Ultrafast Spin Dynamics

2020 ◽  
Vol 29 (9) ◽  
pp. 2-6
Author(s):  
Dong-Hyun KIM

Ultrafast spin dynamics is one of the key aspects in the realization of ultrafast spintronic devices. Moreover, it has attracted much attention due to important fundamental spin phenomena existing on nano-, pico-, and femtosecond timescales. The most important interaction of magnetism is, of course, an exchange interaction. However, in practice, spin generally exists interacting with a lattice and an electron in the form of solid. Therefore, a fundamental understanding of ultrafast spin dynamics is involved in various physical phenomena, such as spin-orbit interactions and optomagnetism. In this article, recent trends in ultrafast spin dynamics research are discussed. Ultrafast spin dynamics, which started with the observation of ultrafast demagnetization/remagnetization triggered by femtosecond laser pulses, has been intensively investigated so far. The magnetooptical Kerr effect and X-ray magnetic circular dichroism techniques are introduced as two of the main experimental techniques for exploring ultrafast spin dynamics. THz emission and ultrafast magnetic cooling phenomena are briefly introduced as examples of recent topics in the field of ultrafast spin dynamics.

Author(s):  
A. Zagdoud ◽  
M. Vomir ◽  
M. Albrecht ◽  
M. Barthelemy ◽  
J.-Y. Bigot

SPIN ◽  
2015 ◽  
Vol 05 (03) ◽  
pp. 1550004 ◽  
Author(s):  
I. Radu ◽  
C. Stamm ◽  
A. Eschenlohr ◽  
F. Radu ◽  
R. Abrudan ◽  
...  

Controlling magnetic order on ultrashort timescales is crucial for engineering the next-generation magnetic devices that combine ultrafast data processing with ultrahigh-density data storage. An appealing scenario in this context is the use of femtosecond (fs) laser pulses as an ultrafast, external stimulus to fully set the orientation and the magnetization magnitude of a spin ensemble. Achieving such control on ultrashort timescales, e.g., comparable to the excitation event itself, remains however a challenge due to the lack of understanding the dynamical behavior of the key parameters governing magnetism: The elemental magnetic moments and the exchange interaction. Here, we investigate the fs laser-induced spin dynamics in a variety of multi-component alloys and reveal a dissimilar dynamics of the constituent magnetic moments on ultrashort timescales. Moreover, we show that such distinct dynamics is a general phenomenon that can be exploited to engineer new magnetic media with tailor-made, optimized dynamic properties. Using phenomenological considerations, atomistic modeling and time-resolved X-ray magnetic circular dichroism (XMCD), we demonstrate demagnetization of the constituent sub-lattices on significantly different timescales that depend on their magnetic moments and the sign of the exchange interaction. These results can be used as a “recipe” for manipulation and control of magnetization dynamics in a large class of magnetic materials.


2021 ◽  
Vol 118 (22) ◽  
pp. e2103696118
Author(s):  
Daniel G. Mazzone ◽  
Derek Meyers ◽  
Yue Cao ◽  
James G. Vale ◽  
Cameron D. Dashwood ◽  
...  

Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic X-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets and that they persist for several picoseconds, which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.


2003 ◽  
Vol 780 ◽  
Author(s):  
R. Houbertz ◽  
J. Schulz ◽  
L. Fröhlich ◽  
G. Domann ◽  
M. Popall ◽  
...  

AbstractReal 3-D sub-νm lithography was performed with two-photon polymerization (2PP) using inorganic-organic hybrid polymer (ORMOCER®) resins. The hybrid polymers were synthesized by hydrolysis/polycondensation reactions (modified sol-gel synthesis) which allows one to tailor their material properties towards the respective applications, i.e., dielectrics, optics or passivation. Due to their photosensitive organic functionalities, ORMOCER®s can be patterned by conventional photo-lithography as well as by femtosecond laser pulses at 780 nm. This results in polymerized (solid) structures where the non-polymerized parts can be removed by conventional developers.ORMOCER® structures as small as 200 nm or even below were generated by 2PP of the resins using femtosecond laser pulses. It is demonstrated that ORMOCER®s have the potential to be used in components or devices built up by nm-scale structures such as, e.g., photonic crystals. Aspects of the materials in conjunction to the applied technology are discussed.


Author(s):  
K. H. Leong ◽  
T. Y. Plew ◽  
R. L. Maynard ◽  
A. A. Said ◽  
L. A. Walker

Author(s):  
V. Pouget ◽  
E. Faraud ◽  
K. Shao ◽  
S. Jonathas ◽  
D. Horain ◽  
...  

Abstract This paper presents the use of pulsed laser stimulation with picosecond and femtosecond laser pulses. We first discuss the resolution improvement that can be expected when using ultrashort laser pulses. Two case studies are then presented to illustrate the possibilities of the pulsed laser photoelectric stimulation in picosecond single-photon and femtosecond two-photon modes.


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