scholarly journals Multiple technical observations of the atmospheric boundary layer structure of a red warning haze episode in Beijing

2019 ◽  
Author(s):  
Yu Shi ◽  
Fei Hu ◽  
Guangqiang Fan ◽  
Zhe Zhang

Abstract. The study and control of air pollution need to detect the structure of atmospheric boundary layer (ABL) in order to understand the mechanism of interaction between atmospheric boundary layer and air pollution. However, when extreme pollution occurs, the detection of atmospheric boundary layer structure is very scarce. Beijing, the capital of China, has experienced a severe haze pollution in December 2016. The city issued its first red air pollution warning of this year (the highest PM2.5 concentration was later monitored to exceed 450 μg m−3). In this paper, the vertical profiles of wind, temperature, humidity and extinction coefficient (reflecting aerosol concentration), as well as ABL heights and turbulence quantities under heavy haze pollution are analyzed, with collected data from Lidar, wind profile radar (WPR), radiosonde, 325-meter meteorological tower (equipped with 7-layer supersonic anemometer and 15-layer low frequency wind, temperature and humidity sensors) and some other ground observations. ABL heights obtained by three different methods based on Lidar extinction coefficient data (Hc) are compared with the heights calculated from radiosonde temperature data (Hθ) and from WPR wind speed data (Hu). The results show that increase of water vapor has greatly promoted the hygroscopic growth of aerosols, the corresponding extinction coefficients also increased significantly. The PBL heights Hθ and Hu of heavy haze pollution day were generally lower than those of clean day, but Hc increased. Turbulent activities were great inhibited during haze pollution, time changes of both friction velocity (u*) and turbulent kinetic energy (TKE) have obvious inverse correlation with that of PM2.5. The results of this paper could provide some reference for the parameterization of the boundary layer height and turbulent diffusion process in the numerical model of severe air pollution.

2019 ◽  
Vol 12 (9) ◽  
pp. 4887-4901 ◽  
Author(s):  
Yu Shi ◽  
Fei Hu ◽  
Guangqiang Fan ◽  
Zhe Zhang

Abstract. The study and control of air pollution involves measuring the structure of the atmospheric boundary layer (ABL) to understand the mechanisms of the interactions occurring between the atmospheric boundary layer and air pollution. Beijing, the capital of China, experienced heavy haze pollution in December 2016, and the city issued its first red-alert air pollution warning of the year (the highest PM2.5 concentrations were later found to exceed 450 µg m−3). In this paper, the vertical profiles of wind, temperature, humidity and the extinction coefficient (reflecting aerosol concentrations), as well as ABL heights and turbulence quantities under heavy haze pollution conditions, are analyzed, with data collected from lidar, wind profile radar (WPR), radiosondes, a 325 m meteorological tower (equipped with a 7-layer ultrasonic anemometer and 15-layer low-frequency wind, temperature, and humidity sensors) and ground observations. The ABL heights obtained by three different methods based on lidar extinction coefficient data (Hc) are compared with the heights calculated from radiosonde temperature data (Hθ), and their correlation coefficient can reach 72 %. Our results show that Hθ measured on heavy haze pollution days was generally lower than that measured on clean days without pollution, but Hc increased from clean to heavy pollution days. The time changes in friction velocity (u*) and turbulent kinetic energy (TKE) were clearly inversely correlated with PM2.5 concentration. Momentum and heat fluxes varied very little with altitude. The nocturnal sensible heat fluxes close to the Earth surface always stay positive. In the daytime of the haze pollution period, sensible heat fluxes were greatly reduced within 300 m of the ground. These findings will deepen our understanding of the boundary layer structure under heavy pollution conditions and improve the boundary layer parameterization in numerical models.


2014 ◽  
Vol 2014 ◽  
pp. 1-14 ◽  
Author(s):  
Lili Wang ◽  
Nan Zhang ◽  
Zirui Liu ◽  
Yang Sun ◽  
Dongsheng Ji ◽  
...  

