scholarly journals Impacts of historical climate and land cover changes on tropospheric ozone air quality and public health in East Asia over 1980–2010

2015 ◽  
Vol 15 (10) ◽  
pp. 14111-14139 ◽  
Author(s):  
Y. Fu ◽  
A. P. K. Tai

Abstract. Understanding how historical climate and land cover changes have affected tropospheric ozone in East Asia would help constrain the large uncertainties associated with future East Asian air quality projections. We perform a series of simulations using a global chemical transport model driven by assimilated meteorological data and a suite of land cover and land use data to examine the public health effects associated with changes in climate, land cover, land use, and anthropogenic emissions over the past 30 years (1980–2010) in East Asia. We find that over 1980–2010 land cover change alone could lead to a decrease in summertime surface ozone by up to 4 ppbv in East Asia and ~2000 fewer ozone-related premature deaths per year, driven mostly by enhanced dry deposition resulting from climate- and CO2-induced increase in vegetation density, which more than offsets the effect of reduced isoprene emission arising from cropland expansion. Over the same period, climate change alone could lead to an increase in summertime ozone by 2–10 ppbv in most regions of East Asia and ~6000 more premature deaths annually, mostly attributable to warming. The combined impacts (−2 to +12 ppbv) show that while the effect of climate change is more pronounced, land cover change could offset part of the climate effect and lead to a previously unknown public health benefit. While the changes in anthropogenic emissions remain the largest contributor to deteriorating ozone air quality in East Asia over the past 30 years, we show that climate change and land cover changes could lead to a substantial modification of ozone levels, and thus should come into consideration when formulating future air quality management strategies. We also show that the sensitivity of surface ozone to land cover change is more dependent on dry deposition than isoprene emission in most of East Asia, leading to ozone responses that are quite distinct from that in North America, where most ozone-vegetation sensitivity studies to date have been conducted.

2015 ◽  
Vol 15 (17) ◽  
pp. 10093-10106 ◽  
Author(s):  
Y. Fu ◽  
A. P. K. Tai

Abstract. Understanding how historical climate and land cover changes have affected tropospheric ozone in East Asia would help constrain the large uncertainties associated with future East Asian air quality projections. We perform a series of simulations using a global chemical transport model driven by assimilated meteorological data and a suite of land cover and land use data to examine the public health effects associated with changes in climate, land cover, land use, and anthropogenic emissions between the 5-year periods 1981–1985 and 2007–2011 in East Asia. We find that between these two periods land cover change alone could lead to a decrease in summertime surface ozone by up to 4 ppbv in East Asia and ~ 2000 fewer ozone-related premature deaths per year, driven mostly by enhanced dry deposition resulting from climate- and CO2-induced increase in vegetation density, which more than offsets the effect of reduced isoprene emission arising from cropland expansion. Climate change alone could lead to an increase in summertime ozone by 2–10 ppbv in most regions of East Asia and ~ 6000 more premature deaths annually, mostly attributable to warming. The combined impacts (−2 to +12 ppbv) show that while the effect of climate change is more pronounced, land cover change could offset part of the climate effect and lead to a previously unknown public health benefit. While the changes in anthropogenic emissions remain the largest contributor to deteriorating ozone air quality in East Asia over the past 30 years, we show that climate change and land cover changes could lead to a substantial modification of ozone levels, and thus should come into consideration when formulating future air quality management strategies. We also show that the sensitivity of surface ozone to land cover change is more dependent on dry deposition than on isoprene emission in most of East Asia, leading to ozone responses that are quite distinct from that in North America, where most ozone-vegetation sensitivity studies to date have been conducted.


Author(s):  
Philip Mzava ◽  
Patrick Valimba ◽  
Joel Nobert

Abstract Over the past half-century, the risk of urban flooding in Dar es Salaam has increased due to changes in land cover coupled with climatic changes. This paper aimed to quantify the impacts of climate and land-cover changes on the magnitudes and frequencies of flood runoffs in urban Dar es Salaam, Tanzania. A calibrated and validated SWAT rainfall-runoff model was used to generate flood hydrographs for the period 1969–2050 using historical rainfall data and projected rainfall based on the CORDEX-Africa regional climate model. Results showed that climate change has a greater impact on change in peak flows than land-cover change when the two are treated separately in theory. It was observed that, in the past, the probability of occurrence of urban flooding in the study area was likely to be increased up to 1.5-fold by climate change relative to land-cover change. In the future, this figure is estimated to decrease to 1.1-fold. The coupled effects of climate and land-cover changes cause a much bigger impact on change in peak flows than any separate scenario; this scenario represents the actual scenario on the ground. From the combined effects of climate and land-cover changes, the magnitudes of mean peak flows were determined to increase between 34.4 and 58.6% in the future relative to the past. However, the change in peak flows from combined effects of climate and land-cover changes will decrease by 36.3% in the future relative to the past; owing to the lesser variations in climate and land-cover changes in the future compared with those of the past.


