scholarly journals Evaluating the simulated radiative forcings, aerosol properties and stratospheric warmings from the 1963 Agung, 1982 El Chichón and 1991 Mt Pinatubo volcanic aerosol clouds

2020 ◽  
Author(s):  
Sandip S. Dhomse ◽  
Graham W. Mann ◽  
Juan Carlos Antuña Marrero ◽  
Sarah E. Shallcross ◽  
Martyn P. Chipperfield ◽  
...  

Abstract. Accurate quantification of the effects of volcanic eruptions on climate is a key requirement for better attribution of anthropogenic climate change. Here we use the UM-UKCA composition-climate model to simulate the atmospheric evolution of the volcanic aerosol clouds from the three largest eruptions of the 20th century: 1963 Agung, 1982 El Chichón and 1991 Pinatubo. The model has interactive stratospheric chemistry and aerosol microphysics, with coupled aerosol–radiation interactions for realistic composition-dynamics feedbacks. Our simulations align with the design of the Interactive Stratospheric Aerosol Model Intercomparison (ISA-MIP) Historical Eruption SO2 Emissions Assessment. For each eruption, we perform 3-member ensemble model experiments with upper, mid-point and lower estimates for SO2 emission, each initialised to a meteorological state to match the observed phase of the quasi-biennial oscillation (QBO) at the times of the eruptions. We assess how each eruption's emitted SO2 evolves into a tropical reservoir of volcanic aerosol and analyse the subsequent dispersion to mid-latitudes. We compare the simulations to the three volcanic forcing datasets used in historical integrations for the two most recent Coupled Model Intercomparison Project (CMIP) assessments: the Global Space-based Stratospheric Aerosol Climatology (GloSSAC) for CMIP6, and the Sato et al. (1993) and Ammann et al. (2003) datasets used in CMIP5. We also assess the vertical extent of the volcanic aerosol clouds by comparing simulated extinction to Stratospheric Aerosol and Gas Experiment II (SAGE-II) v7.0 satellite aerosol data (1985–1995) for Pinatubo and El Chichón, and to 1964–65 northern hemisphere ground-based lidar measurements for Agung. As an independent test for the simulated volcanic forcing after Pinatubo, we also compare to the shortwave (SW) and longwave (LW) Top-of-the-Atmosphere flux anomalies measured by the Earth Radiation Budget Experiment (ERBE) satellite instrument. For the Pinatubo simulations, an injection of 10 to 14 Tg SO2 gives the best match to the High Resolution Infrared Sounder (HIRS) satellite-derived global stratospheric sulphur burden, with good agreement also to SAGE-II mid-visible and near-infrared extinction measurements. This 10–14 Tg range of emission also generates a heating of the tropical stratosphere that is comparable with the temperature anomaly seen in the ERA-Interim reanalyses. For El Chichón the simulations with 5 Tg and 7 Tg SO2 emission give best agreement with the observations. However, these runs predict a much deeper volcanic cloud than present in the CMIP6 data, with much higher aerosol extinction than the GloSSAC data up to October 1984, but better agreement during the later SAGE-II period. For 1963 Agung, the 9 Tg simulation compares best to the forcing datasets with the model capturing the lidar-observed signature of peak extinction descending from 20 km in 1964 to 16 km in 1965. Overall, our results indicate that the downward adjustment to previous SO2 emission estimates for Pinatubo as suggested by several interactive modelling studies is also needed for the Agung and El Chichón aerosol clouds. This strengthens the hypothesis that interactive stratospheric aerosol models may be missing an important removal or redistribution process (e.g. effects of co-emitted ash) which changes how the tropical reservoir of volcanic aerosol evolves in the initial months after an eruption. Our analysis identifies potentially important inhomogeneities in the CMIP6 dataset for all three periods that are hard to reconcile with variations predicted by the interactive stratospheric aerosol model. We also highlight large differences between the CMIP5 and CMIP6 volcanic aerosol datasets for the Agung and El Chichón periods. Future research should aim to reduce this uncertainty by reconciling the datasets with additional stratospheric aerosol observations.

