scholarly journals Spatial and Temporal Variability of Total Column Ozone over the Indian Subcontinent: A Study Based on Nimbus-7 TOMS Satellite

2014 ◽  
Vol 04 (05) ◽  
pp. 884-898 ◽  
Author(s):  
Vazhathottathil Madhu
2009 ◽  
Vol 9 (4) ◽  
pp. 16233-16266
Author(s):  
G. W. K. Moore ◽  
S. Abernethy ◽  
J. L. Semple

Abstract. Ozone is an important atmospheric constituent due to its role as both a greenhouse gas and an oxidant. Recent measurements in the Mount Everest region indicate the presence of ozone at elevations from 5000 to 9000 m a.s.l. that are the result of both stratospheric and tropospheric sources. Here we examine the temporal variability in the surface ozone concentration measurements from the ABC-Pyramid Observatory in the Mount Everest region during 2006 and compare it to the total column ozone data from the OMI instrument as well as meteorological fields from the ECMWF Interim Reanalysis. Both the surface ozone at and the total column ozone over the ABC-Pyramid Observatory site have maxima in the pre-monsoon period. We show that during this period, there is a statistically significant correlation between the two suggesting that the stratosphere was an important contributor to the high levels of ozone observed during the period. There was a hiatus in the monsoon in June that resulted in a return of westerlies over northern Indian and southern Tibet and as a result, the aforementioned correlation extended into June. No such correlation exists during the monsoon and post-monsoon periods. Spatial correlation maps between the surface ozone and total column ozone as well as meteorological fields from the ECMWF Interim Reanalysis support the contention that there is a significant stratospheric contribution in the pre-monsoon period that is absent during and after the monsoon.


2017 ◽  
Vol 30 (8) ◽  
pp. 2961-2988 ◽  
Author(s):  
Krzysztof Wargan ◽  
Gordon Labow ◽  
Stacey Frith ◽  
Steven Pawson ◽  
Nathaniel Livesey ◽  
...  

The assimilated ozone product from the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), produced at NASA’s Global Modeling and Assimilation Office (GMAO) spanning the time period from 1980 to the present is described herein, and its quality is assessed. MERRA-2 assimilates partial column ozone retrievals from a series of Solar Backscatter Ultraviolet Radiometer (SBUV) instruments on NASA and NOAA spacecraft between January 1980 and September 2004: starting in October 2004, retrieved ozone profiles from the Microwave Limb Sounder (MLS) and total column ozone from the Ozone Monitoring Instrument on NASA’s EOS Aura satellite are assimilated. The MERRA-2 ozone is compared with independent satellite and ozonesonde data, focusing on the representation of the spatial and temporal variability of stratospheric and upper-tropospheric ozone and on implications of the change in the observing system from SBUV to EOS Aura. The comparisons show agreement within 10% (standard deviation of the difference) between MERRA-2 profiles and independent satellite data in most of the stratosphere. The agreement improves after 2004, when EOS Aura data are assimilated. The standard deviation of the differences between the lower-stratospheric and upper-tropospheric MERRA-2 ozone and ozonesondes is 11.2% and 24.5%, respectively, with correlations of 0.8 and above, indicative of a realistic representation of the near-tropopause ozone variability in MERRA-2. The agreement improves significantly in the EOS Aura period; however, MERRA-2 is biased low in the upper troposphere with respect to the ozonesondes. Caution is recommended when using MERRA-2 ozone for decadal changes and trend studies.


2015 ◽  
Vol 8 (10) ◽  
pp. 4487-4505 ◽  
Author(s):  
K.-L. Chang ◽  
S. Guillas ◽  
V. E. Fioletov

Abstract. Total column ozone variations estimated using ground-based stations provide important independent source of information in addition to satellite-based estimates. This estimation has been vigorously challenged by data inhomogeneity in time and by the irregularity of the spatial distribution of stations, as well as by interruptions in observation records. Furthermore, some stations have calibration issues and thus observations may drift. In this paper we compare the spatial interpolation of ozone levels using the novel stochastic partial differential equation (SPDE) approach with the covariance-based kriging. We show how these new spatial predictions are more accurate, less uncertain and more robust. We construct long-term zonal means to investigate the robustness against the absence of measurements at some stations as well as instruments drifts. We conclude that time series analyzes can benefit from the SPDE approach compared to the covariance-based kriging when stations are missing, but the positive impact of the technique is less pronounced in the case of drifts.


Elem Sci Anth ◽  
2021 ◽  
Vol 9 (1) ◽  
Author(s):  
María Cazorla ◽  
René Parra ◽  
Edgar Herrera ◽  
Francisco Raimundo da Silva

