scholarly journals Impact of aerosols on photovoltaic energy production using a spectrally resolved model chain: A case study for Sub-Sahara West-Africa

2021 ◽  
Author(s):  
Stefanie Meilinger ◽  
Anna Herman-Czezuch ◽  
Armelle Zemo Mekeng ◽  
Nicola Kimiaie ◽  
James Barry
Keyword(s):  
Optical Properties ◽  
West Africa ◽  
Biomass Burning ◽  
Energy Production ◽  
Mineral Dust ◽  
Power Reduction ◽  
Photovoltaic Power ◽  
Spectrally Resolved ◽  
Model Chain

<p>West Africa has a great potential for the application of solar energy systems, as it combines high levels of solar irradiance with a lack of energy production. Southern West Africa is a region with a very high aerosol load. Urbanization, uncontrolled fires, traffic as well as power plants and oil rigs lead to increasing anthropogenic emissions. The naturally circulating north winds bring mineral dust from the Sahel and Sahara and monsoons - sea salt and other oceanic compounds from the south. The EU-funded Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa (DACCIWA) project (2014–2018), dlivered the most complete dataset of the atmosphere over the region to date. In our study, we use in-situ measured optical properties of aerosols from the airborne campaign over the Gulf of Guinea and inland, and from ground measurements in coastal cities.</p> <p>Based on an analysis of the aerosol optical properties form the DACCIWA measurement campaign, the impact of aerosol on PV power is investigated for polycrystalline silicon and amorphous silicon technology using a spectrally resolved model chain. The model considers both spectral effects on global irradiance due to different aerosol properties as well as the spectral response of different PV technologies. First, the contribution of various aerosol types (mineral dust, biomass burning and anthropogenic pollution) derived from a post-project classification is studied. Subsequently, differences between these imaginary aerosol scenarios and a real case during a biomass burning outbreak on July 13, 2016 in Benin are presented. The results show that aerosol emissions due to the biomass outbreak on the day of the case study in Cotonou lead to solar flux losses of up to 55% and photovoltaic power reduction of up to 81% for the polycrystalline cell and 78% for the amorphous cell. The relative impact of aerosols differs depending on aerosol type and concentration, being larger for low solar zenith angles than at noon. For the situation studied in Cotonou, Benin, we are able to show that the inclusion of spectral aspects leads to a significant effect when calculating the PV power. Comparing the effects of aerosols on the photovoltaic power of the two technologies, we find that the amorphous cell suffers a greater reduction in power during the morning and evening hours - when there is more diffuse irradiance - of 36% than the polycrystalline cell (27%). Conversely, in the middle of the day, we observe greater PV power reduction of the polycrystalline cell of 12% compared to the amorphous cell (8%).</p> <p><strong>Acknowledgements:</strong> Funding was provided by  the German BMWi under contract 0350009A and BMBF under contract 03SF0567A-.</p>

scholarly journals Detection of Saharan dust and biomass burning events using near real-time intensive aerosol optical properties in the northwestern Mediterranean

2016 ◽  
Author(s):  
M. Ealo ◽  
A. Alastuey ◽  
A. Ripoll ◽  
N. Pérez ◽  
M. C. Minguillón ◽  
...  
Keyword(s):  
Optical Properties ◽  
Biomass Burning ◽  
Mineral Dust ◽  
Organic Aerosol ◽  
Saharan Dust ◽  
Aerosol Optical Properties ◽  
Angstrom Exponent ◽  
Ångström Exponent ◽  
Dust Events ◽  
Ångstrom Exponent