2020 ◽  
Vol 20 (21) ◽  
pp. 13627-13654
Author(s):  
Sandip S. Dhomse ◽  
Graham W. Mann ◽  
Juan Carlos Antuña Marrero ◽  
Sarah E. Shallcross ◽  
Martyn P. Chipperfield ◽  
...  

Abstract. Accurately quantifying volcanic impacts on climate is a key requirement for robust attribution of anthropogenic climate change. Here we use the Unified Model – United Kingdom Chemistry and Aerosol (UM-UKCA) composition–climate model to simulate the global dispersion of the volcanic aerosol clouds from the three largest eruptions of the 20th century: 1963 Mt Agung, 1982 El Chichón, and 1991 Mt Pinatubo. The model has interactive stratospheric chemistry and aerosol microphysics, with coupled aerosol–radiation interactions for realistic composition–dynamics feedbacks. Our simulations align with the design of the Interactive Stratospheric Aerosol Model Intercomparison (ISA-MIP) “Historical Eruption SO2 Emissions Assessment”. For each eruption, we perform three-member ensemble model experiments for upper, mid-point, and lower estimates of SO2 emission, each re-initialised from a control run to approximately match the observed transition in the phase of the quasi-biennial oscillation (QBO) in the 6 months after the eruptions. With this experimental design, we assess how each eruption's emitted SO2 translates into a tropical reservoir of volcanic aerosol and analyse the subsequent dispersion to mid-latitudes. We compare the simulations to the volcanic forcing datasets (e.g. Space-based Stratospheric Aerosol Climatology (GloSSAC); Sato et al., 1993, and Ammann et al., 2003) that are used in historical integrations for the two most recent Coupled Model Intercomparison Project (CMIP) assessments. For Pinatubo and El Chichón, we assess the vertical extent of the simulated volcanic clouds by comparing modelled extinction to the Stratospheric Aerosol and Gas Experiment (SAGE-II) v7.0 satellite measurements and to 1964–1965 Northern Hemisphere ground-based lidar measurements for Agung. As an independent test for the simulated volcanic forcing after Pinatubo, we also compare simulated shortwave (SW) and longwave (LW) top-of-the-atmosphere radiative forcings to the flux anomalies measured by the Earth Radiation Budget Experiment (ERBE) satellite instrument. For the Pinatubo simulations, an injection of 10 to 14 Tg SO2 gives the best match to the High Resolution Infrared Sounder (HIRS) satellite-derived global stratospheric sulfur burden, with good agreement also with SAGE-II mid-visible and near-infra-red extinction measurements. This 10–14 Tg range of emission also generates a heating of the tropical stratosphere that is consistent with the temperature anomaly present in the ERA-Interim reanalysis. For El Chichón, the simulations with 5 and 7 Tg SO2 emission give best agreement with the observations. However, these simulations predict a much deeper volcanic cloud than represented in the GloSSAC dataset, which is largely based on an interpolation between Stratospheric Aerosol Measurements (SAM-II) satellite and aircraft measurements. In contrast, these simulations show much better agreement during the SAGE-II period after October 1984. For 1963 Agung, the 9 Tg simulation compares best to the forcing datasets with the model capturing the lidar-observed signature of the altitude of peak extinction descending from 20 km in 1964 to 16 km in 1965. Overall, our results indicate that the downward adjustment to SO2 emission found to be required by several interactive modelling studies when simulating Pinatubo is also needed when simulating the Agung and El Chichón aerosol clouds. This strengthens the hypothesis that interactive stratospheric aerosol models may be missing an important removal or re-distribution process (e.g. effects of co-emitted ash) which changes how the tropical reservoir of volcanic aerosol evolves in the initial months after an eruption. Our model comparisons also identify potentially important inhomogeneities in the CMIP6 dataset for all three eruption periods that are hard to reconcile with variations predicted in the interactive stratospheric aerosol simulations. We also highlight large differences between the CMIP5 and CMIP6 volcanic aerosol datasets for the Agung and El Chichón periods. Future research should aim to reduce this uncertainty by reconciling the datasets with additional stratospheric aerosol observations.


2016 ◽  
Author(s):  
Cristen Adams ◽  
Adam E. Bourassa ◽  
Chris A. McLinden ◽  
Chris E. Sioris ◽  
Thomas von Clarmann ◽  
...  