2015 ◽  
Vol 15 (21) ◽  
pp. 31385-31432
Author(s):  
Y. H. Lee ◽  
D. T. Shindell ◽  
G. Faluvegi ◽  
R. W. Pinder

Abstract. We have investigated how future air quality and climate change are influenced by the US air quality regulations that existed or were proposed in 2013 and a hypothetical climate mitigation policy that reduces 2050 CO2 emissions to be 50 % below 2005 emissions. Using NASA GISS ModelE2, we look at the impacts in year 2030 and 2055. The US energy-sector emissions are from the GLIMPSE project (GEOS-Chem LIDORT Integrated with MARKAL for the Purpose of Scenario Exploration), and other US emissions and the rest of the world emissions are based on the RCP4.5 scenario. The US air quality regulations are projected to have a strong beneficial impact on US air quality and public health in the future but result in positive radiative forcing. Surface PM2.5 is reduced by ~ 2 μg m−3 on average over the US, and surface ozone by ~ 8 ppbv. The improved air quality prevents about 91 400 premature deaths in the US, mainly due to the PM2.5 reduction (~ 74 200 lives saved). The air quality regulations reduces the light-reflecting aerosols (i.e., sulfate and organic matter) more than the light-absorbing species (i.e., black carbon and ozone), leading a strong positive radiative forcing (RF) by both aerosols direct and indirect forcing: total RF is ~ 0.04 W m−2 over the globe; ~ 0.8 W m−2 over the US. Under the hypothetical climate policy, future US energy relies less on coal and thus SO2 emissions are noticeably reduced. This provides air quality co-benefits, but it leads to climate dis-benefits over the US. In 2055, the US mean total RF is +0.22 W m−2 due to positive aerosol direct and indirect forcing, while the global mean total RF is −0.06 W m−2 due to the dominant negative CO2 RF (instantaneous RF). To achieve a regional-scale climate benefit via a climate policy, it is critical (1) to have multi-national efforts to reduce GHGs emissions and (2) to target emission reduction of light-absorbing species (e.g., BC and O3) on top of long-lived species. The latter is very desirable as the resulting climate benefit occurs faster and provides co-benefits to air quality and public health.


2016 ◽  
Author(s):  
Yu Fu ◽  
Amos P. K. Tai ◽  
Hong Liao

Abstract. To examine the effects of changes in climate, land cover and land use (LCLU), and anthropogenic emissions on fine particulate matter (PM2.5) between the 5-year periods 1981–1985 and 2007–2011 in East Asia, we perform a series of simulations using a global chemical transport model (GEOS-Chem) driven by assimilated meteorological data and a suite of land cover and land use data. Our results indicate that climate change alone could lead to a decrease in wintertime PM2.5 concentration by 4.0–12.0 μg m−3 in northern China, but an increase in summertime PM2.5 by 6.0–8.0 μg m−3 in those regions. These changes are attributable to the changing chemistry and transport of all PM2.5 components driven by long-term trends in temperature, wind speed and mixing depth. The concentration of secondary organic aerosol (SOA) is simulated to increase by 0.2–0.8 μg m−3 in both summer and winter in most regions of East Asia due to climate change alone, mostly reflecting higher biogenic volatile organic compound (VOC) emissions under warming. The impacts of LCLU change alone on PM2.5 (−2.1 to +1.3 μg m−3) are smaller than that of climate change, but among the various components the sensitivity of SOA and thus organic carbon to LCLU change (−0.4 to +1.2 μg m−3) is quite significant especially in summer, which is driven mostly by changes in biogenic VOC emissions following cropland expansion and changing vegetation density. The combined impacts show that while the effect of climate change on PM2.5 air quality is more pronounced, LCLU change could offset part of the climate effect in some regions but exacerbate it in others. As a result of both climate and LCLU changes combined, PM2.5 levels are estimated to change by −12.0 to +12.0 μg m−3 across East Asia between the two periods. Changes in anthropogenic emissions remain the largest contributor to deteriorating PM2.5 air quality in East Asia during the study period, but climate and LCLU changes could lead to a substantial modification of PM2.5 levels.