Abstract. The study of Saharan dust events (SDE) and biomass burning (BB) emissions are both topic of great scientific interest since they are frequent and important polluting scenarios affecting air quality and climate. The main aim of this work is evaluating the feasibility of using near real-time in situ aerosol optical measurements for the detection of these atmospheric events in the Western Mediterranean Basin (WMB). With this aim, intensive aerosol optical properties (SAE: scattering Ångström exponent, AAE: absorption Ångström exponent, SSAAE: single scattering albedo Ångström exponent, and g: asymmetry parameter) were derived from multi-wavelength aerosol light scattering, hemispheric backscattering and absorption measurements performed at regional (Montseny; MSY, 720 m a.s.l.) and continental (Montsec; MSA, 1570 m a.s.l.) background sites in the WMB. A sensitivity study aiming at calibrating the measured intensive optical properties for SDE and BB detection is presented and discussed. The detection of Saharan dust events (SDE) by means of the SSAAE parameter and Ångström matrix depended on the altitude of the measurement station, and on SDE intensity. At MSA (mountain-top site) SSAAE detected around 85% of SDE compared with 50% at MSY station, where pollution episodes dominated by fine anthropogenic particles frequently masked the effect of mineral dust on optical properties during less intense SDE. Furthermore, an interesting feature of SSAAE was its capability to detect the presence of mineral dust after the end of SDE. Thus, resuspension processes driven by summer regional atmospheric circulations and dry conditions after SDE favored the accumulation of mineral dust at regional level having important consequences for air quality. On average, SAE, AAE and g ranged between -0.7 and 1, 1.3 and 2.5, and 0.5 and 0.75, respectively, during SDE. Based on the Aethalometer model, biomass burning (BB) contribution to equivalent black carbon (BC) accounted for 36% and 40% at MSY and MSA respectively. Linear relationships were found between AAE and %BCbb, with AAE values reaching around 1.5 when %BCbb was higher than 50%. BB contribution to organic matter (OM) at MSY was around 30%. Thus FF combustion sources showed important contributions to both BC and OM in the region under study. Results for OM source apportionment showed good agreement with simultaneous biomass burning organic aerosol (BBOA) and hydrocarbon-like organic aerosol (HOA) calculated from Positive Matrix Factorization (PMF) applied to simultaneous Aerosol Mass Spectrometer (ACSM) measurements. A wildfire episode was identified at MSY, showing AAE values up to 2 when daily BB contributions to BC and OM were 73% and 78% respectively.

scholarly journals Overview of aerosol optical properties over southern West Africa from DACCIWA aircraft measurements

2020 ◽  
Vol 20 (8) ◽  
pp. 4735-4756 ◽  
Author(s):  
Cyrielle Denjean ◽  
Thierry Bourrianne ◽  
Frederic Burnet ◽  
Marc Mallet ◽  
Nicolas Maury ◽  
...  
Keyword(s):  
Optical Properties ◽  
West Africa ◽  
Black Carbon ◽  
Biomass Burning ◽  
Aerosol Particles ◽  
Anthropogenic Pollution ◽  
Aerosol Optical Properties ◽  
Air Masses ◽  
Carbon Particles ◽  
Biomass Burning Particles

Abstract. Southern West Africa (SWA) is an African pollution hotspot but a relatively poorly sampled region of the world. We present an overview of in situ aerosol optical measurements collected over SWA in June and July 2016 as part as of the DACCIWA (Dynamics-Aerosol-Chemistry-Clouds Interactions in West Africa) airborne campaign. The aircraft sampled a wide range of air masses, including anthropogenic pollution plumes emitted from the coastal cities, long-range transported biomass burning plumes from central and southern Africa and dust plumes from the Sahara and Sahel region, as well as mixtures of these plumes. The specific objective of this work is to characterize the regional variability of the vertical distribution of aerosol particles and their spectral optical properties (single scattering albedo: SSA, asymmetry parameter, extinction mass efficiency, scattering Ångström exponent and absorption Ångström exponent: AAE). The first findings indicate that aerosol optical properties in the planetary boundary layer were dominated by a widespread and persistent biomass burning loading from the Southern Hemisphere. Despite a strong increase in aerosol number concentration in air masses downwind of urban conglomerations, spectral SSA were comparable to the background and showed signatures of the absorption characteristics of biomass burning aerosols. In the free troposphere, moderately to strongly absorbing aerosol layers, dominated by either dust or biomass burning particles, occurred occasionally. In aerosol layers dominated by mineral dust particles, SSA varied from 0.81 to 0.92 at 550 nm depending on the variable proportion of anthropogenic pollution particles externally mixed with the dust. For the layers dominated by biomass burning particles, aerosol particles were significantly more light absorbing than those previously measured in other areas (e.g. Amazonia, North America), with SSA ranging from 0.71 to 0.77 at 550 nm. The variability of SSA was mainly controlled by variations in aerosol composition rather than in aerosol size distribution. Correspondingly, values of AAE ranged from 0.9 to 1.1, suggesting that lens-coated black carbon particles were the dominant absorber in the visible range for these biomass burning aerosols. Comparison with the literature shows a consistent picture of increasing absorption enhancement of biomass burning aerosol from emission to remote location and underscores that the evolution of SSA occurred a long time after emission. The results presented here build a fundamental basis of knowledge about the aerosol optical properties observed over SWA during the monsoon season and can be used in climate modelling studies and satellite retrievals. In particular and regarding the very high absorbing properties of biomass burning aerosols over SWA, our findings suggest that considering the effect of internal mixing on absorption properties of black carbon particles in climate models should help better assess the direct and semi-direct radiative effects of biomass burning particles.