Abstract. Following the large volcanic eruptions of Pinatubo in 1991 and El Chichón in 1982, decreases in stratospheric NO2 associated with enhanced aerosol were observed. The Optical Spectrograph and InfraRed Imaging Spectrometer (OSIRIS) likewise measured widespread enhancements of stratospheric aerosol following seven volcanic eruptions between 2002 and 2014, although the magnitudes of these eruptions were all much smaller than the Pinatubo and El Chichón eruptions. In order to isolate and quantify the relationship between volcanic aerosol and NO2, NO2 anomalies were calculated using measurements from OSIRIS and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). In the tropics, variability due to the quasi-biennial oscillation was subtracted from the timeseries. OSIRIS profile measurements indicate that the strongest relationships between NO2 and volcanic aerosol extinction were for the layer ~ 3–7 km above the tropopause, where OSIRIS stratospheric NO2 partial columns for ~ 3–7 km above the tropopause were found to be smaller than baseline levels during these aerosol enhancements by up to ~ 60 % with typical Pearson correlation coefficients of R ~ −0.7. MIPAS also observed decreases in NO2 partial columns during periods of affected by volcanic aerosol, with percent differences of up to ~ 25 %. An even stronger relationship was observed between OSIRIS aerosol optical depth and MIPAS N2O5 partial columns, with R ~ −0.9, although no link with MIPAS HNO3 was observed. The variation of OSIRIS NO2 with increasing aerosol was found to be quantitatively consistent with simulations from a photochemical box model in terms of both magnitude and degree of non-linearity.


2017 ◽  
Vol 17 (13) ◽  
pp. 8063-8080 ◽  
Author(s):  
Cristen Adams ◽  
Adam E. Bourassa ◽  
Chris A. McLinden ◽  
Chris E. Sioris ◽  
Thomas von Clarmann ◽  
...  

Abstract. Following the large volcanic eruptions of Pinatubo in 1991 and El Chichón in 1982, decreases in stratospheric NO2 associated with enhanced aerosol were observed. The Optical Spectrograph and Infrared Imaging Spectrometer (OSIRIS) measured the widespread enhancements of stratospheric aerosol following seven volcanic eruptions between 2002 and 2014, although the magnitudes of these eruptions were all much smaller than the Pinatubo and El Chichón eruptions. In order to isolate and quantify the relationship between volcanic aerosol and NO2, NO2 anomalies were calculated using measurements from OSIRIS and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). In the tropics, variability due to the quasi-biennial oscillation was subtracted from the time series. OSIRIS profile measurements indicate that the strongest anticorrelations between NO2 and volcanic aerosol extinction were for the 5 km layer starting  ∼  3 km above the climatological mean tropopause at the given latitude. OSIRIS stratospheric NO2 partial columns in this layer were found to be smaller than background NO2 levels during these aerosol enhancements by up to  ∼  60 % with typical Pearson correlation coefficients of R ∼ −0. 7. MIPAS also observed decreases in NO2 partial columns during periods affected by volcanic aerosol, with percent differences of up to  ∼  25 % relative to background levels. An even stronger anticorrelation was observed between OSIRIS aerosol optical depth and MIPAS N2O5 partial columns, with R ∼ −0. 9, although no link with MIPAS HNO3 was observed. The variation in OSIRIS NO2 with increasing aerosol was found to be consistent with simulations from a photochemical box model within the estimated model uncertainty.


2016 ◽  
Author(s):  
Davide Zanchettin ◽  
Myriam Khodri ◽  
Claudia Timmreck ◽  
Matthew Toohey ◽  
Anja Schmidt ◽  
...  

Abstract. The enhancement of the stratospheric aerosol layer by volcanic eruptions induces a complex set of responses causing global and regional climate effects on a broad range of timescales. Uncertainties exist regarding the climatic response to strong volcanic forcing identified in coupled climate simulations that contributed to the fifth phase of the Climate Model Intercomparison Project (CMIP5). In order to better understand the sources of these model diversities, the model intercomparison project on the climate response to volcanic forcing (VolMIP) has defined a coordinated set of idealized volcanic perturbation experiments to be carried out in alignment with the CMIP6 protocol. VolMIP provides a common stratospheric aerosol dataset for each experiment to eliminate differences in the applied volcanic forcing, and defines a set of initial conditions to determine how internal climate variability contributes to determining the response. VolMIP will assess to what extent volcanically-forced responses of the coupled ocean-atmosphere system are robustly simulated by state-of-the-art coupled climate models and identify the causes that limit robust simulated behavior, especially differences in the treatment of physical processes. This paper illustrates the design of the idealized volcanic perturbation experiments in the VolMIP protocol and describes the common aerosol forcing input datasets to be used.


