Abstract. The Multi-sensor Cloud and Aerosol Retrieval Simulator (MCARS) presently
produces synthetic radiance data from Goddard Earth Observing System version
5 (GEOS-5) model output as if the Moderate Resolution Imaging
Spectroradiometer (MODIS) were viewing a combination of atmospheric column
inclusive of clouds, aerosols, and a variety of gases and land–ocean surface
at a specific location. In this paper we use MCARS to study the MODIS
Above-Cloud AEROsol retrieval algorithm (MOD06ACAERO). MOD06ACAERO is
presently a regional research algorithm able to retrieve aerosol optical
thickness over clouds, in particular absorbing biomass-burning aerosols
overlying marine boundary layer clouds in the southeastern Atlantic Ocean.
The algorithm's ability to provide aerosol information in cloudy conditions
makes it a valuable source of information for modeling and climate studies
in an area where current clear-sky-only operational MODIS aerosol retrievals
effectively have a data gap between the months of June and October. We use
MCARS for a verification and closure study of the MOD06ACAERO algorithm. The
purpose of this study is to develop a set of constraints a model developer
might use during assimilation of MOD06ACAERO data. Our simulations indicate that the MOD06ACAERO algorithm performs well for
marine boundary layer clouds in the SE Atlantic provided some specific
screening rules are observed. For the present study, a combination of five
simulated MODIS data granules were used for a dataset of 13.5 million samples
with known input conditions. When pixel retrieval uncertainty was less than
30 %, optical thickness of the underlying cloud layer was greater than 4,
and scattering angle range within the cloud bow was excluded, MOD06ACAERO
retrievals agreed with the underlying ground truth (GEOS-5 cloud and aerosol
profiles used to generate the synthetic radiances) with a slope of 0.913,
offset of 0.06, and RMSE=0.107. When only near-nadir pixels were
considered (view zenith angle within ±20∘) the agreement with
source data further improved (0.977, 0.051, and 0.096 respectively).
Algorithm closure was examined using a single case out of the five used for
verification. For closure, the MOD06ACAERO code was modified to use GEOS-5
temperature and moisture profiles as an ancillary. Agreement of MOD06ACAERO
retrievals with source data for the closure study had a slope of 0.996 with
an offset of −0.007 and RMSE of 0.097 at a pixel uncertainty level of less than
40 %, illustrating the benefits of high-quality ancillary atmospheric data
for such retrievals.