2016 ◽  
Vol 16 (16) ◽  
pp. 10369-10383 ◽  
Author(s):  
Yu Fu ◽  
Amos P. K. Tai ◽  
Hong Liao

Abstract. To examine the effects of changes in climate, land cover and land use (LCLU), and anthropogenic emissions on fine particulate matter (PM2.5) between the 5-year periods 1981–1985 and 2007–2011 in East Asia, we perform a series of simulations using a global chemical transport model (GEOS-Chem) driven by assimilated meteorological data and a suite of land cover and land use data. Our results indicate that climate change alone could lead to a decrease in wintertime PM2.5 concentration by 4.0–12.0 µg m−3 in northern China, but to an increase in summertime PM2.5 by 6.0–8.0 µg m−3 in those regions. These changes are attributable to the changing chemistry and transport of all PM2.5 components driven by long-term trends in temperature, wind speed and mixing depth. The concentration of secondary organic aerosol (SOA) is simulated to increase by 0.2–0.8 µg m−3 in both summer and winter in most regions of East Asia due to climate change alone, mostly reflecting higher biogenic volatile organic compound (VOC) emissions under warming. The impacts of LCLU change alone on PM2.5 (−2.1 to +1.3 µg m−3) are smaller than that of climate change, but among the various components the sensitivity of SOA and thus organic carbon to LCLU change (−0.4 to +1.2 µg m−3) is quite significant especially in summer, which is driven mostly by changes in biogenic VOC emissions following cropland expansion and changing vegetation density. The combined impacts show that while the effect of climate change on PM2.5 air quality is more pronounced, LCLU change could offset part of the climate effect in some regions but exacerbate it in others. As a result of both climate and LCLU changes combined, PM2.5 levels are estimated to change by −12.0 to +12.0 µg m−3 across East Asia between the two periods. Changes in anthropogenic emissions remain the largest contributor to deteriorating PM2.5 air quality in East Asia during the study period, but climate and LCLU changes could lead to a substantial modification of PM2.5 levels.


2015 ◽  
Vol 15 (13) ◽  
pp. 18459-18485
Author(s):  
T. Verbeke ◽  
J. Lathière ◽  
S. Szopa ◽  
N. de Noblet-Ducoudré

Abstract. Dry deposition is a key component of surface–atmosphere exchange of compounds, acting as a sink for several chemical species. Meteorological factors, chemical properties of the trace gas considered and land surface properties are strong drivers of dry deposition efficiency and variability. Under both climatic and anthropogenic pressure, the vegetation distribution over the Earth has been changing a lot over the past centuries, and could be significantly altered in the future. In this study, we perform a modeling investigation of the potential impact of land-cover changes between present-day (2006) and the future (2050) on dry deposition rates, with special interest for ozone (O3) and nitric acid vapor (HNO3), two compounds which are characterized by very different physico-chemical properties. The 3-D chemistry transport model LMDz-INCA is used, considering changes in vegetation distribution based on the three future projections RCPs 2.6, 4.5 and 8.5. The 2050 RCP 8.5 vegetation distribution leads to a rise up to 7 % (+0.02 cm s−1) in VdO3 and a decrease of −0.06 cm s−1 in VdHNO3 relative to the present day values in tropical Africa, and up to +18 and −15 % respectively in Australia. When taking into account the RCP 4.5 scenario, which shows dramatic land cover change in Eurasia, VdHNO3 increases by up to 20 % (annual-mean value) and reduces VdO3 by the same magnitude in this region. When analyzing the impact of dry deposition change on atmospheric chemical composition, our model calculates that the effect is lower than 1 ppb on annual mean surface ozone concentration, for both for the RCP8.5 and RCP2.6 scenarios. The impact on HNO3 surface concentrations is more disparate between the two scenarios, regarding the spatial repartition of effects. In the case of the RCP 4.5 scenario, a significant increase of the surface O3 concentration reaching locally up to 5 ppb (+5 %) is calculated on average during the June–August period. This scenario induces also an increase of HNO3 deposited flux exceeding locally 10 % for monthly values. Comparing the impact of land-cover change to the impact of climate change, considering a 0.93 °C increase of global temperature, on dry deposition velocities, we estimate that the strongest increase over lands occurs in the North Hemisphere during winter especially in Eurasia, by +50 % (+0.07 cm s−1) for VdO3 and +100 % (+0.9 cm s−1) for VdHNO3. However, different regions are affected by both changes, with climate change impact on deposition characterized by a latitudinal gradient, while the land-cover change impact is much more heterogeneous depending on vegetation distribution modification described in the future RCP scenarios. The impact of long-term land-cover changes on dry deposition is shown to be non-negligible and should be therefore considered in biosphere-atmospheric chemistry interaction studies in order to have a fully consistent picture.