2018 ◽  
Vol 11 (7) ◽  
pp. 2581-2608 ◽  
Author(s):  
Claudia Timmreck ◽  
Graham W. Mann ◽  
Valentina Aquila ◽  
Rene Hommel ◽  
Lindsay A. Lee ◽  
...  

Abstract. The Stratospheric Sulfur and its Role in Climate (SSiRC) Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP) explores uncertainties in the processes that connect volcanic emission of sulfur gas species and the radiative forcing associated with the resulting enhancement of the stratospheric aerosol layer. The central aim of ISA-MIP is to constrain and improve interactive stratospheric aerosol models and reduce uncertainties in the stratospheric aerosol forcing by comparing results of standardized model experiments with a range of observations. In this paper we present four co-ordinated inter-model experiments designed to investigate key processes which influence the formation and temporal development of stratospheric aerosol in different time periods of the observational record. The Background (BG) experiment will focus on microphysics and transport processes under volcanically quiescent conditions, when the stratospheric aerosol is controlled by the transport of aerosols and their precursors from the troposphere to the stratosphere. The Transient Aerosol Record (TAR) experiment will explore the role of small- to moderate-magnitude volcanic eruptions, anthropogenic sulfur emissions, and transport processes over the period 1998–2012 and their role in the warming hiatus. Two further experiments will investigate the stratospheric sulfate aerosol evolution after major volcanic eruptions. The Historical Eruptions SO2 Emission Assessment (HErSEA) experiment will focus on the uncertainty in the initial emission of recent large-magnitude volcanic eruptions, while the Pinatubo Emulation in Multiple models (PoEMS) experiment will provide a comprehensive uncertainty analysis of the radiative forcing from the 1991 Mt Pinatubo eruption.


2021 ◽  
Author(s):  
Thomas Aubry ◽  
Anja Schmidt ◽  
Alix Harrow ◽  
Jeremy Walton ◽  
Jane Mulcahy ◽  
...  

<p>Reconstructions of volcanic aerosol forcing and its climatic impacts are undermined by uncertainties in both the models used to build these reconstructions as well as the proxy and observational records used to constrain those models. Reducing these uncertainties has been a priority and in particular, several modelling groups have developed interactive stratospheric aerosol models. Provided with an initial volcanic injection of sulfur dioxide, these models can interactively simulate the life cycle and optical properties of sulfate aerosols, and their effects on climate. In contrast, most climate models that took part in the Coupled Model Intercomparison Project Phase 5 and 6 (CMIP6) directly prescribe perturbations in atmospheric optical properties associated with an eruption. However, before the satellite era, the volcanic forcing dataset used for CMIP6 mostly relies on a relatively simple aerosol model and a volcanic sulfur inventory derived from ice-cores, both of which have substantial associated uncertainties.</p><p>In this study, we produced a new set of historical simulations using the UK Earth System Model UKESM1, with interactive stratospheric aerosol capability (referred to as interactive runs hereafter) instead of directly prescribing the CMIP6 volcanic forcing dataset as was done for CMIP6 (standard runs, hereafter). We used one of the most recent volcanic sulfur inventories as input for the interactive runs, in which aerosol properties are consistent with the model chemistry, microphysics and atmospheric components. We analyzed how the stratospheric aerosol optical depth, the radiative forcing and the climate response to volcanic eruptions differed between interactive and standard runs, and how these compare to observations and proxy records. In particular, we investigate in detail the differences in the response to the large-magnitude Krakatoa 1883 eruption between the two sets of runs. We also discuss differences for the 1979-2015 period where the forcing data in standard runs is directly constrained from satellite observations. Our results shed new light on uncertainties affecting the reconstruction of past volcanic forcing and highlight some of the benefits and disadvantages of using interactive stratospheric aerosol capabilities instead of a unique prescribed volcanic forcing dataset in CMIP’s historical runs.</p>


2018 ◽  
Author(s):  
Claudia Timmreck ◽  
Graham W. Mann ◽  
Valentina Aquila ◽  
Rene Hommel ◽  
Lindsay A. Lee ◽  
...  

