scholarly journals The roles of dynamical variability and aerosols in cirrus cloud formation

2003 ◽  
Vol 3 (2) ◽  
pp. 1415-1451 ◽  
Author(s):  
B. Kärcher ◽  
J. Ström

Abstract. The probability of occurrence of ice crystal number densities in young cirrus clouds is examined based on airborne measurements. The observations have been carried out at midlatitudes in both hemispheres at equivalent latitudes (~52–55° N/S) during the same season (local autumn in 2000). The in situ measurements considered in the present study include temperatures, vertical velocities, and ice crystal concentrations, the latter determined with high precision and accuracy using a counterflow virtual impactor. Most young cirrus clouds typically contain high number densities (1–10 cm−3) of small (diameter <20 μm) ice crystals. This mode dominates the probability distributions in both hemispheres and is shown to be caused by rapid cooling rates associated with updraft speeds in the range 10–100 cm s-1. A second mode containing larger crystals extends from ~1 cm−3 to low concentrations close to the detection threshold (~3×104cm−3) and is associated with lower updraft speeds. Results of a statistical analysis provide compelling evidence that the dynamical variability of vertical air motions on the mesoscale is the key factor determining the observed probability distributions of pristine ice crystal concentrations in cirrus. Other factors considered are variations of temperature as well as size, number, and ice nucleation thresholds of the freezing aerosol particles. The variability in vertical velocities is likely caused by atmospheric waves. Inasmuch as gravity waves are widespread, mesoscale variability in vertical velocities can be viewed as a universa  feature of young cirrus clouds. Large-scale models that do not account for this subgrid-scale variability yield erroneous predictions of the variability of basic cirrus cloud properties. Climate change may bring about changes in the global distribution of updraft speeds, mean air temperatures, and aerosol properties. As shown in this work, these changes could significantly modify the probability distribution of cirrus ice crystal concentrations. This study emphasizes the key role of vertical velocities and mesoscale variability in vertical velocities in controlling cirrus properties. The results suggest that, in any effort to ascribe cause to trends of cirrus cloud properties, a careful evaluation of dynamical changes in cloud formation should be done before conclusions regarding the role of other anthropogenic factors, such as changes in aerosol composition, are made.

2003 ◽  
Vol 3 (3) ◽  
pp. 823-838 ◽  
Author(s):  
B. Kärcher ◽  
J. Ström

Abstract. The probability of occurrence of ice crystal number densities in young cirrus clouds is examined based on airborne measurements. The observations have been carried out at midlatitudes in both hemispheres at equivalent latitudes (52-55°N/S) during the same season (local autumn in 2000). The in situ measurements considered in the present study include temperatures, vertical velocities, and total ice crystal concentrations, the latter determined with high precision and accuracy using a counterflow virtual impactor. Most young cirrus clouds typically contain high number densities (1-10 cm-3) of small (diameter <20 mm) ice crystals. This mode dominates the probability distributions and is shown to be caused by rapid cooling rates associated with updraft speeds in the range 10-100 cm s-1. A second mode containing larger crystals extends from ~1 cm-3 to low concentrations close to the detection threshold (~3 x 10-4 cm-3) and could be associated with lower updraft speeds. Results of a statistical analysis provide compelling evidence that the dynamical variability of vertical air motions on the mesoscale is the key factor determining the observed probability distributions of pristine ice crystal concentrations in cirrus. Other factors considered are changes of temperature as well as size, number, and ice nucleation thresholds of the freezing aerosol particles. The variability in vertical velocities is caused by atmospheric gravity waves leading to small-scale temperature fluctuations. Inasmuch as gravity waves are widespread, mesoscale variability in vertical velocities can be viewed as a universal feature of young cirrus clouds. Large-scale models that do not account for this subgrid-scale variability yield erroneous predictions of the variability of basic cirrus cloud properties. Climate change may bring about changes in the global distribution of updraft speeds, mean air temperatures, and aerosol properties. As shown in this work, these changes could significantly modify the probability distribution of cirrus ice crystal concentrations. This study emphasizes the key role of vertical velocities and mesoscale variability in vertical velocities in controlling cirrus properties. The results suggest that, in any effort to ascribe cause to trends of cirrus cloud properties, a careful evaluation of dynamical changes in cloud formation should be done before conclusions regarding the role of other anthropogenic factors, such as changes in aerosol composition, are made.