scholarly journals Variability of aerosol vertical distribution in the Sahel

2010 ◽  
Vol 10 (24) ◽  
pp. 12005-12023 ◽  
Author(s):  
O. Cavalieri ◽  
F. Cairo ◽  
F. Fierli ◽  
G. Di Donfrancesco ◽  
M. Snels ◽  
...  
Keyword(s):  
Optical Properties ◽  
West Africa ◽  
Vertical Distribution ◽  
Southern Hemisphere ◽  
Biomass Burning ◽  
Dry Season ◽  
Aerosol Transport ◽  
Air Masses ◽  
Monsoon Flow ◽  
Biomass Burning Aerosol

Abstract. In this work, we have studied the seasonal and inter-annual variability of the aerosol vertical distribution over Sahelian Africa for the years 2006, 2007 and 2008, characterizing the different kind of aerosols present in the atmosphere in terms of their optical properties observed by ground-based and satellite instruments, and their sources searched for by using trajectory analysis. This study combines data acquired by three ground-based micro lidar systems located in Banizoumbou (Niger), Cinzana (Mali) and M'Bour (Senegal) in the framework of the African Monsoon Multidisciplinary Analysis (AMMA), by the AEROsol RObotic NETwork (AERONET) sun-photometers and by the space-based Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard the CALIPSO satellite (Cloud-Aerosol Lidar and Infrared Pathfinder Observations). During winter, the lower levels air masses arriving in the Sahelian region come mainly from North, North-West and from the Atlantic area, while in the upper troposphere air flow generally originates from West Africa, crossing a region characterized by the presence of large biomass burning sources. The sites of Cinzana, Banizoumbou and M'Bour, along a transect of aerosol transport from East to West, are in fact under the influence of tropical biomass burning aerosol emission during the dry season, as revealed by the seasonal pattern of the aerosol optical properties, and by back-trajectory studies. Aerosol produced by biomass burning are observed mainly during the dry season and are confined in the upper layers of the atmosphere. This is particularly evident for 2006, which was characterized by a large presence of biomass burning aerosols in all the three sites. Biomass burning aerosol is also observed during spring when air masses originating from North and East Africa pass over sparse biomass burning sources, and during summer when biomass burning aerosol is transported from the southern part of the continent by the monsoon flow. During summer months, the entire Sahelian region is under the influence of Saharan dust aerosols: the air masses in low levels arrive from West Africa crossing the Sahara desert or from the Southern Hemisphere crossing the Guinea Gulf while in the upper layers air masses still originate from North, North-East. The maximum of the desert dust activity is observed in this period which is characterized by large AOD (above 0.2) and backscattering values. It also corresponds to a maximum in the extension of the aerosol vertical distribution (up to 6 km of altitude). In correspondence, a progressive cleaning up of the lowermost layers of the atmosphere is occurring, especially evident in the Banizoumbou and Cinzana sites. Summer is in fact characterized by extensive and fast convective phenomena. Lidar profiles show at times large dust events loading the atmosphere with aerosol from the ground up to 6 km of altitude. These events are characterized by large total attenuated backscattering values, and alternate with very clear profiles, sometimes separated by only a few hours, indicative of fast removal processes occurring, likely due to intense convective and rain activity. The inter-annual variability in the three year monitoring period is not very significant. An analysis of the aerosol transport pathways, aiming at detecting the main source regions, revealed that air originated from the Saharan desert is present all year long and it is observed in the lower levels of the atmosphere at the beginning and at the end of the year. In the central part of the year it extends upward and the lower levels are less affected by air masses from Saharan desert when the monsoon flow carries air from the Guinea Gulf and the Southern Hemisphere inland.

scholarly journals Physical and optical properties of mineral dust aerosol during the Dust and Biomass-burning Experiment

2008 ◽  
Vol 113 ◽  
Author(s):  
S. R. Osborne ◽  
B. T. Johnson ◽  
J. M. Haywood ◽  
A. J. Baran ◽  
M. A. J. Harrison ◽  
...  
Keyword(s):  
Optical Properties ◽  
Biomass Burning ◽  
Mineral Dust ◽  
Dust Aerosol

scholarly journals Light absorption properties of aerosols over Southern West Africa

