scholarly journals CCN characteristics during the Indian Summer Monsoon over a rain-shadow region

2020 ◽  
Author(s):  
Venugopalan Nair Jayachandran ◽  
Mercy Varghese ◽  
Palani Murugavel ◽  
Kiran S. Todekar ◽  
Shivdas P. Bankar ◽  
...  

Abstract. Continuous aerosol and Cloud Condensation Nuclei (CCN) measurements carried out at the ground observational facility situated in the rain-shadow region of the Indian sub-continent are illustrated. These observations were part of the Cloud-Aerosol Interaction Precipitation Enhancement EXperiment (CAIPEEX) during the Indian Summer Monsoon season (June to September) of 2018. Observations are classified as dry-continental (monsoon break) and wet-marine (monsoon active) according to air mass history. CCN concentrations measured for a range of supersaturations (0.2–1.2 %) are parameterized using Twomey's empirical relationship. CCN concentrations even at low (0.2 %) supersaturation (SS) were high (> 1,000 cm-3) during continental conditions associated with high black carbon (BC~2,000 ng m-3) and columnar aerosol loading. During the marine air mass conditions, CCN concentrations diminished to ~ 350 cm-3 at 0.3 % SS and low aerosol loading persisted (BC~900 ng m-3). High CCN activation fraction (AF) of ~ 0.55 (at 0.3 % SS) were observed before the monsoon rainfall, which reduced to ~ 0.15 during the monsoon and enhanced to ~ 0.32 after that. Mostly mono-modal aerosol number-size distribution (NSD) with a mean geometric mean diameter (GMD) of ~ 85 nm, with least (~ 9 %) contribution from nucleation mode (

2020 ◽  
Vol 20 (12) ◽  
pp. 7307-7334 ◽  
Author(s):  
Venugopalan Nair Jayachandran ◽  
Mercy Varghese ◽  
Palani Murugavel ◽  
Kiran S. Todekar ◽  
Shivdas P. Bankar ◽  
...  

Abstract. Continuous aerosol and cloud condensation nuclei (CCN) measurements carried out at the ground observational facility situated in the rain-shadow region of the Indian subcontinent are illustrated. These observations were part of the Cloud Aerosol Interaction Precipitation Enhancement Experiment (CAIPEEX) during the Indian summer monsoon season (June to September) of 2018. Observations are classified as dry–continental (monsoon break) and wet–marine (monsoon active) according to the air mass history. CCN concentrations measured for a range of supersaturations (0.2 %–1.2 %) are parameterized using Twomey's empirical relationship. CCN concentrations at low (0.2 %) supersaturation (SS) were high (>1000cm-3) during continental conditions and observed together with high black carbon (BC∼2000ngm-3) and columnar aerosol loading. During the marine air mass conditions, CCN concentrations diminished to ∼350cm-3 at 0.3 % SS and low aerosol loading persisted (BC∼800ngm-3). High CCN activation fraction (AF) of ≅0.55 (at 0.3 % SS) was observed before the monsoon rainfall, which reduced to ≅0.15 during the marine air mass and enhanced to ≅0.32 after that. There was mostly monomodal aerosol number size distribution (NSD) with a mean geometric mean diameter (GMD) of ≅85 nm, with least (≅9 %) contribution from nucleation mode (<30 nm) particles persisted before the monsoon, while multimode NSD with ≅19 % of nucleation mode particles was found during the marine air mass. Critical activation diameters (dcri) for 0.3 % SS were found to be about 72, 169, and 121 nm prior to, during, and after the marine conditions, respectively. The better association of CCN with aerosol absorption, and the concurrent accumulation mode particles during continental conditions, points to the possibility of aged (oxygenated) carbonaceous aerosols enhancing the CCN activity prior to the marine conditions. An enhancement in CCN concentrations and k values during the daytime along with absorption Ångström exponent was observed during the marine conditions. Best closure obtained using measured critical diameter and ammonium sulfate composition during continental conditions emphasizes the role of aged aerosols contributing to the accumulation mode, enhancing the CCN efficiency. The overestimation of CCN and less hygroscopicity of accumulation mode aerosols during the marine air mass indicate the role of size-dependent aerosol composition in CCN activity during the period.


2020 ◽  
Vol 20 (1) ◽  
pp. 561-576 ◽  
Author(s):  
Venugopalan Nair Jayachandran ◽  
Surendran Nair Suresh Babu ◽  
Aditya Vaishya ◽  
Mukunda M. Gogoi ◽  
Vijayakumar S. Nair ◽  
...  