2010 ◽  
Vol 10 (12) ◽  
pp. 5449-5474 ◽  
Author(s):  
M. Wang ◽  
J. E. Penner

Abstract. A statistical cirrus cloud scheme that accounts for mesoscale temperature perturbations is implemented in a coupled aerosol and atmospheric circulation model to better represent both subgrid-scale supersaturation and cloud formation. This new scheme treats the effects of aerosol on cloud formation and ice freezing in an improved manner, and both homogeneous freezing and heterogeneous freezing are included. The scheme is able to better simulate the observed probability distribution of relative humidity compared to the scheme that was implemented in an older version of the model. Heterogeneous ice nuclei (IN) are shown to decrease the frequency of occurrence of supersaturation, and improve the comparison with observations at 192 hPa. Homogeneous freezing alone can not reproduce observed ice crystal number concentrations at low temperatures (<205 K), but the addition of heterogeneous IN improves the comparison somewhat. Increases in heterogeneous IN affect both high level cirrus clouds and low level liquid clouds. Increases in cirrus clouds lead to a more cloudy and moist lower troposphere with less precipitation, effects which we associate with the decreased convective activity. The change in the net cloud forcing is not very sensitive to the change in ice crystal concentrations, but the change in the net radiative flux at the top of the atmosphere is still large because of changes in water vapor. Changes in the magnitude of the assumed mesoscale temperature perturbations by 25% alter the ice crystal number concentrations and the net radiative fluxes by an amount that is comparable to that from a factor of 10 change in the heterogeneous IN number concentrations. Further improvements on the representation of mesoscale temperature perturbations, heterogeneous IN and the competition between homogeneous freezing and heterogeneous freezing are needed.


2021 ◽  
Vol 21 (19) ◽  
pp. 14573-14590
Author(s):  
Qiang Li ◽  
Silke Groß

Abstract. By inducing linear contrails and contrail cirrus, air traffic has a main impact on the ice cloud coverage and occurrence. During the COVID-19 pandemic, civil air traffic over Europe was significantly reduced, in March and April 2020, to about 80 % compared to the year before. This unique situation allows us to study the effect of air traffic on cirrus clouds. This work investigates, based on satellite lidar measurements, if and how cirrus cloud properties and occurrence changed over Europe in the course of COVID-19. Cirrus cloud properties are analyzed for different years between 2014 and 2019, which showed similar meteorological conditions for the month of April as in 2020. The meteorological conditions for March, however, were warmer and drier in 2020 than the previous years. The average thickness of cirrus clouds was reduced to 1.18 km in March 2020 compared to a value of 1.40 km under normal conditions, which is stronger than expected from the aviation reduction due to the less favorable meteorology for ice cloud formation. While the April results in 2020 were only slightly reduced, with an average thickness of 70 m thinner than the composite mean of the previous 6 years. Comparing the different years shows that the cirrus cloud occurrence was reduced by about 17 %–30 %, with smaller cloud thicknesses found in 2020 for both months. In addition, the cirrus clouds measured in 2020 possess smaller values of the particle linear depolarization ratio (PLDR) than the previous years at a high significance level for both months, especially at colder temperatures (T<-50 ∘C). The same analyses are extended to the observations over the USA and China. Besides the regional discrimination of cirrus clouds, we reach the final conclusion that cirrus clouds show significant changes in PLDR in both March and April over Europe, no changes in both months over China, and significant changes only in April over the USA.


2018 ◽  
Vol 18 (9) ◽  
pp. 6157-6169 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Johannes Quaas ◽  
Tom Goren ◽  
Daniel Klocke ◽  
Matthias Brueck

Abstract. Cirrus clouds play an important role in determining the radiation budget of the earth, but many of their properties remain uncertain, particularly their response to aerosol variations and to warming. Part of the reason for this uncertainty is the dependence of cirrus cloud properties on the cloud formation mechanism, which itself is strongly dependent on the local meteorological conditions. In this work, a classification system (Identification and Classification of Cirrus or IC-CIR) is introduced to identify cirrus clouds by the cloud formation mechanism. Using reanalysis and satellite data, cirrus clouds are separated into four main types: orographic, frontal, convective and synoptic. Through a comparison to convection-permitting model simulations and back-trajectory-based analysis, it is shown that these observation-based regimes can provide extra information on the cloud-scale updraughts and the frequency of occurrence of liquid-origin ice, with the convective regime having higher updraughts and a greater occurrence of liquid-origin ice compared to the synoptic regimes. Despite having different cloud formation mechanisms, the radiative properties of the regimes are not distinct, indicating that retrieved cloud properties alone are insufficient to completely describe them. This classification is designed to be easily implemented in GCMs, helping improve future model–observation comparisons and leading to improved parametrisations of cirrus cloud processes.