Abstract. The Stratospheric Sulfur and its Role in Climate (SSiRC) interactive stratospheric aerosol model intercomparison project (ISA-MIP) explores uncertainties in the processes that connect volcanic emission of sulphur gas species and the radiative forcing associated with the resulting enhancement of the stratospheric aerosol layer. The central aim of ISA-MIP is to constrain and improve interactive stratospheric aerosol models and reduce uncertainties in the stratospheric aerosol forcing by comparing results of standardized model experiments with a range of observations. In this paper we present 4 co-ordinated inter-model experiments designed to investigate key processes which influence the formation and temporal development of stratospheric aerosol in different time periods of the observational record. The Background (BG) experiment will focus on microphysics and transport processes under volcanically quiescent conditions, when the stratospheric aerosol is controlled by the transport of aerosols and their precursors from the troposphere to the stratosphere. The Transient Aerosol Record (TAR) experiment will explore the role of small- to moderate-magnitude volcanic eruptions, anthropogenic sulphur emissions and transport processes over the period 1998–2012 and their role in the warming hiatus. Two further experiments will investigate the stratospheric sulphate aerosol evolution after major volcanic eruptions. The Historical Eruptions SO2 Emission Assessment (HErSEA) experiment will focus on the uncertainty in the initial emission of recent large-magnitude volcanic eruptions, while the Pinatubo Emulation in Multiple models (PoEMS) experiment will provide a comprehensive uncertainty analysis of the radiative forcing from the 1991 Mt. Pinatubo eruption.


2016 ◽  
Vol 9 (8) ◽  
pp. 2701-2719 ◽  
Author(s):  
Davide Zanchettin ◽  
Myriam Khodri ◽  
Claudia Timmreck ◽  
Matthew Toohey ◽  
Anja Schmidt ◽  
...  

Abstract. The enhancement of the stratospheric aerosol layer by volcanic eruptions induces a complex set of responses causing global and regional climate effects on a broad range of timescales. Uncertainties exist regarding the climatic response to strong volcanic forcing identified in coupled climate simulations that contributed to the fifth phase of the Coupled Model Intercomparison Project (CMIP5). In order to better understand the sources of these model diversities, the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP) has defined a coordinated set of idealized volcanic perturbation experiments to be carried out in alignment with the CMIP6 protocol. VolMIP provides a common stratospheric aerosol data set for each experiment to minimize differences in the applied volcanic forcing. It defines a set of initial conditions to assess how internal climate variability contributes to determining the response. VolMIP will assess to what extent volcanically forced responses of the coupled ocean–atmosphere system are robustly simulated by state-of-the-art coupled climate models and identify the causes that limit robust simulated behavior, especially differences in the treatment of physical processes. This paper illustrates the design of the idealized volcanic perturbation experiments in the VolMIP protocol and describes the common aerosol forcing input data sets to be used.


Author(s):  
Graham Mann ◽  
Juan Carlos Antuna Marrero ◽  
Amanda Maycock ◽  
Christine McKenna ◽  
Sarah Shallcross ◽  
...  

