggering and limits opportunities to study electrical control of emitters. Here, we show an approach to electrically modulate quantum emitters in an hBN–graphene van der Waals heterostructure. We show that quantum emitters in hBN can be reversibly activated and modulated by applying a bias across the device. Notably, a significant number of quantum emitters are intrinsically dark, and become optically active at non-zero voltages. To explain the results, we provide a heuristic electrostatic model of this unique behaviour. Finally, employing these devices we demonstrate a nearly-coherent source with linewidths of ~ 160 MHz. Our results enhance the potential of hBN for tunable solid state quantum emitters for the growing field of quantum information science.

2019 ◽  
Vol 114 (6) ◽  
pp. 062104 ◽  
Author(s):  
Alessio Scavuzzo ◽  
Shai Mangel ◽  
Ji-Hoon Park ◽  
Sanghyup Lee ◽  
Dinh Loc Duong ◽  
...  

2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Arunabh Mukherjee ◽  
Kamran Shayan ◽  
Lizhong Li ◽  
Jie Shan ◽  
Kin Fai Mak ◽  
...  

Abstract Isolated spins are the focus of intense scientific exploration due to their potential role as qubits for quantum information science. Optical access to single spins, demonstrated in III-V semiconducting quantum dots, has fueled research aimed at realizing quantum networks. More recently, quantum emitters in atomically thin materials such as tungsten diselenide have been demonstrated to host optically addressable single spins by means of electrostatic doping the localized excitons. Electrostatic doping is not the only route to charging localized quantum emitters and another path forward is through band structure engineering using van der Waals heterojunctions. Critical to this second approach is to interface tungsten diselenide with other van der Waals materials with relative band-alignments conducive to the phenomenon of charge transfer. In this work we show that the Type-II band-alignment between tungsten diselenide and chromium triiodide can be exploited to excite localized charged excitons in tungsten diselenide. Leveraging spin-dependent charge transfer in the device, we demonstrate spin selectivity in the preparation of the spin-valley state of localized single holes. Combined with the use of strain-inducing nanopillars to coordinate the spatial location of tungsten diselenide quantum emitters, we uncover the possibility of realizing large-scale deterministic arrays of optically addressable spin-valley holes in a solid state platform.


Nano Letters ◽  
2021 ◽  
Vol 21 (6) ◽  
pp. 2634-2641 ◽  
Author(s):  
Weijun Ren ◽  
Yulou Ouyang ◽  
Pengfei Jiang ◽  
Cuiqian Yu ◽  
Jia He ◽  
...  

Nanoscale ◽  
2021 ◽  
Author(s):  
Wenxuan Wang ◽  
Wei Sun ◽  
Hang Li ◽  
Ying Bai ◽  
Fengzhu Ren ◽  
...  

One of the promising research topics on two-dimensional (2D) van der Waals (vdW) material based devices is the nonvolatile electrical control of magnetism. Usually, it is very hard to tune...


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