2014 ◽  
Vol 14 (12) ◽  
pp. 17635-17679 ◽  
Author(s):  
X. Shi ◽  
X. Liu ◽  
K. Zhang

Abstract. In order to improve the treatment of ice nucleation in a more realistic manner in the Community Atmospheric Model version 5.3 (CAM5.3), the effects of preexisting ice crystals on ice nucleation in cirrus clouds are considered. In addition, by considering the in-cloud variability in ice saturation ratio, homogeneous nucleation takes place spatially only in a portion of cirrus cloud rather than in the whole area of cirrus cloud. With these improvements, the two unphysical limiters used in the representation of ice nucleation are removed. Compared to observations, the ice number concentrations and the probability distributions of ice number concentration are both improved with the updated treatment. The preexisting ice crystals significantly reduce ice number concentrations in cirrus clouds, especially at mid- to high latitudes in the upper troposphere (by a factor of ~10). Furthermore, the contribution of heterogeneous ice nucleation to cirrus ice crystal number increases considerably. Besides the default ice nucleation parameterization of Liu and Penner (2005, hereafter LP) in CAM5.3, two other ice nucleation parameterizations of Barahona and Nenes (2009, hereafter BN) and Kärcher et al. (2006, hereafter KL) are implemented in CAM5.3 for the comparison. In-cloud ice crystal number concentration, percentage contribution from heterogeneous ice nucleation to total ice crystal number, and preexisting ice effects simulated by the three ice nucleation parameterizations have similar patterns in the simulations with present-day aerosol emissions. However, the change (present-day minus pre-industrial times) in global annual mean column ice number concentration from the KL parameterization (3.24 × 106 m−2) is obviously less than that from the LP (8.46 × 106 m−2) and BN (5.62 × 106 m−2) parameterizations. As a result, experiment using the KL parameterization predicts a much smaller anthropogenic aerosol longwave indirect forcing (0.24 W m−2) than that using the LP (0.46 W m−2) and BN (0.39 W m−2) parameterizations.


2005 ◽  
Vol 62 (7) ◽  
pp. 2274-2283 ◽  
Author(s):  
I. Schlimme ◽  
A. Macke ◽  
J. Reichardt

Abstract The solar radiative properties of cirrus clouds depend on ice particle shape, size, and orientation, as well as on the spatial cloud structure. Radiation schemes in atmospheric circulation models rely on estimates of cloud optical thickness only. In the present work, a Monte Carlo radiative transfer code is applied to various cirrus cloud scenarios to obtain the radiative response of uncertainties in the above-mentioned microphysical and spatial cloud properties (except orientation). First, plane-parallel homogeneous (0D) clouds with different crystal shapes (hexagonal columns, irregular polycrystals) and 114 different size distributions have been considered. The resulting variabilities in the solar radiative fluxes are in the order of a few percent for the reflected and about 1% for the diffusely transmitted fluxes. Largest variabilities in the order of 10% to 30% are found for the solar broadband absorptance. However, these variabilities are smaller than the flux differences caused by the choice of ice particle geometries. The influence of cloud inhomogeneities on the radiative fluxes has been examined with the help of time series of Raman lidar extinction coefficient profiles as input for the radiative transfer calculations. Significant differences between results for inhomogeneous and plane-parallel clouds were found. These differences are in the same order of magnitude as those arising from using extremely different crystal shapes for the radiative transfer calculations. From this sensitivity study, the ranking of cirrus cloud properties according to their importance in solar broadband radiative transfer is optical thickness, ice crystal shape, ice particle size, and spatial structure.


Cirrus ◽  
2002 ◽  
Author(s):  
David O’C. Starr ◽  
Markus Quante

Advancement in the understanding of cirrus clouds and their life cycle comes through symbiotic use of models, observations, and related concepts (fig. 18.1). Models of cirrus clouds represent an integration of our knowledge of cirrus cloud properties and processes. They provide a capacity to extend knowledge and enhance understanding in ways that complement existing observational capabilities. Models can be used to develop new theories, such as parameterizations, and focus science issues and observational requirements and developments. For example, early model results of Starr and Cox (1985a) and Starr (1987b) predicted that fine cellular structure (~lkm or less) would be found in the upper part of extended stratiform cirrus clouds. This prediction was confirmed when high-frequency sensors were deployed both for active remote sensing (Sassen et al. 1990a, 1995) and later for in-situ measurements (Quante and Brown 1992; Gultepe et al. 1995; Quante et al. 1996). Sampling rates of 10Hz, or better, are now accepted as a minimum requirement for resolving cirrus cloud internal structure and circulation where 1-Hz or coarser measurements were previously used. Similarly, discrepancies between observed cloud radiative properties and calculations (theory) based on corresponding in-situ observations of cloud microphysical properties (Sassen et al. 1990b) led to the development of improved observing capabilities for small ice crystals (Arnott et al. 1994; Miloshevich and Heymsfield 1997; Lawson et al. 1998). Such sensors are now regarded as part of the standard complement when doing in-situ microphysical measurements in cirrus. At the same time, observations are absolutely essential in developing and evaluating cloud models. No cloud modeler wants to apply a model or theory too far beyond the limits of what can be observationally confirmed, at least in gross terms. The third aspect of this triad is concepts. Although models and observations can lead to predictions or diagnosis of unexpected relationships, they are each limited by the concepts that were used in their design and/or implementation. In the end, new concepts arising from analogy to other phenomena and/or from synergistic integration of existing knowledge can lead to new understanding, new models, new instruments, and new sampling strategies (fig. 18.1). Chapter 17 focuses on observations of internal cloud circulation and structure.


