Aerosols Direct Radiative Effects Combined Ground-Based Lidar and Sun-Photometer Observations: Cases Comparison between Haze and Dust Events in Beijing

Aerosols can affect vertical thermal structure during heavily polluted episodes (HPEs). Here, we selected four typical HPEs in 2018, which were further subdivided into dust and haze events. The vertical distribution of aerosols extinction coefficient (EC) and variations in columnar optical properties were investigated based on sun-photometer and Lidar observation at an urban site in Beijing. The vertical characteristics in shortwave radiative heating rate (HR) of aerosols were studied using NASA/Goddard radiative transfer model along with observational data. In the haze episode, EC layer is less than 1.5 km and shows strong scattering, with single-scattering albedo (SSA440nm) of ~0.97. The heating effects are observed at the middle and upper atmosphere, and slight heating effects are found at the lower layer. The mean HR within 1.5 km can be up to 16.3 K day−1 with EC of 1.27 km−1, whereas the HR within 0.5 km is only 1.3 K day−1. In the dust episode, dust aerosols present the absorption with SSA440nm of ~0.88, which would heat the lower atmosphere to promote vertical turbulence, and the height of EC layer can be up to 2.0–3.5 km. In addition, the strong heating effects of dust layer produced cooling effects near the surface. Therefore, the accurate measurement of aerosols optical properties in HPEs is of great significance for modeling aerosols direct radiative effects.

Contrasting source contributions of Arctic black carbon to atmospheric concentrations, deposition flux, and atmospheric and snow radiative effects

Black carbon (BC) particles in the Arctic contribute to rapid warming of the Arctic by heating the atmosphere and snow and ice surfaces. Understanding the source contributions to Arctic BC is therefore important, but they are not well understood, especially those for atmospheric and snow radiative effects. Here we estimate simultaneously the source contributions of Arctic BC to near-surface and vertically integrated atmospheric BC mass concentrations (MBC_SRF and MBC_COL), BC deposition flux (MBC_DEP), and BC radiative effects at the top of the atmosphere and snow surface (REBC_TOA and REBC_SNOW), and show that the source contributions to these five variables are highly different. In our estimates, Siberia makes the largest contribution to MBC_SRF, MBC_DEP, and REBC_SNOW in the Arctic (defined as > 70° N), accounting for 70 %, 53 %, and 43 %, respectively. In contrast, Asia’s contributions to MBC_COL and REBC_TOA are largest, accounting for 38 % and 45 %, respectively. In addition, the contributions of biomass burning sources are larger (24−34 %) to MBC_DEP, REBC_TOA, and REBC_SNOW, which are highest from late spring to summer, and smaller (4.2−14 %) to MBC_SRF and MBC_COL, whose concentrations are highest from winter to spring. These differences in source contributions to these five variables are due to seasonal variations in BC emission, transport, and removal processes and solar radiation, as well as to differences in radiative effect efficiency (radiative effect per unit BC mass) among sources. Radiative effect efficiency varies by a factor of up to 4 among sources (1465−5439 W g–1) depending on lifetimes, mixing states, and heights of BC and seasonal variations of emissions and solar radiation. As a result, source contributions to radiative effects and mass concentrations (i.e., REBC_TOA and MBC_COL, respectively) are substantially different. The results of this study demonstrate the importance of considering differences in the source contributions of Arctic BC among mass concentrations, deposition, and atmospheric and snow radiative effects for accurate understanding of Arctic BC and its climate impacts.

Solar radiation in the cloud-free atmosphere

<p>The quantification of Earth’s solar radiation budget and its temporal changes is essential for the understanding of the genesis and evolution of climate on our planet. While the solar radiative fluxes in and out of the climate system can be accurately tracked and quantified from space by satellite programs such as CERES or SORCE, the disposition of solar energy within in the climate system is afflicted with larger uncertainties. A better quantification of the solar radiative fluxes not only under cloudy, but also under cloud-free conditions can help to reduce these uncertainties and is essential for example for the determination of cloud radiative effects or for the understanding of  temporal changes in the solar radiative components of the climate system.</p> <p>We combined satellite observations of Top of Atmosphere fluxes with the information contained in surface flux observations and climate models to infer the absorption of solar radiation in the atmosphere, which we estimated at 73 Wm<sup>-2</sup> globally under cloud-free conditions (Wild et al. 2019 Clim Dyn). The latest generation of climate models participating in CMIP6 is now able to reproduce this magnitude surprisingly well, whereas in previous climate model  generations the cloud-free atmosphere was typically too transparent for solar radiation, which stated a long-standing modelling issue (Wild 2020 Clim Dyn, Wild et al. 1995 JClim).</p> <p>With respect to changes in solar fluxes, there is increasing evidence that the substantial long-term decadal variations in surface solar radiation known as dimming and brightening occur not only under all-sky, but similarly also under clear-sky conditions (Manara et al. 2016 ACP, Yang et al. 2019 JClim; Wild et al. 2021 GRL). This points to aerosol radiative effects as major factor for the explanation of this phenomenon.</p>

Environmental Response in Coupled Energy and Water Cloud Impact Parameters Derived from A-Train Satellite, ERA-Interim and MERRA-2

Understanding the connections between latent heating from precipitation and cloud radiative effects is essential for accurately parameterizing cross-scale links between cloud microphysics and global energy and water cycles in climate models. While commonly examined separately, this study adopts two cloud impact parameters (CIPs), the surface radiative cooling efficiency, Rc, and atmospheric radiative heating efficiency, Rh, that explicitly couple cloud radiative effects and precipitation to characterize how efficiently precipitating cloud systems influence the energy budget and water cycle using A-Train observations and two reanalyses. These CIPs exhibit distinct global distributions that suggest cloud energy and water cycle coupling are highly dependent on cloud regime. The dynamic regime (ω500) controls the sign of Rh, while column water vapor (CWV) appears to be the larger control on the magnitude. The magnitude of Rc is highly coupled to the dynamic regime. Observations show that clouds cool the surface very efficiently per unit rainfall at both low and high sea surface temperature (SST) and CWV, but reanalyses only capture the former. Reanalyses fail to simulate strong Rh and moderate Rc in deep convection environments but produce stronger Rc and Rh than observations in shallow, warm rain systems in marine stratocumulus regions. While reanalyses generate fairly similar climatologies in the frequency of environmental states, the response of Rc and Rh to SST and CWV results in systematic differences in zonal and meridional gradients of cloud atmospheric heating and surface cooling relative to A-Train observations that may have significant implications for global circulations and cloud feedbacks.

Method to quantify black carbon aerosol light absorption enhancement with a mixing state index

Large uncertainties remain when estimating the warming effects of ambient black carbon (BC) aerosols on climate. One of the key challenges in modeling the radiative effects is predicting the BC light absorption enhancement, which is mainly determined by the mass ratio (MR) of non-BC coating material to BC in the population of BC-containing aerosols. For the same MR, recent research has found that the radiative absorption enhancements by BC are also controlled by its particle-to-particle heterogeneity. In this study, the BC mixing state index (χ) is developed to quantify the dispersion of ambient black carbon aerosol mixing states based on binary systems of BC and other non-black carbon components. We demonstrate that the BC light absorption enhancement increases with χ for the same MR, which indicates that χ can be employed as a factor to constrain the light absorption enhancement of ambient BC. Our framework can be further used in the model to study the radiative effects of black carbon on climate change.