2019 ◽  
Author(s):  
Cyrielle Denjean ◽  
Thierry Bourrianne ◽  
Frederic Burnet ◽  
Marc Mallet ◽  
Nicolas Maury ◽  
...  
Keyword(s):  
Optical Properties ◽  
West Africa ◽  
Biomass Burning ◽  
Aerosol Particles ◽  
Anthropogenic Pollution ◽  
Absorption Properties ◽  
Air Masses ◽  
Carbon Particles ◽  
Biomass Burning Aerosol ◽  
Biomass Burning Particles

Abstract. Southern West Africa (SWA) is an African pollution hotspot but a relatively poorly sampled region of the world. We present an overview of in-situ aerosol optical measurements collected over SWA in June and July 2016 as part as the DACCIWA (Dynamics–Aerosol–Chemistry–Clouds Interactions in West Africa) airborne campaign. The aircraft sampled a wide range of air masses, including anthropogenic pollution plumes emitted from the coastal cities, long-range transported biomass burning plumes from Central and Southern Africa and dust plumes from the Sahara and Sahel region, as well as mixtures of these plumes. The specific objective of this work is to characterize the regional variability of the vertical distribution of aerosol particles and their spectral optical properties (single scattering albedo: SSA, asymmetry parameter, extinction mass efficiency, scattering Ångström exponent and absorption Ångström exponent: AAE). First findings indicate that aerosol optical properties in the planetary boundary layer were dominated by a widespread and persistent biomass burning loading from the Southern Hemisphere. Despite a strong increase of aerosol number concentration in air masses downwind of urban conglomerations, spectral SSA were comparable to the background and showed signatures of the absorption characteristics of biomass burning aerosols. In the free troposphere, moderately to strongly absorbing aerosol layers, dominated by either dust or biomass burning particles, occurred occasionally. In aerosol layers dominated by mineral dust particles, SSA varied from 0.81 to 0.92 at 550 nm depending on the variable proportion of anthropogenic pollution particles externally mixed with the dust. Biomass burning aerosol particles were significantly more light absorbing than those previously measured in other areas (e.g. Amazonia, North America) with SSA ranging from 0.71 to 0.77 at 550 nm. The variability of SSA was mainly controlled by variations in aerosol composition rather than in aerosol size distribution. Correspondingly, values of AAE ranged from 0.9 to 1.1, suggesting that lens-coated black carbon particles were the dominant absorber in the visible range for these biomass burning aerosols. Comparison with literature shows a consistent picture of increasing absorption enhancement of biomass burning aerosol from emission to remote location and underscores that the evolution of SSA occurred a long time after emission. The results presented here build a fundamental basis of knowledge about the aerosol optical properties observed over SWA during the monsoon season and can be used in climate modelling studies and satellite retrievals. In particular and regarding the very high absorbing properties of biomass burning aerosols over SWA, our findings suggest that considering the effect of internal mixing on absorption properties of black carbon particles in climate models should help better assessing the direct and semi-direct radiative effects of biomass burning particles.

scholarly journals Long-term simulations (2001–2006) of biomass burning and mineral dust optical properties over West Africa: comparisons with new satellite retrievals

2011 ◽  
Vol 11 (10) ◽  
pp. 28587-28626 ◽  
Author(s):  
F. Malavelle ◽  
M. Mallet ◽  
V. Pont ◽  
C. Liousse ◽  
F. Solmon
Keyword(s):  
Remote Sensing ◽  
Optical Properties ◽  
West Africa ◽  
Biomass Burning ◽  
Hydrological Cycle ◽  
Regional Scale ◽  
Aerosol Optical Properties ◽  
Deep Blue ◽  
Satellite Retrievals

Abstract. The West African region is characterized by large concentrations of smoke and biomass burning aerosols, which could significantly modify the regional radiative budget and the hydrological cycle. Here, we propose long-term (2001–2006) RegCM simulations of aerosol optical properties over West Africa together with their spectral dependences. Results of simulations are evaluated at local and regional scale by using surface network (AERONET/PHOTON) and remote sensing observations (MODIS, MISR, OMI) especially during the dry season, December-January-February, DJF. New original satellite retrievals are tested and compared to RegCM simulations. Concerning AOD, we obtain values in agreement with AERONET/PHOTON observations at the local scale but some differences clearly appear between simulated AOD and regional MISR, OMI and MODIS view, especially over (1) the central Africa and (2) the gulf of Guinea during DJF. Concerning simulated SSA (for visible wavelengths), our results display (1) comparable values with level 2 AERONET/PHOTON local observations together with (2) non negligible differences with satellite (MODIS Deep blue, OMI and MISR products) observations. In most cases, satellite SSA is found to be higher than those simulated by RegCM and retrieved through AERONET/PHOTON network. In parallel, we also note significant differences on retrieved SSA from each satellite (OMI, MISR, MODIS Deep Blue) remote sensing techniques over this specific region. Finally, our work highlights that the spectral dependence of aerosol optical properties is a useful parameter to adapt so that modeled simulations should be be better evaluated and constrained.