2018 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Odran Sourdeval ◽  
Johannes Quaas ◽  
Julien Delanoë ◽  
Philipp Kühne

Abstract. The ice crystal number concentration (Ni) is a key property of ice clouds, both radiatively and microphysically. However, due to sparse in-situ measurements of ice cloud properties, the controls on the Ni have remained difficult to determine. As more advanced treatments of ice clouds are included in global models, it is becoming increasingly necessary to develop strong observational constraints on the processes involved. This work uses the DARDAR-LIM Ni retrieval described in part one to investigate the controls of the Ni at a global scale. The retrieved clouds are separated by type. The effects of temperature, proxies for in-cloud updraught and aerosol concentrations are investigated. Variations in the cloud top Ni (Ni(top)) consistent with both homogeneous and heterogeneous nucleation are observed and along with a possible role of aerosol both increasing and decreasing the Ni(top) depending on the prevailing meteorological situation. Away from the cloud top, the Ni displays a different sensitivity to these controlling factors, providing a possible explanation to the low Ni sensitivity to temperature and INP observed in previous in-situ studies. This satellite dataset provides a new way of investigating the response of cloud properties to meteorological and aerosol controls. The results presented in this work increase our confidence in the retrieved Ni and will form the basis for further study into the processes influencing ice and mixed phase clouds.


2013 ◽  
Vol 6 (2) ◽  
pp. 4087-4121
Author(s):  
E. G. Larroza ◽  
W. M. Nakaema ◽  
R. Bourayou ◽  
C. Hoareau ◽  
E. Landulfo ◽  
...  

Abstract. In the present study, a methodology to calculate lidar ratios for distinct cirrus clouds has been implemented for a site located in the Southern Hemisphere. The cirrus cloud lidar data processing has been developed to consider a large cloud variability with the final aim of cirrus cloud monitoring through a robust retrieval process. Among the many features lidar systems can extract for cirrus detection, we highlight: cloud geometrical information and extinction-to-backscatter ratio (also called lidar ratio – LR). LR's can, in general, provide important information on cirrus cloud microphysics due to the presence of ice crystals and their properties such as shape, size, composition and orientation of particles and their effect on LR values. Conditions for LR calculations and their resulting uncertainty have been improved as their analysis requires identifying cirrus cloud stationary periods through the use of a specific statistical approach well-established in the literature and employed here with good results, allowing for the study of specific cases with multi-layer cirrus cloud occurrence. The results from the measurements taken in the region of the Metropolitan City of São Paulo – MSP have been used to implement and test the methodology developed herein. In addition to the geometrical parameters extracted, improved values of LR's were calculated and showed significantly different values for the different layers inspected, varying between 19 ± 01 sr and 74 ± 13 sr. This large value interval allowed us to indirectly verify the presence of different ice crystal sizes and shapes and those associated with different air mass sources for the cirrus cloud formation.


2013 ◽  
Vol 13 (14) ◽  
pp. 6951-6963 ◽  
Author(s):  
C. Hoareau ◽  
P. Keckhut ◽  
V. Noel ◽  
H. Chepfer ◽  
J.-L. Baray

Abstract. This study provides an analysis of cirrus cloud properties at midlatitude in the southern part of France from ground-based and spaceborne lidars. A climatology of cirrus cloud properties and their evolution over more than 12 yr is presented and compared to other mid-latitude climatological studies. Cirrus clouds occur ~37% of the total observation time and remain quasi-constant across seasons with a variation within ~5% around the mean occurrence. Similar results are obtained from CALIOP and the ground-based lidar, with a mean difference in occurrence of ~5% between both instruments. From the ground-based lidar data, a slight decrease in occurrence of ~3% per decade is observed but found statistically insignificant. Based on a clustering analysis of cirrus cloud parameters, three distinct classes have been identified and investigations concerning their origin are discussed. Properties of these different classes are analysed, showing that thin cirrus in the upper troposphere represent ~50% of cloud cover detected in summer and fall, decreasing by 15–20% for other seasons.


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