In this study, we characterize atmospheric ozone over the tropical Andes in the boundary layer, the free troposphere, and the stratosphere; we quantify each contribution to total column ozone, and we evaluate the performance of the multi-sensor reanalysis (MSR2) in the region. Thus, we present data taken in Ecuador and Peru (2014–2019). The contribution from the surface was determined by integrating ozone concentrations measured in Quito and Cuenca (Ecuador) up to boundary layer height. In addition, tropospheric and stratospheric column ozone were quantified from ozone soundings (38) launched from Quito during the study time period. Profiles were compared against soundings at Natal (SHADOZ network) for being the closest observational reference with sufficient data in 2014–2019. Data were also compared against stratospheric mixing ratios from the Aura Microwave Limb Sounder (Aura MLS). Findings demonstrate that the stratospheric component of total column ozone over the Andes (225.2 ± 8.9 Dobson Units [DU]) is at similar levels as those observed at Natal (223.3 ± 8.6 DU), and observations are comparable to Aura MLS data. In contrast, the tropospheric contribution is lower over the Andes (20.2 ± 4.3 DU) when compared to Natal (35.4 ± 6.4 DU) due to a less deep and cleaner troposphere. From sounding extrapolation of Quito profiles down to sea level, we determined that altitude deducts about 5–7 DU from the total column, which coincides with a 3%–4% overestimation of the MSR2 over Quito and Marcapomacocha (Peru). In addition, when MSR2 data are compared along a transect that crosses from the Amazon over Quito, the Ecuadorian coast side, and into the Pacific, observations are not significantly different among the three first locations. Results point to coarse reanalysis resolution not being suitable to resolve the formidable altitude transition imposed by the Andes mountain chain. This work advances our knowledge of atmospheric ozone over the study region and provides a robust time series of upper air measurements for future evaluations of satellite and reanalysis products.


2013 ◽  
Vol 6 (6) ◽  
pp. 10081-10115 ◽  
Author(s):  
E. W. Chiou ◽  
P. K. Bhartia ◽  
R. D. McPeters ◽  
D. G. Loyola ◽  
M. Coldewey-Egbers ◽  
...  

Abstract. This paper describes the comparison of the variability of total column ozone inferred from the three independent multi-year data records, namely, (i) SBUV(v8.6) profile total ozone, (ii) GTO(GOME-Type total ozone), and (iii) Ground-based total ozone data records covering the 16-yr overlap period (March 1996 through June 2011). Analyses are conducted based on area weighted zonal means for (0–30° S), (0–30° N), (50–30° S), and (30–60° N). It has been found that on average, the differences in monthly zonal mean total ozone vary between −0.32 to 0.76 % and are well within 1%. For "GTO minus SBUV", the standard deviations and ranges (maximum minus minimum) of the differences regarding monthly zonal mean total ozone vary between 0.58 to 0.66% and 2.83 to 3.82% respectively, depending on the latitude band. The corresponding standard deviations and ranges regarding the differences in monthly zonal mean anomalies show values between 0.40 to 0.59% and 2.19 to 3.53%. The standard deviations and ranges of the differences "Ground-based minus SBUV" regarding both monthly zonal means and anomalies are larger by a factor of 1.4 to 2.9 in comparison to "GTO minus SBUV". The Ground-based zonal means, while show no systematic differences, demonstrate larger scattering of monthly data compared to satellite-based records. The differences in the scattering are significantly reduced if seasonal zonal averages are analyzed. The trends of the differences "GTO minus SBUV" and "Ground-based minus SBUV" are found to vary between −0.04 and 0.12% yr−1 (−0.11 and 0.31 DU yr−1). These negligibly small trends have provided strong evidence that there are no significant time dependent differences among these multi-year total ozone data records. Analyses of the deviations from pre-1980 level indicate that for the overlap period of 1996 to 2010, all three data records show gradual recovery at (30–60° N) from −5% in 1996 to −2% in 2010. The corresponding recovery at (50–30° S) is not as obvious until after 2006.


2013 ◽  
Vol 8 (3) ◽  
pp. 204-209

Results of the total column ozone and ultraviolet (UV-B) erythemally weighted irradiance measurements at the ground-based solar monitoring station at the Kishinev (Moldova) are presented. Diffuse and global components of solar UV-B erythemal irradiance on horizontal plane were continuously measured with sensors UV-S-B-C (of broadband 280-315 nm), Kipp&Zonen. Monthly totals of global and diffuse components of solar UV-B erythemal radiation reveal distinct seasonal variation with respective minimum in winter and maximum in summer. Typical values for these components in limiting cases are presented. A simple polynomial relationship between the global and diffuse components of solar UV-B erythemal radiation measured for cloudless days was derived. It was shown that coefficients of the polynomial depend on daily mean value of aerosol optical thickness (AOT). Collocated measurements of AOT have been carried out with the sunphotometer Cimel CE-318 within the framework of the Aerosol Robotic Network (AERONET) program, managed by NASA/GSFC. Total column ozone content was retrieved from direct solar ultraviolet radiation measurements at 3 discrete wavelengths centered at 305.5, 312.5, and 320 nm within the UV-B range. Ozone measurements were regularly carried out with the hand-held MICROTOPS II Ozonemeter, Solar Light Co. Monthly average values of total column ozone content measured with the MICROTOPS II at the Kishinev are in close agreement with those ones retrieved from the multiyear (1978-2004) database statistics acquired from satellite platforms measurements with the Total Ozone Mapping Spectrometer (TOMS). It was shown the existence of seasonal variability of the total column ozone content with respective minimum values observed at the end of autumn and winter, and maximum values observed at the end of winter and in spring. The maximum and minimum of daily mean values of total column ozone ever measured with TOMS at the satellite platforms overpassed Kishinev site, amounted of ~540 DU (on February 19, 1985) and ~204 DU (on December 1, 1999). Yearly mean value of total column ozone measured at the Kishinev was ~ 338 DU. Total column ozone measurements carried out with MICROTOPS at the Kishinev site from September 2003 to August 2004, gave maximum and minimum values of ozone daily means at ~ 489 DU (on February 12, 2004) and ~259 DU (on December 3, 2003). The estimation of total column ozone trend derived from the TOMS multi-year statistics was ~ -10 DU/decade.


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