Impact of biomass burning on regional aerosol optical properties: A case study over northern India

2019 ◽  
Vol 244 ◽  
pp. 328-343 ◽  
Author(s):  
Darga Saheb Shaik ◽  
Yogesh Kant ◽  
Debashis Mitra ◽  
Atinderpal Singh ◽  
H.C. Chandola ◽  
...  
Keyword(s):  
Optical Properties ◽  
Biomass Burning ◽  
Aerosol Optical Properties ◽  
Northern India

scholarly journals Detection of Saharan dust and biomass burning events using near-real-time intensive aerosol optical properties in the north-western Mediterranean

2016 ◽  
Vol 16 (19) ◽  
pp. 12567-12586 ◽  
Author(s):  
Marina Ealo ◽  
Andrés Alastuey ◽  
Anna Ripoll ◽  
Noemí Pérez ◽  
María Cruz Minguillón ◽  
...  
Keyword(s):  
Optical Properties ◽  
Biomass Burning ◽  
Mineral Dust ◽  
Organic Aerosol ◽  
Western Mediterranean ◽  
Saharan Dust ◽  
Aerosol Optical Properties ◽  
Angstrom Exponent ◽  
Ångström Exponent ◽  
Ångstrom Exponent

Abstract. The study of Saharan dust events (SDEs) and biomass burning (BB) emissions are both topics of great scientific interest since they are frequent and important polluting scenarios affecting air quality and climate. The main aim of this work is evaluating the feasibility of using near-real-time in situ aerosol optical measurements for the detection of these atmospheric events in the western Mediterranean Basin (WMB). With this aim, intensive aerosol optical properties (SAE: scattering Ångström exponent, AAE: absorption Ångström exponent, SSAAE: single scattering albedo Ångström exponent and g: asymmetry parameter) were derived from multi-wavelength aerosol light scattering, hemispheric backscattering and absorption measurements performed at regional (Montseny; MSY, 720 m a.s.l.) and continental (Montsec; MSA, 1570 m a.s.l.) background sites in the WMB. A sensitivity study aiming at calibrating the measured intensive optical properties for SDEs and BB detection is presented and discussed. The detection of SDEs by means of the SSAAE parameter and Ångström matrix (made up by SAE and AAE) depended on the altitude of the measurement station and on SDE intensity. At MSA (mountain-top site) SSAAE detected around 85 % of SDEs compared with 50 % at the MSY station, where pollution episodes dominated by fine anthropogenic particles frequently masked the effect of mineral dust on optical properties during less intense SDEs. Furthermore, an interesting feature of SSAAE was its capability to detect the presence of mineral dust after the end of SDEs. Thus, resuspension processes driven by summer regional atmospheric circulations and dry conditions after SDEs favoured the accumulation of mineral dust at regional level having important consequences for air quality. On average, SAE, AAE and g ranged between −0.7 and 1, 1.3 and 2.5 and 0.5 and 0.75 respectively during SDEs. Based on the aethalometer model, BB contribution to equivalent black carbon (BC) accounted for 36 and 40 % at MSY and MSA respectively. Linear relationships were found between AAE and %BCbb, with AAE values reaching around 1.5 when %BCbb was higher than 50 %. BB contribution to organic matter (OM) at MSY was around 30 %. Thus fossil fuel (FF) combustion sources showed important contributions to both BC and OM in the region under study. Results for OM source apportionment showed good agreement with simultaneous biomass burning organic aerosol (BBOA) and hydrocarbon-like organic aerosol (HOA) obtained by applying a positive matrix factorization model (PMF) to simultaneous Aerosol Chemical Speciation Monitor (ACSM) measurements. A wildfire episode was identified at MSY, showing AAE values up to 2 when daily BB contributions to BC and OM were 73 and 78 % respectively.

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