<p>The WCRP-SPARC initiative on stratospheric sulphur (SSiRC) has begun a new activity to recover past observational datasets of the stratospheric aerosol layer.</p><p>The data rescue activity aims to provide additional constraints for volcanic impacts on climate and is organised into three time-periods:</p><ol><li>The quiescent period prior to the major eruption 1963 Agung eruption,</li> <li>The period of strong volcanic activity during 1963-1969,</li> <li>The Jul-Dec 1991 period after Pinatubo when the SAGE-II signal was saturated.</li> </ol><p>A new page within the SSiRC website gives further information on the datasets within this activity ( http://www.sparc-ssirc.org  --> Activities --> Data Rescue).</p><p>In this presentation, we explain the 1963-1969 component of the data rescue, and compare the CMIP5 and CMIP6 volcanic aerosol datasets during this period, post-Agung interactive stratospheric aerosol model simulations and a preliminary analysis of 15-year global-mean surface temperature trends from CMIP6 historical integrations for 1950-1980.</p><p>The 1960s was a strongly volcanically active decade, with the major 1963 Agung eruption and tropical stratosphere-injecting eruptions in 1965 (Taal), 1966 (Awu) and 1968 (Fernandina) generating a prolonged period of strong natural surface cooling.</p><p>Less than a year after the Agung eruption, the first in-situ measurements of a major volcanic aerosol cloud were made with dust-sondes from Minneapolis measuring aerosol particle concentrations with 10 soundings between 1963 and 1965 (6 in 1963-4).</p><p>Global surveys with the U-2 aircraft were equipped with impactors to measure stratospheric aerosol particle size distribution and composition, for example detecting the presence of volcanic ash within the Agung volcanic plume.</p><p>Early ground-based active remote sensing measurements (lidar, searchlight) also measured the vertical profile of the Agung-enhanced stratospheric aerosol layer.</p><p>The main purpose of the SSiRC data rescue is to provide constraints for interactive stratospheric aerosol models, aligning with the ISA-MIP activity, which could potentially lead to new volcanic forcing datasets for climate models, ultimately thereby aiming to improve attribution of anthropogenic change and future projections.</p>


2020 ◽  
Author(s):  
Juan-Carlos Antuña-Marrero ◽  
Graham W. Mann ◽  
Philippe Keckhut ◽  
Sergey Avdyushin ◽  
Bruno Nardi ◽  
...  

Abstract. A key limitation of volcanic forcing datasets for the Pinatubo period, is the large uncertainty that remains with respect to the extent of the optical depth of the Pinatubo aerosol cloud in the first year after the eruption, the saturation of the SAGE-II instrument restricting it to only be able to measure the upper part of the aerosol cloud in the tropics. Here we report the recovery of stratospheric aerosol measurements from two ship-borne lidars, both of which measured the tropical reservoir of volcanic aerosol produced by the June 1991 Mount Pinatubo eruption. The lidars were on-board two Soviet vessels, each ship crossing the Atlantic, their measurement datasets providing unique observational transects of the Pinatubo cloud across the tropics from Europe to the Caribbean (~ 40° N to 8° N) from July to September 1991 (the Prof Zubov ship) and from Europe to south of the Equator (8° S to ~ 40° N) between January and February 1992 (the Prof Vize ship). Our philosophy with the data recovery is to follow the same algorithms and parameters appearing in the two peer-reviewed articles that presented these datasets in the same issue of GRL in 1993, and here we provide all 48 lidar soundings made from the Prof. Zubov, and 11 of the 20 conducted from the Prof. Vize, ensuring we have reproduced the aerosols backscatter and extinction values in the Figures of those two papers. These original approaches used thermodynamic properties from the CIRA-86 standard atmosphere to derive the molecular backscattering, vertically and temporally constant values applied for the aerosol backscatter to extinction ratio and the correction factor of the aerosols backscattering wavelength dependence. We demonstrate this initial validation of the recovered stratospheric aerosol extinction profiles, providing full details of each dataset in this paper's Supplement S1, the original text files of the backscatter ratio, the calculated aerosols backscatter and extinction profiles. We anticipate the data providing potential new observational case studies for modelling analyses, including a 1-week series of consecutive soundings (in September 1991) at the same location showing the progression of the entrainment of part of the Pinatubo plume into the upper troposphere and the formation of an associated cirrus cloud. The Zubov lidar dataset illustrates how the tropically confined Pinatubo aerosol cloud transformed from a highly heterogeneous vertical structure in August 1991, maximum aerosol extinction values around 19 km for the lower layer and 23–24 for the upper layer, to a more homogeneous and deeper reservoir of volcanic aerosol in September 1991. We encourage modelling groups to consider new analyses of the Pinatubo cloud, comparing to the recovered datasets, with the potential to increase our understanding of the evolution of the Pinatubo aerosol cloud and its effects. Data described in this work are available at https://doi.pangaea.de/10.1594/PANGAEA.912770 (Antuña-Marrero et al., 2020).


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