2021 ◽  
Vol 21 (21) ◽  
pp. 16479-16497
Author(s):  
Anthony Y. H. Wong ◽  
Jeffrey A. Geddes

Abstract. Our work explores the impact of two important dimensions of land system changes, land use and land cover change (LULCC) as well as direct agricultural reactive nitrogen (Nr) emissions from soils, on ozone (O3) and fine particulate matter (PM2.5) in terms of air quality over contemporary (1992 to 2014) timescales. We account for LULCC and agricultural Nr emissions changes with consistent remote sensing products and new global emission inventories respectively estimating their impacts on global surface O3 and PM2.5 concentrations as well as Nr deposition using the GEOS-Chem global chemical transport model. Over this time period, our model results show that agricultural Nr emission changes cause a reduction of annual mean PM2.5 levels over Europe and northern Asia (up to −2.1 µg m−3) while increasing PM2.5 levels in India, China and the eastern US (up to +3.5 µg m−3). Land cover changes induce small reductions in PM2.5 (up to −0.7 µg m−3) over Amazonia, China and India due to reduced biogenic volatile organic compound (BVOC) emissions and enhanced deposition of aerosol precursor gases (e.g., NO2, SO2). Agricultural Nr emission changes only lead to minor changes (up to ±0.6 ppbv) in annual mean surface O3 levels, mainly over China, India and Myanmar. Meanwhile, our model result suggests a stronger impact of LULCC on surface O3 over the time period across South America; the combination of changes in dry deposition and isoprene emissions results in −0.8 to +1.2 ppbv surface ozone changes. The enhancement of dry deposition reduces the surface ozone level (up to −1 ppbv) over southern China, the eastern US and central Africa. The enhancement of soil NO emission due to crop expansion also contributes to surface ozone changes (up to +0.6 ppbv) over sub-Saharan Africa. In certain regions, the combined effects of LULCC and agricultural Nr emission changes on O3 and PM2.5 air quality can be comparable (>20 %) to anthropogenic emission changes over the same time period. Finally, we calculate that the increase in global agricultural Nr emissions leads to a net increase in global land area (+3.67×106km2) that potentially faces exceedance of the critical Nr load (>5 kg N ha−1 yr−1). Our result demonstrates the impacts of contemporary LULCC and agricultural Nr emission changes on PM2.5 and O3 in terms of air quality, as well as the importance of land system changes for air quality over multidecadal timescales.


2014 ◽  
Vol 46 (2) ◽  
pp. 138 ◽  
Author(s):  
Dedi Hermon

ἀe purpose of this study was to analyze the trend of climate change through changes in the elements of Green House Gases (GHGs),   includes the trend of CO2, N2O, and CH4. ἀe change of the  extreme rainfall and temperature  indices due to land cover change into developed area in Padang. IdentiḀcation and analysis trends of climate change and extreme climatic events were analyzed by using RclimDex the Expert Team for Climate Change Detection and Indices (ETCCDMI) technique. Where as the analysis and interpretation of  land cover changes  into developed area used Landsat TM 5 and Landsat 1985 7 ETM +  of 2011 by ERDAS 9.2 GIS with the supervised classiḀcation method and GIS Matrix. ἀe results of the study provide informations of land cover changes into developed area at forest land  (11,758.9 ha), shrub (3,337.3 ha), rice Ḁelds (5,977.1 ha), and garden (5,872.4 ha). It has an implication on increasing of  the ele-ments of GHGs concentration such as CO2 (14,1 ppm), N2O (5,4 ppb) and CH4 (24,8 ppb). ἀis condition lead to an extreme temperature and presipitation indexs trends in Padang.


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