The air-pollution episodes in China in January 2013 were the most hazardous in the Beijing-Tianjin-Hebei (BTH) region. PM2.5, AOD, and long-term visibility data, along with various climate and meteorological factors and the boundary-layer structure, were used to investigate the cause of the heavy-haze pollution events in January 2013. The result suggests that unfavorable diffusion conditions (weak surface winds and high humidity) and high primary-pollutant emissions have induced heavy-haze pollution in the BTH region over the past two decades. A sudden stratospheric warming (SSW), weak East Asian winter monsoon, a weak Siberian High, weak meridional circulation, southerly wind anomalies in the lower troposphere, and abnormally weak surface winds and high humidity were responsible for the severe haze pollution events, rather than an abrupt increase in emissions. Heavy/severe haze pollution is associated with orographic wind convergence zones along the Taihang and Yanshan Mountains, slight winds (1.7∼2.1 m/s), and high humidity (70%∼90%), which limits the diffusion of pollutants and facilitates the hygroscopic growth of aerosols. Recirculation and regional transport, along with the poorest diffusion conditions and favorable conditions for hygroscopic growth of aerosols and secondary transformation under the high emission, led to explosive growth and the record high hourly average concentration of PM2.5in Beijing.


2021 ◽  
Author(s):  
Hannah Marley ◽  
Kim Dirks ◽  
Andrew Neverman ◽  
Ian McKendry ◽  
Jennifer Salmond

<p><span><span>A brown air pollution haze that forms over some international cities during the winter has been found to be associated with negative health outcomes and high surface air pollution levels. Previous research has demonstrated a well-established link between the structure of the atmospheric boundary layer (ABL) and surface air quality; however, the degree to which the structure of the ABL influences for formation of local-</span></span><span><span>scale</span></span><span><span> brown haze is unknown. Using continuous ceilometer data covering seven consecutive winters, we investigate the influence of the structure of the ABL in relation to surface air pollution and brown haze formation over an urban area of complex coastal terrain in the Southern Hemisphere city of Auckland, New Zealand. Our results suggest the depth and evolution of the ABL has a strong influence on severe brown haze formation. When days with severe brown haze are compared with those when brown haze is expected but not observed (based on favorable meteorology and high surface air pollution levels), days with severe brown haze are found to coincide with significantly shallower daytime convective boundary layers (~ 48% lower), and the nights preceding brown haze formation are found to have significantly shallower nocturnal boundary layers (~ 28% lower). On severe brown haze days the growth rate during the morning transition phase from a nocturnal boundary layer to a convective daytime boundary layer is found to be significantly reduced (70 m h</span></span><sup><span><span>-1</span></span></sup><span><span>) compared to days on which brown haze is expected but not observed (170 m h</span></span><sup><span><span>-1</span></span></sup><span><span>). Compared with moderate brown haze, severe brown haze conditions are found to be associated with a significantly higher proportion of days with a distinct residual layer present in the ceilometer profiles, suggesting the entrainment of residual layer pollutants may contribute to the severity of the haze. This study illustrates the complex interaction between the ABL structure, air pollution, and the presence of brown haze, and demonstrates the utility of a ceilometer instrument in understanding and predicting the occurrence of brown haze events. </span></span></p>


2020 ◽  
Vol 13 (12) ◽  
pp. 6965-6987
Author(s):  
Jae-Sik Min ◽  
Moon-Soo Park ◽  
Jung-Hoon Chae ◽  
Minsoo Kang

Abstract. Accurate boundary layer structure and height are critical in the analysis of the features of air pollutants and local circulation. Although surface-based remote sensing instruments provide a high temporal resolution of the boundary layer structure, there are numerous uncertainties in terms of the accurate determination of the atmospheric boundary layer heights (ABLHs). In this study, an algorithm for an integrated system for ABLH estimation (ISABLE) was developed and applied to the vertical profile data obtained using a ceilometer and a microwave radiometer in Seoul city, Korea. A maximum of 19 ABLHs were estimated via the conventional time-variance, gradient, wavelet, and clustering methods using the backscatter coefficient from the ceilometer. Meanwhile, several stable boundary layer heights were extracted through near-surface inversion and environmental lapse rate methods using the potential temperature from the microwave radiometer. The ISABLE algorithm can find an optimal ABLH from post-processing, such as k-means clustering and density-based spatial clustering of applications with noise (DBSCAN) techniques. It was found that the ABLH determined using ISABLE exhibited more significant correlation coefficients and smaller mean bias and root mean square error between the radiosonde-derived ABLHs than those obtained using the most conventional methods. Clear skies exhibited higher daytime ABLH than cloudy skies, and the daily maximum ABLH was recorded in summer because of the more intense radiation. The ABLHs estimated by ISABLE are expected to contribute to the parameterization of vertical diffusion in the atmospheric boundary layer.


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