scholarly journals Supplementary material to "The Vulcan Version 3.0 High-Resolution Fossil Fuel CO<sub>2</sub> Emissions for the United States"

Author(s):  
Kevin R. Gurney ◽  
Jianming Liang ◽  
Risa Patarasuk ◽  
Yang Song ◽  
Jianhua Huang ◽  
...  
2020 ◽  
Vol 125 (19) ◽  
Author(s):  
Kevin R. Gurney ◽  
Jianming Liang ◽  
Risa Patarasuk ◽  
Yang Song ◽  
Jianhua Huang ◽  
...  

2009 ◽  
Vol 43 (14) ◽  
pp. 5535-5541 ◽  
Author(s):  
Kevin R. Gurney ◽  
Daniel L. Mendoza ◽  
Yuyu Zhou ◽  
Marc L. Fischer ◽  
Chris C. Miller ◽  
...  

2019 ◽  
Author(s):  
Kevin R. Gurney ◽  
Jianming Liang ◽  
Risa Patarasuk ◽  
Yang Song ◽  
Jianhua Huang ◽  
...  

Abstract. Estimates of greenhouse gas emissions, quantified at fine space and time scales, has become a critical component of new multi-constraint flux information systems in addition to providing relevant information to decisionmakers when considering GHG mitigation opportunities. The Vulcan Project is an effort to estimate bottom-up fossil fuel emissions and CO2 emissions from cement production (FFCO2) for the entire United States landscape at space and time scales that satisfy both scientific and policy needs. Here, we report on version 3.0 of the Vulcan emissions which quantifies FFCO2 emissions for the U.S. at a spatial resolution of 1 km × 1 km and hourly temporal resolution for the 2010–2015 time period. We provide a complete description of the updated methods, data sources, results, and comparison to a global gridded FFCO2 data product. We estimate FFCO2 emissions for the year 2011 of 1589.3 TgC with a 95 % confidence interval of 1299/1917 TgC (+18.3 %/−20.6 %), implying a one-sigma uncertainty of ~&amp;pm;10%. We find that per capita FFCO2 emissions are larger in states dominated by the electricity production and industrial sectors and smaller in states dominated by onroad and residential/commercial building emissions. The center of mass (CoM) of FFCO2 emissions in the US are located in the state of Missouri with mean seasonality that moves on a NE/SW near-elliptical path. Comparison to ODIAC, a global gridded FFCO2 emissions estimate shows large differences in both total emissions (100.1 TgC for year 2011) and spatial patterns. The spatial correlation (R2) between the two data products was 0.38 and the mean absolute difference at the individual gridcell scale was 80.04 %. The Vulcan v3.0 FFCO2 emissions data product offers an immediate high-resolution estimate of emissions in every city within the U.S., providing a large potential savings of time and effort for cities planning to develop self-reported city inventories. The Vulcan v3.0 annual gridded emissions data product can be downloaded from the data repository at Oak Ridge National Laboratory (https://doi.org/10.3334/ORNLDAAC/1741, Gurney et al., 2019).


2020 ◽  
Author(s):  
Ben Orsburn

AbstractThe production of hemp and products derived from these plants that contain zero to trace amounts of the psychoactive cannabinoid tetrahydrocannabidiol (THC) is a rapidly growing new market in the United States. The most common products today contain relatively high concentrations of the compound cannabidiol (CBD). Recent studies have investigated commercial CBD products using targeted assays and have found varying degrees of misrepresentation and contamination of these products. To expand on previous studies, we demonstrate the application of non-targeted screening by high resolution accurate mass spectrometry to more comprehensively identify potential adulterants and contaminants. We find evidence to support previous conclusions that CBD products are commonly misrepresented in terms of cannabinoid concentrations present. Specifically, we observe a wide variation in relative THC concentrations across the product tested, with some products containing 10-fold more relative signal than others. In addition, we find that several products appear to be purposely adulterated with over the counter drugs such as caffeine and melatonin. We also observe multiple small molecule contaminants that are typically linked to improper production or packaging methods in food or pharmaceutical production. Finally, we present high resolution accurate mass spectrometry data and tandem MS/MS fragments supporting the presence of trace amounts of fluorofentanyl in a single mail order CBD product. We conclude that the CBD industry would benefit from more robust testing regulations and that the cannabis testing industry, in general, would benefit from the use of non-targeted screening technologies.


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