Abstract. Concurrent measurements of the altitude profiles of the concentration of cloud condensation nuclei (CCN), as a function of supersaturation (ranging from 0.2 % to 1.0 %), and aerosol optical properties (scattering and absorption coefficients) were carried out aboard an instrumented aircraft across the Indo-Gangetic Plain (IGP) just prior to the onset of the Indian summer monsoon (ISM) of 2016. The experiment was conducted under the aegis of the combined South-West Asian Aerosol–Monsoon Interactions and Regional Aerosol Warming Experiment (SWAAMI–RAWEX) campaign. The measurements covered coastal, urban and arid environments. In general, the CCN concentration was highest in the central IGP, decreasing spatially from east to west above the planetary boundary layer (PBL), which is ∼1.5 km for the IGP during pre-monsoon period. Despite this, the CCN activation efficiency at 0.4 % supersaturation was, interestingly, the highest over the eastern IGP (∼72 %), followed by that in the west (∼61 %), and it was the least over the central IGP (∼24 %) within the PBL. In general, higher activation efficiency is noticed above the PBL than below it. The central IGP showed remarkably low CCN activation efficiency at all altitudes, which appears to be associated with high black carbon (BC) mass concentration there, indicating the role of anthropogenic sources in suppressing the CCN efficiency. These first-ever CCN measurements over the western IGP, encompassing “the Great Indian Desert” also known as “the Thar Desert”, showed high CCN efficiency, ∼61 % at 0.4 % supersaturation, indicating the hygroscopic nature of the dust. The vertical structure of CCN properties is found to be air mass dependent, with higher activation efficiency even over the central IGP during the prevalence of marine air mass. Wet scavenging associated with precipitation episodes seems to have reduced the CCN activation efficiency below cloud level. An empirical relation has emerged between the CCN concentration and the scattering aerosol index (AI), which would facilitate the prediction of CCN from aerosol optical properties.


2018 ◽  
Vol 35 (2) ◽  
pp. 218-223
Author(s):  
D. M. Chate ◽  
R. T. Waghmare ◽  
C. K. Jena ◽  
V. Gopalakrishnan ◽  
P. Murugavel ◽  
...  

2021 ◽  
pp. 105976
Author(s):  
V. Jayachandran ◽  
Sudarsan Bera ◽  
Shivdas P. Bankar ◽  
Neelam Malap ◽  
Mercy Varghese ◽  
...  

Author(s):  
Raghavendra Ashrit ◽  
S. Indira Rani ◽  
Sushant Kumar ◽  
S. Karunasagar ◽  
T. Arulalan ◽  
...  

MAUSAM ◽  
2021 ◽  
Vol 49 (2) ◽  
pp. 229-234
Author(s):  
V. THAPLIYAL ◽  
M. RAJEEVAN ◽  
S. R. PATIL

Sea surface temperature (SST) variations over the three key regions over equatorial Pacific, viz., Nino (1+2), Nino 3 and Nino 4 and their relationships with Indian summer monsoon rainfall have been examined in this study. On monthly scale, SST anomalies over the three key regions show an oscillatory type of lagged correlations with Indian monsoon rainfall, positive correlations almost one year before the monsoon season (CC's are of the order of 0.3) which gradually change to significant negative correlation peaking in September/October during/after the monsoon season. The variations on seasonal scale also exhibit the same pattern of monthly variations but more smooth in nature. Composites of similar monsoon years show that during deficient (excess) monsoon years SST anomalies over all the three regions have warmer (cooler) trend which starts about 6 months prior to monsoon season. Tendencies of SST anomalies from previous winter (DJF) to summer (MAM) seasons over Nino 3 and Nino 4 regions are better predictors than EI-Nino categories currently being used in IMD's operational LRF model. By using tendency of SST over EI- Nino -4 region, in place of the category of EI-Nino, the 16 parameter operational Power Regression Model of IMD has been modified. The new forecast model shows better reduction in the forecast error.


2016 ◽  
Author(s):  
Chandan Sarangi ◽  
Sachchida Nand Tripathi ◽  
Vijay P. Kanawade ◽  
Ilan Koren ◽  
D. Sivanand Pai

Abstract. Monsoonal rainfall is the primary source of surface water in India. Using 12 years of in-situ and satellite observations, we examined association of aerosol loading with cloud fraction, cloud top pressure, cloud top temperature, and daily surface rainfall over Indian summer monsoon region (ISMR). The analyses showed positive correlations between aerosol loading and cloud properties as well as rainfall. A decrease in outgoing longwave radiation and increase in reflected shortwave radiation at the top of the atmosphere with an increase in aerosol loading further supported a seminal role of aerosols on cloud systems. Significant perturbation in liquid- and ice-phase microphysics was also evident over ISMR. For the polluted cases, delay in the onset of collision-coalescence processes and enhancement in the condensation efficiency, allows for more condensate mass to be lifted up to the mixed-colder phases. This results in the higher mass concentration of bigger sized ice-phase hydrometeors and, therefore, implies that the delayed rain processes eventually lead to more surface rainfall. Numerical simulation of a typical rainfall event case over ISMR using spectral bin microphysical scheme coupled with Weather Research Forecasting (WRF-SBM) model was also performed. Simulated microphysics also illustrated the initial suppression of warm rain coupled with increase in updraft velocity under high aerosol loading leads to enhanced super-cooled liquid droplets above freezing level and ice-phase hydrometeors, resulting in increased accumulated surface rainfall. Thus, both observational and numerical analysis suggest that high aerosol loading may induce cloud invigoration and thereby increasing surface rainfall over the ISMR. While the meteorological variability influence the strength of the observed positive associations, our results suggest that the persistent aerosol-associated deepening of cloud systems and intensification of surface rain amounts was applicable to all the meteorological sub-regimes over the ISMR. Hence, we believe that these results provide a step forward in our ability to address aerosol-cloud-rainfall associations based on satellite observations over ISMR.


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